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Author:

Zhu, Guang Shuo (Zhu, Guang Shuo.) | Zheng, Jia Yu (Zheng, Jia Yu.) | Han, Chang Bao (Han, Chang Bao.) | Zhang, Hao (Zhang, Hao.) | Chang, Peiyu (Chang, Peiyu.) | Zhao, Wen Kang (Zhao, Wen Kang.) | He, Junda (He, Junda.) | Xia, Yi (Xia, Yi.) | Song, Xuemei (Song, Xuemei.) | Yan, Hui (Yan, Hui.)

Indexed by:

Scopus SCIE

Abstract:

Indoor formaldehyde (HCHO) pollution has more and more serious adverse effects on human health, it is urgent to develop a material that can be embedded in the air purifier to achieve HCHO's degradation efficiently. In this work, based on the carrier material of polyurethane foam (PUF) modified by amino groups diethanolamine (DEA), we propose a strategy to prepare a manganese oxide compound catalyst (DEA-MnOx-PUF). During the static testing (C-HCHO: 11.591 ppm, T: 25 degrees C), the catalyst shows higher HCHO removal efficiency (93.9 %) than that of unmodified MnOx-PUF catalyst (88.6 %), and it achieves high HCHO-to-CO2 conversion (68.5 %). Additionally, during the continuous single-pass catalysis testing (C-HCHO: 11.591 ppm, T: 25 degrees C, 240000 mL/(g(cat)h)), HCHO removal efficiency can be maintained around at 95 % within 50 hours. The excellent performance is attributed to the continuous decomposition of intermediates during the catalytic process by amino groups cross-linked on the surface of the catalyst. Based on the block whole MnOx-based catalyst DEA-MnOx-PUF, this work will provide a new route to develop a powerful purifier material with long-term efficient removal of HCHO.

Keyword:

Polyurethane foam (PUF) Amino groups Manganese dioxide (MnOx) Formaldehyde (HCHO) Room temperature

Author Community:

  • [ 1 ] [Zhu, Guang Shuo]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 2 ] [Zheng, Jia Yu]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 3 ] [Han, Chang Bao]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 4 ] [Zhang, Hao]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 5 ] [Zhao, Wen Kang]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 6 ] [He, Junda]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 7 ] [Xia, Yi]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 8 ] [Song, Xuemei]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 9 ] [Yan, Hui]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China
  • [ 10 ] [Chang, Peiyu]Beijing Univ tradit Chinese Med, 11,Beisanhuan East Rd, Beijing 100029, Peoples R China
  • [ 11 ] [He, Junda]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China

Reprint Author's Address:

  • [Han, Chang Bao]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China;;[Xia, Yi]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China;;[Song, Xuemei]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ China, Beijing 100124, Peoples R China;;

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Source :

CHEMISTRYSELECT

ISSN: 2365-6549

Year: 2023

Issue: 9

Volume: 8

2 . 1 0 0

JCR@2022

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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