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Author:

Wang, Xuekai (Wang, Xuekai.) | Wang, Jinshu (Wang, Jinshu.) (Scholars:王金淑) | Li, Jianjun (Li, Jianjun.) | Du, Yucheng (Du, Yucheng.) | Wu, Junshu (Wu, Junshu.) | He, Heng (He, Heng.)

Indexed by:

EI Scopus SCIE

Abstract:

Tetracycline (TC) and arsenic contaminants are two main pollutants in aquaculture and livestock husbandry, and they have drawn worldwide attention. To address this issue, a novel N-doped carbon@magnesium silicate (CMS) was fabricated via a facile and low-cost hydrothermal route, adopting glucose and ammonia as C and N sources, respectively. The synergetic combination of carbon and magnesium silicate makes CMS possess a high surface area of 201 m(2)/g and abundant functional groups. Due to the abundant C- and N-containing functional groups and Mg-containing adsorptive sites, the maximum adsorption capacity values of CMS towards As(V) and TC are 498.75 mg/g and 1228.5 mg/g, respectively. The type of adsorption of As(V) and TC onto CMS is monolayer adsorption. An adsorption kinetic study revealed that the mass transfer and intraparticle process dominates the sorption rate of As(V) and TC adsorption onto CMS, respectively. Various functional groups synthetically participate in the adsorption process through complexion, & pi;-& pi; EDA interactions, and hydrogen bonds. This work provides a one-step, low-cost route to fabricate a N-doped carbonaceous adsorbent with a high surface area and abundant functional groups, which has great potential in the application of practical sewage treatment.

Keyword:

adsorption capacity N-doped carbon diatomite

Author Community:

  • [ 1 ] [Wang, Xuekai]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 2 ] [Wang, Jinshu]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 3 ] [Du, Yucheng]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 4 ] [Wu, Junshu]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 5 ] [He, Heng]Beijing Univ Technol, Fac Mat & Mfg, Key Lab Adv Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 6 ] [Wang, Xuekai]Anhui Univ Sci & Technol, Sch Mat Sci & Engn, Huainan 232001, Peoples R China
  • [ 7 ] [Li, Jianjun]Anhui Univ Sci & Technol, Sch Mat Sci & Engn, Huainan 232001, Peoples R China

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Source :

MATERIALS

Year: 2023

Issue: 15

Volume: 16

3 . 4 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:26

Cited Count:

WoS CC Cited Count: 2

SCOPUS Cited Count: 2

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 4

Affiliated Colleges:

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