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Abstract:
To realize the rapid separation of photogenerated carriers in photocatalytic reactions, large-sized porous carbon nanosheets with Pt dots were utilized as cocatalysts and coupled with TiO2 particles to construct photocatalytic systems. The optimized photocatalytic H-2 yield is similar to 108 times higher than that of TiO2, fully demonstrating the important role of large-sized porous carbon nanosheets with Pt dots for fast charge separation. The shift of the main peak in high-resolution X-ray photoelectron spectroscopies (XPS) verifies the electron transfer from TiO2 to porous carbon nanosheets. The dense distribution of photo-induced Pt deposition on porous carbon nanosheets confirms that active centers for H-2 evolution are mainly located on porous carbon nanosheets. Our work here provides the practicability of constructing large-sized conductive materials as cocatalysts for fast charge separation in photocatalytic reactions.
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Source :
SEPARATION AND PURIFICATION TECHNOLOGY
ISSN: 1383-5866
Year: 2023
Volume: 324
8 . 6 0 0
JCR@2022
ESI Discipline: CHEMISTRY;
ESI HC Threshold:20
Cited Count:
WoS CC Cited Count: 12
SCOPUS Cited Count: 20
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 11
Affiliated Colleges: