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Author:

Luo, Qiang (Luo, Qiang.) | Ma, He (Ma, He.) (Scholars:马赫) | Hou, Qinzhi (Hou, Qinzhi.) | Li, Yingxiang (Li, Yingxiang.) | Ren, Jing (Ren, Jing.) | Dai, Xuezeng (Dai, Xuezeng.) | Yao, Zhibo (Yao, Zhibo.) | Zhou, Yu (Zhou, Yu.) | Xiang, Lichen (Xiang, Lichen.) | Du, Huayun (Du, Huayun.) | He, Hongcai (He, Hongcai.) | Wang, Ning (Wang, Ning.) | Jiang, Kaili (Jiang, Kaili.) | Lin, Hong (Lin, Hong.) | Zhang, Huaiwu (Zhang, Huaiwu.) | Guo, Zhanhu (Guo, Zhanhu.)

Indexed by:

EI Scopus SCIE

Abstract:

Endured, low-cost, and high-performance flexible perovskite solar cells (PSCs) featuring lightweight and mechanical flexibility have attracted tremendous attention for portable power source applications. However, flexible PSCs typically use expensive and fragile indium-tin oxide as transparent anode and high-vacuum processed noble metal as cathode, resulting in dramatic performance degradation after continuous bending or thermal stress. Here, all-carbon-electrode-based flexible PSCs are fabricated employing graphene as transparent anode and carbon nanotubes as cathode. All-carbon-electrode-based flexible devices with and without spiro-OMeTAD (2,2,7,7-tetrakis-(N,N-di-p-methoxyphenylamine)-9,9-spirobifluorene) hole conductor achieve power conversion efficiencies (PCEs) of 11.9% and 8.4%, respectively. The flexible carbon-electrode-based solar cells demonstrate superior robustness against mechanical deformation in comparison with their counterparts fabricated on flexible indium-tin oxide substrates. Moreover, all carbon-electrode-based flexible PSCs also show significantly enhanced stability compared to the flexible devices with gold and silver cathodes under continuous light soaking or 60 degrees C thermal stress in air, retaining over 90% of their original PCEs after 1000 h. The promising durability and stability highlight that flexible PSCs are fully compatible with carbon materials and pave the way toward the realization of rollable and low-cost flexible perovskite photovoltaic devices.

Keyword:

carbon materials perovskite solar cells stability flexibility conductivity

Author Community:

  • [ 1 ] [Luo, Qiang]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China
  • [ 2 ] [Hou, Qinzhi]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China
  • [ 3 ] [Li, Yingxiang]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China
  • [ 4 ] [He, Hongcai]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China
  • [ 5 ] [Wang, Ning]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China
  • [ 6 ] [Zhang, Huaiwu]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China
  • [ 7 ] [Ma, He]Beijing Univ Technol, Coll Appl Sci, Beijing 100124, Peoples R China
  • [ 8 ] [Ma, He]Tsinghua Univ, Collaborat Innovat Ctr Quantum Matter, Dept Phys, Nanotechnol Res Ctr,State Key Lab Low Dimens Quan, Beijing 100084, Peoples R China
  • [ 9 ] [Jiang, Kaili]Tsinghua Univ, Collaborat Innovat Ctr Quantum Matter, Dept Phys, Nanotechnol Res Ctr,State Key Lab Low Dimens Quan, Beijing 100084, Peoples R China
  • [ 10 ] [Dai, Xuezeng]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 11 ] [Yao, Zhibo]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 12 ] [Lin, Hong]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 13 ] [Du, Huayun]Univ Tennessee, Dept Chem & Biomol Engn, ICL, Knoxville, TN 37996 USA
  • [ 14 ] [Guo, Zhanhu]Univ Tennessee, Dept Chem & Biomol Engn, ICL, Knoxville, TN 37996 USA
  • [ 15 ] [Xiang, Lichen]Zhengzhou Univ, Minist Educ, Key Lab Mat Proc & Mold, Zhengzhou 450001, Henan, Peoples R China
  • [ 16 ] [Wang, Ning]Hainan Univ, State Key Lab Marine Resource Utilizat South Chin, Haikou 570228, Hainan, Peoples R China

Reprint Author's Address:

  • [Wang, Ning]Univ Elect Sci & Technol China, State Key Lab Elect Thin Film & Integrated Device, Chengdu 610054, Sichuan, Peoples R China;;[Jiang, Kaili]Tsinghua Univ, Collaborat Innovat Ctr Quantum Matter, Dept Phys, Nanotechnol Res Ctr,State Key Lab Low Dimens Quan, Beijing 100084, Peoples R China;;[Lin, Hong]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China;;[Guo, Zhanhu]Univ Tennessee, Dept Chem & Biomol Engn, ICL, Knoxville, TN 37996 USA;;[Wang, Ning]Hainan Univ, State Key Lab Marine Resource Utilizat South Chin, Haikou 570228, Hainan, Peoples R China

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Source :

ADVANCED FUNCTIONAL MATERIALS

ISSN: 1616-301X

Year: 2018

Issue: 11

Volume: 28

1 9 . 0 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:260

JCR Journal Grade:1

Cited Count:

WoS CC Cited Count: 314

SCOPUS Cited Count: 323

ESI Highly Cited Papers on the List: 39 Unfold All

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WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 5

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