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Author:

Xi, Kaibiao (Xi, Kaibiao.) | Hou, Yudong (Hou, Yudong.) (Scholars:侯育冬) | Yu, Xiaole (Yu, Xiaole.) | Zheng, Mupeng (Zheng, Mupeng.) | Zhu, Mankang (Zhu, Mankang.)

Indexed by:

EI Scopus SCIE

Abstract:

Lead-free piezoceramics with a temperature-insensitive figure of merit (FOM = d(2)/epsilon) are urgently required to build a new generation of piezoelectric energy harvesters (PEHs) that can be used for environmental protection and new energy applications. Although (K,Na)NbO3 (KNN)-based ceramics are among the most promising lead-free piezoelectric candidates, the piezoelectric charge constant (d(33)) and dielectric constant (epsilon(r)) of KNN with an individual orthorhombic (O) phase exhibit opposite change trends in a certain temperature range, resulting in FOM with poor temperature stability. To break this bottleneck, a diffuse multiphase coexistence (DMC) strategy is proposed to realize a temperature-insensitive FOM. By constructing a DMC-featured orthorhombic-tetragonal (O-T) phase boundary associated with a hierarchical domain configuration, the temperature-driven synergistic variation of d(33) and epsilon(r) was realized in the 0.965(K0.48Na0.52)NbO3-0.035(Bi0.5Li0.5)ZrO3 (KNN-BLZ) system. Benefiting from an excellent temperature-insensitive FOM, the power density of the cantilever beam-type PEH produced by KNN-BLZ obtained a record value of 865 mu W cm(-3) at 80 degrees C, which was superior to the reported value of approximately 380 mu W cm(-3) for KNN-based PEHs measured at room temperature. These results pave the way for applications of KNN-BLZ piezoceramics, and also greatly impact our understanding of the strong correlations between the thermal stability of DMC structure and temperature-dependent energy-harvesting properties.

Keyword:

Author Community:

  • [ 1 ] [Xi, Kaibiao]Beijing Univ Technol, Coll Mat Sci & Engn, Educ Minist China, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China
  • [ 2 ] [Hou, Yudong]Beijing Univ Technol, Coll Mat Sci & Engn, Educ Minist China, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China
  • [ 3 ] [Yu, Xiaole]Beijing Univ Technol, Coll Mat Sci & Engn, Educ Minist China, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China
  • [ 4 ] [Zheng, Mupeng]Beijing Univ Technol, Coll Mat Sci & Engn, Educ Minist China, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China
  • [ 5 ] [Zhu, Mankang]Beijing Univ Technol, Coll Mat Sci & Engn, Educ Minist China, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China

Reprint Author's Address:

  • [Hou, Yudong]Beijing Univ Technol, Coll Mat Sci & Engn, Educ Minist China, Key Lab Adv Funct Mat, Beijing 100124, Peoples R China;;

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Source :

JOURNAL OF MATERIALS CHEMISTRY A

ISSN: 2050-7488

Year: 2023

Issue: 7

Volume: 11

Page: 3556-3564

1 1 . 9 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:26

Cited Count:

WoS CC Cited Count: 16

SCOPUS Cited Count: 16

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 12

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