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Author:

Nie, X. C. (Nie, X. C..) | Song, Hai-Ying (Song, Hai-Ying.) | Zhang, Xiu (Zhang, Xiu.) | Gu, Peng (Gu, Peng.) | Liu, Shi-Bing (Liu, Shi-Bing.) (Scholars:刘世炳) | Li, Fan (Li, Fan.) (Scholars:李钒) | Meng, Jian-Qiao (Meng, Jian-Qiao.) | Duan, Yu-Xia (Duan, Yu-Xia.) | Liu, H. Y. (Liu, H. Y..)

Indexed by:

EI Scopus SCIE

Abstract:

We present systematic studies of the transient dynamics of GaAs by ultrafast time-resolved reflectivity. In photoexcited non-equilibrium states, we found a sign reverse in reflectivity change Delta R/R, from positive around room temperature to negative at cryogenic temperatures. The former corresponds to a free carrier metallic state, while the latter is attributed to an exciton insulating state, in which the transient electronic properties is mostly dominated by excitons, resulting in a transient metal-insulator transition (MIT). Two transition temperatures (T-1 and T-2) are well identified by analyzing the intensity change of the transient reflectivity. We found that photoexcited MIT starts emerging at T-1 as high as similar to 230 K, in terms of a dip feature at 0.4 ps, and becomes stabilized below T-2 that is up to similar to 180 K, associated with a negative constant after 40 ps. Our results address a phase diagram that provides a framework for the inducing of MIT through temperature and photoexcitation, and may shed light on the understanding of light-semiconductor interaction and exciton physics.

Keyword:

exciton metal-insulator transition ultrafast pump-probe spectroscopy

Author Community:

  • [ 1 ] [Nie, X. C.]Beijing Univ Technol, Inst Laser Engn, Strong Field & Ultrafast Photon Lab, Beijing 100124, Peoples R China
  • [ 2 ] [Song, Hai-Ying]Beijing Univ Technol, Inst Laser Engn, Strong Field & Ultrafast Photon Lab, Beijing 100124, Peoples R China
  • [ 3 ] [Zhang, Xiu]Beijing Univ Technol, Inst Laser Engn, Strong Field & Ultrafast Photon Lab, Beijing 100124, Peoples R China
  • [ 4 ] [Gu, Peng]Beijing Univ Technol, Inst Laser Engn, Strong Field & Ultrafast Photon Lab, Beijing 100124, Peoples R China
  • [ 5 ] [Liu, Shi-Bing]Beijing Univ Technol, Inst Laser Engn, Strong Field & Ultrafast Photon Lab, Beijing 100124, Peoples R China
  • [ 6 ] [Liu, H. Y.]Beijing Univ Technol, Inst Laser Engn, Strong Field & Ultrafast Photon Lab, Beijing 100124, Peoples R China
  • [ 7 ] [Li, Fan]Beijing Univ Technol, Dept Chem & Chem Engn, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 8 ] [Meng, Jian-Qiao]Cent South Univ, Sch Phys & Elect, Hunan Key Lab Super Microstruct & Ultrafast Proc, Changsha 410083, Hunan, Peoples R China
  • [ 9 ] [Duan, Yu-Xia]Cent South Univ, Sch Phys & Elect, Changsha 410083, Hunan, Peoples R China

Reprint Author's Address:

  • [Song, Hai-Ying]Beijing Univ Technol, Inst Laser Engn, Strong Field & Ultrafast Photon Lab, Beijing 100124, Peoples R China

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Source :

NEW JOURNAL OF PHYSICS

ISSN: 1367-2630

Year: 2018

Volume: 20

3 . 3 0 0

JCR@2022

ESI Discipline: PHYSICS;

ESI HC Threshold:145

JCR Journal Grade:1

Cited Count:

WoS CC Cited Count: 9

SCOPUS Cited Count: 8

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 9

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