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Author:

Li, Yanxia (Li, Yanxia.) | Luo, Chaoming (Luo, Chaoming.) | Liu, Zhongliang (Liu, Zhongliang.) (Scholars:刘中良) | Lin, Feng (Lin, Feng.)

Indexed by:

Scopus SCIE

Abstract:

Utilizing catalysts in microcombustors is probably an excellent practical solution to stabilize fuel combustion because of the relatively fast reaction speed. In the present work, the monolithic catalyst Pd/A(2)O(3)/Fe-Ni with metal foam as matrix was used inside a 5 mm in diameter microcombustor. Then the effects of inlet velocity and equivalent ratio on catalytic combustion characteristics of methane were studied experimentally. The results showed that the methane and air mixture with the stoichiometric ratio Phi = 1.0 could be ignited at v = 0.2-0.6 m/s. The velocity of premixed mixture had a great influence on the catalytic combustion of methane. The larger the inlet velocity, the higher the temperature and the brighter the flame were. The experiment results also showed that the equivalence ratio had a large essential impact on the catalytic combustion, especially for the lean mixture of methane and air. It seemed the addition of the porous matrix with catalysts could significantly extend the limits of stable combustion. In the detection of exhaust gas, CO selectivity increased and CO2 selectivity decreased with the equivalence ratio. When Phi was between 0.94 and 1.0 m/s, a little amount of hydrogen was produced due to the lack of oxygen. The measured conversion of methane to CO and CO2 was very high, usually greater than 99%, which indicated the excellent performance of the catalyst.

Keyword:

methane monolithic catalyst catalytic combustion metal foam substrate

Author Community:

  • [ 1 ] [Li, Yanxia]Beijing Univ Technol, MOE Key Lab Enhanced Heat Transfer & Energy Conse, Beijing Key Lab Heat Transfer & Energy Convers, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 2 ] [Luo, Chaoming]Beijing Univ Technol, MOE Key Lab Enhanced Heat Transfer & Energy Conse, Beijing Key Lab Heat Transfer & Energy Convers, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 3 ] [Liu, Zhongliang]Beijing Univ Technol, MOE Key Lab Enhanced Heat Transfer & Energy Conse, Beijing Key Lab Heat Transfer & Energy Convers, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 4 ] [Luo, Chaoming]Energy Supervis Unit Ctr Tonglu, Hangzhou 311501, Zhejiang, Peoples R China
  • [ 5 ] [Lin, Feng]Energy Supervis Unit Ctr Tonglu, Hangzhou 311501, Zhejiang, Peoples R China

Reprint Author's Address:

  • 刘中良

    [Liu, Zhongliang]Beijing Univ Technol, MOE Key Lab Enhanced Heat Transfer & Energy Conse, Beijing Key Lab Heat Transfer & Energy Convers, Coll Environm & Energy Engn, Beijing 100124, Peoples R China

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Source :

CATALYSTS

ISSN: 2073-4344

Year: 2018

Issue: 11

Volume: 8

3 . 9 0 0

JCR@2022

ESI Discipline: CHEMISTRY;

ESI HC Threshold:192

Cited Count:

WoS CC Cited Count: 6

SCOPUS Cited Count: 7

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 4

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