Tetrabromobisphenol　A　(TBBPA)　is　a　kind　of　widely　used　brominated　flame　retardant　(BFR),　which　is　proven　to　be　harmful　to　ecological　systems　and　public　health.　It　is　very　important　to　remove　TBBPA　from　the　environment.　In　our　study,　a　magnetic　composite　named　Fe3O4/GO/ZIF-67　was　synthesized　by　a　coprecipitation　method　and　applied　in　the　highly　efficient　adsorption　of　TBBPA　from　water.　Static　adsorption　experiments　demonstrated　that　the　adsorption　capacity　could　reach　232　mgg-1　within　120　min,　which　is　much　higher　than　those　reported　in　the　other　literature.　The　experimental　results　show　that　the　adsorption　of　TBBPA　on　Fe3O4/GO/ZIF-67　followed　Langmuir　and　pseudo-second-order　kinetic　adsorption　models.　The　main　mechanisms　for　these　adsorptions　were　identified　as　hydrogen　bonds　between　OH　groups　in　TBBPA　and　COOHs　of　Fe3O4/GO/ZIF-67,　and　pi-pi　stacking　between　Fe3O4/GO/ZIF-67　and　TBBPA.　This　study　provides　a　method　with　great　promise　for　the　design　and　synthesis　of　better　adsorbents　for　the　removal　of　TBBPA　from　the　water　environment.