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Author:

Xie, Xinchun (Xie, Xinchun.) | Zhang, Yuzhong (Zhang, Yuzhong.) | Liang, Ruosi (Liang, Ruosi.) | Chen, Wei (Chen, Wei.) | Zhang, Peixuan (Zhang, Peixuan.) | Wang, Xuan (Wang, Xuan.) | Zhou, Ying (Zhou, Ying.) | Cheng, Yuan (Cheng, Yuan.) | Liu, Jiumeng (Liu, Jiumeng.)

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EI Scopus SCIE

Abstract:

Heavy haze events occur frequently over northeast China during the winter, despite the successful implementation of the Clean Air Act, which primarily targets fossil fuel sources, in recent years. Agricultural fires have been suggested as one of the main causes of these haze episodes. However, their regional contribution to fine particulate matter (PM2.5) pollution has not been systematically evaluated. In this study, we use the GEOS-Chem model to investigate the role of agricultural fires in heavy haze episodes from December 2018 to March 2019 in Heilongjiang province. Our results show significant discrepancies between the simulated and observed PM2.5 concentrations during severe haze pollution days. By increasing agricultural fire emissions in the GFED4s inventory by a factor of ∼23, we are able to better replicate the haze episodes in the model, indicating a severe under-representation of agricultural fires in the inventory. Furthermore, the baseline simulation overestimates the observed black carbon to organic carbon ratio in Harbin, suggesting a biased emission ratio specified in the inventory. Our assessment underscores that agriculture fires constitute the main cause of the extreme haze episodes during the study period, and a strictly implemented ban would improve air quality with substantial health benefits. © 2024 American Chemical Society.

Keyword:

Particulate emissions Fires Fossil fuels Agriculture Air quality Organic carbon Particles (particulate matter)

Author Community:

  • [ 1 ] [Xie, Xinchun]College of Environmental and Resource Sciences, Zhejiang University, Zhejiang, Hangzhou; 310058, China
  • [ 2 ] [Xie, Xinchun]Key Laboratory of Coastal Environment and Resources of Zhejiang Province, School of Engineering, Westlake University, Zhejiang, Hangzhou; 310030, China
  • [ 3 ] [Xie, Xinchun]Institute of Advanced Technology, Westlake Institute for Advanced Study, Zhejiang, Hangzhou; 310024, China
  • [ 4 ] [Zhang, Yuzhong]Key Laboratory of Coastal Environment and Resources of Zhejiang Province, School of Engineering, Westlake University, Zhejiang, Hangzhou; 310030, China
  • [ 5 ] [Zhang, Yuzhong]Institute of Advanced Technology, Westlake Institute for Advanced Study, Zhejiang, Hangzhou; 310024, China
  • [ 6 ] [Liang, Ruosi]College of Environmental and Resource Sciences, Zhejiang University, Zhejiang, Hangzhou; 310058, China
  • [ 7 ] [Liang, Ruosi]Key Laboratory of Coastal Environment and Resources of Zhejiang Province, School of Engineering, Westlake University, Zhejiang, Hangzhou; 310030, China
  • [ 8 ] [Liang, Ruosi]Institute of Advanced Technology, Westlake Institute for Advanced Study, Zhejiang, Hangzhou; 310024, China
  • [ 9 ] [Chen, Wei]College of Environmental and Resource Sciences, Zhejiang University, Zhejiang, Hangzhou; 310058, China
  • [ 10 ] [Chen, Wei]Key Laboratory of Coastal Environment and Resources of Zhejiang Province, School of Engineering, Westlake University, Zhejiang, Hangzhou; 310030, China
  • [ 11 ] [Chen, Wei]Institute of Advanced Technology, Westlake Institute for Advanced Study, Zhejiang, Hangzhou; 310024, China
  • [ 12 ] [Zhang, Peixuan]Key Laboratory of Coastal Environment and Resources of Zhejiang Province, School of Engineering, Westlake University, Zhejiang, Hangzhou; 310030, China
  • [ 13 ] [Zhang, Peixuan]Institute of Advanced Technology, Westlake Institute for Advanced Study, Zhejiang, Hangzhou; 310024, China
  • [ 14 ] [Zhang, Peixuan]Fudan University, Shanghai; 200437, China
  • [ 15 ] [Wang, Xuan]School of Energy and Environment, City University of Hong Kong, Tong, Kowloon; 999077, Hong Kong
  • [ 16 ] [Zhou, Ying]Key Laboratory of Beijing on Regional Air Pollution Control, Faculty of Environment and Life, Beijing University of Technology, Beijing; 100124, China
  • [ 17 ] [Cheng, Yuan]State Key Laboratory of Urban Water Resource and Environment, School of Environment, Harbin Institute of Technology, Harbin; 150090, China
  • [ 18 ] [Liu, Jiumeng]State Key Laboratory of Urban Water Resource and Environment, School of Environment, Harbin Institute of Technology, Harbin; 150090, China

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Source :

Environmental Science and Technology Letters

Year: 2024

Issue: 2

Volume: 11

Page: 150-157

Cited Count:

WoS CC Cited Count: 0

SCOPUS Cited Count: 5

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 4

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