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Author:

Yue, Z. (Yue, Z..) | Ji, X. (Ji, X..) | Zhou, W. (Zhou, W..) | Ji, Z. (Ji, Z..) | Guo, F. (Guo, F..)

Indexed by:

EI Scopus SCIE

Abstract:

Due to a lower intrinsic thermal conductivity, Cu2S-based thermoelectric materials are attracting extensive attention. However, they still confront the problem of higher electrical resistivity, which distinctly restricts their thermoelectric application. Herein, we synthesized Ag-incorporated Cu2-xS micro/nano composites using a hydrothermal method. It was found that the doping of Ag nanoparticles could effectively enhance the electrical transport, while the generated nanopores, caused by the sintering of Ag nanoparticles during the SPS process, reduced the thermal conductivity. As a result, a maximum ZT value of ∼1.5 was obtained at 773 K in the Cu2-xAgδS (δ = 0.5%) micro/nano composites, much higher than that of the pristine Cu2-xS micro/nano composites. This work provides a new pathway to boosting thermoelectric performance through microstructural engineering. © 2022

Keyword:

Thermoelectric materials Hydrothermal synthesized Ag-incorporated Cu2-xS Nanopores

Author Community:

  • [ 1 ] [Yue Z.]Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing, 100124, China
  • [ 2 ] [Yue Z.]Key Laboratory of Advanced Functional Materials, Ministry of Education, Beijing University of Technology, Beijing, 100124, China
  • [ 3 ] [Ji X.]Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing, 100124, China
  • [ 4 ] [Ji X.]Key Laboratory of Advanced Functional Materials, Ministry of Education, Beijing University of Technology, Beijing, 100124, China
  • [ 5 ] [Zhou W.]Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing, 100124, China
  • [ 6 ] [Zhou W.]Key Laboratory of Advanced Functional Materials, Ministry of Education, Beijing University of Technology, Beijing, 100124, China
  • [ 7 ] [Ji Z.]Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing, 100124, China
  • [ 8 ] [Ji Z.]Key Laboratory of Advanced Functional Materials, Ministry of Education, Beijing University of Technology, Beijing, 100124, China
  • [ 9 ] [Guo F.]Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing, 100124, China
  • [ 10 ] [Guo F.]Key Laboratory of Advanced Functional Materials, Ministry of Education, Beijing University of Technology, Beijing, 100124, China
  • [ 11 ] [Guo F.]College of Robotics, Beijing Union University, Beijing, 100101, China

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Source :

Ceramics International

ISSN: 0272-8842

Year: 2023

Issue: 5

Volume: 49

Page: 8428-8434

5 . 2 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:26

Cited Count:

WoS CC Cited Count: 0

SCOPUS Cited Count: 5

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 16

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