Based　on　the　interface　bonding　function　of　polydopamine　(PDA)　coating,　GO/PDA/CNT　double-layer　low-pressure　membrane　with　stable　mechanical　properties　was　successfully　loaded　on　the　PES　membrane　by　vacuum　filtration　method.　From　the　perspective　of　the　structure-performance　relationship,　the　upper　carbon　nanotube　(CNT)　layer　can　play　the　role　of　pre-filtration　and　pre-adsorption,　which　possess　an　antifouling　function.　The　lower　layer　contains　a　lot　of　narrow　nanochannels　formed　by　stacking　graphene　oxide　(GO)　nanosheets,　which　further　reject　the　pollutants.　The　filtration　experiments　with　humic　acid　(HA),　a　significant　component　of　natural　organic　matter　(NOM),　showed　that　the　GO/PDA/CNT　double-layer　membrane　demonstrated　better　HA　removal　(88.5%)　and　better　antifouling　performance.　In　addition,　the　GO/PDA/CNT　membrane　can　be　restored　entirely　after　simply　rinsing　with　pure　water.　Compared　with　the　GO　membrane,　the　GO/PDA/CNT　double-layer　membrane　flux　is　more　stable　and　higher　than　the　single-layer　GO　membrane　in　the　whole　filtration　process,　which　solves　the　compaction　problem　of　the　GO　membrane　in　the　pressure-driven　filtration　process.　©　The　Author(s),　under　exclusive　license　to　Springer　Nature　Switzerland　AG　2024.