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Author:

Bi, Chenghao (Bi, Chenghao.) | Yao, Zhiwei (Yao, Zhiwei.) | Hu, Jingcong (Hu, Jingcong.) | Wang, Xingyu (Wang, Xingyu.) | Zhang, Mengqi (Zhang, Mengqi.) | Tian, Shuyu (Tian, Shuyu.) | Liu, Aqiang (Liu, Aqiang.) | Lu, Yue (Lu, Yue.) | de Leeuw, Nora H. (de Leeuw, Nora H..) | Sui, Manling (Sui, Manling.) | Tian, Jianjun (Tian, Jianjun.)

Indexed by:

EI Scopus SCIE

Abstract:

It is a big challenge to achieve pure-blue (<= 470 nm) perovskite light-emitting diodes (PeLEDs) with high efficiency and stability. Here, we report pure-blue (electroluminescence at 469 nm) PeLEDs with a full width at half-maximum of 21 nm, high external quantum efficiency of 10.3%, luminance of 12 060 cd m-2, and continuous operation half-life of 25 h, representing the state-of-the-art performance. This design is based on strongly quantum confined CsPbBr3 quantum dots (QDs) with suppression of Auger recombination, which was enabled by inorganic ligands, replacing initial organic ligands on the QDs. The inorganic ligand acts as a "capacitor" to alleviate the charge accumulation and reduce the exciton binding energy of the QDs, which suppresses the Auger recombination, resulting in much lower efficiency roll-off of PeLEDs. Thus, the devices maintain high efficiency (>10%) at high luminance (>2000 cd m-2), which is of considerable significance for the display application.

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Author Community:

  • [ 1 ] [Bi, Chenghao]Univ Sci & Technol Beijing, Inst Adv Mat & Technol, Beijing 100083, Peoples R China
  • [ 2 ] [Yao, Zhiwei]Univ Sci & Technol Beijing, Inst Adv Mat & Technol, Beijing 100083, Peoples R China
  • [ 3 ] [Zhang, Mengqi]Univ Sci & Technol Beijing, Inst Adv Mat & Technol, Beijing 100083, Peoples R China
  • [ 4 ] [Tian, Shuyu]Univ Sci & Technol Beijing, Inst Adv Mat & Technol, Beijing 100083, Peoples R China
  • [ 5 ] [Liu, Aqiang]Univ Sci & Technol Beijing, Inst Adv Mat & Technol, Beijing 100083, Peoples R China
  • [ 6 ] [Tian, Jianjun]Univ Sci & Technol Beijing, Inst Adv Mat & Technol, Beijing 100083, Peoples R China
  • [ 7 ] [Hu, Jingcong]Beijing Univ Technol, Inst Microstruct & Properties Adv Mat, Beijing Key Lab Microstruct & Properties Solids, Beijing 100124, Peoples R China
  • [ 8 ] [Lu, Yue]Beijing Univ Technol, Inst Microstruct & Properties Adv Mat, Beijing Key Lab Microstruct & Properties Solids, Beijing 100124, Peoples R China
  • [ 9 ] [Sui, Manling]Beijing Univ Technol, Inst Microstruct & Properties Adv Mat, Beijing Key Lab Microstruct & Properties Solids, Beijing 100124, Peoples R China
  • [ 10 ] [Wang, Xingyu]Univ Leeds, Sch Chem, Leeds LS2 9JT, England
  • [ 11 ] [de Leeuw, Nora H.]Univ Leeds, Sch Chem, Leeds LS2 9JT, England
  • [ 12 ] [de Leeuw, Nora H.]Univ Utrecht, Dept Earth Sci, NL-3584 CB Utrecht, Netherlands
  • [ 13 ] [Tian, Jianjun]Univ Sci & Technol Beijing, Shunde Innovat Sch, Beijing 100083, Peoples R China

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Source :

ACS ENERGY LETTERS

ISSN: 2380-8195

Year: 2022

Page: 731-739

2 2 . 0

JCR@2022

2 2 . 0 0 0

JCR@2022

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 70

SCOPUS Cited Count: 75

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 7

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