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学者姓名：戴洪兴
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Abstract ：
The Pt/CeO2 catalyst has attracted significant attention due to its exceptional performance in NO oxidation. This study comprehensively examines the effects of calcination temperature and H-2 pretreatment on the structure and activity of the Pt/CeO2 catalyst. Experimental findings indicate that the calcination temperature significantly affects the catalyst's redox performance, thereby modulating its efficacy in NO oxidation reactions. H-2 pretreatment facilitates the creation of oxygen vacancies on the catalyst, assisted by the reduction in PtOx to Pt, enhancing the formation of activated oxygen and thereby improving NO oxidation. This study offers valuable insights into the design and optimization of Pt/CeO2 catalysts for environmental applications, particularly in the development of exhaust gas after-treatment technologies.
Keyword ：
H-2 pretreatment H-2 pretreatment oxygen species activation oxygen species activation Pt/CeO2 catalyst Pt/CeO2 catalyst NO oxidation NO oxidation
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| GB/T 7714 | Li, Xiangru , Li, Shuangye , Cheng, Yao et al. The Activation of Oxygen Species on the Pt/CeO2 Catalyst by H2 for NO Oxidation [J]. | CATALYSTS , 2024 , 14 (11) . |
| MLA | Li, Xiangru et al. "The Activation of Oxygen Species on the Pt/CeO2 Catalyst by H2 for NO Oxidation" . | CATALYSTS 14 . 11 (2024) . |
| APA | Li, Xiangru , Li, Shuangye , Cheng, Yao , Zheng, Lechen , Song, Liyun , Zi, Xuehong et al. The Activation of Oxygen Species on the Pt/CeO2 Catalyst by H2 for NO Oxidation . | CATALYSTS , 2024 , 14 (11) . |
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Abstract ：
To improve catalytic activity and sulfur dioxide and water resistance of the 0.25Pt/TiO2 catalyst and explore the simple catalyst preparation method suitable for industrial production, we developed a 0.25Pt-CoOx/TiO2 catalyst in the present work. The 0.25Pt-CoOx/TiO2 catalyst was prepared via the impregnation-, precipitation-, and ball milling-combined method, and its catalytic CO oxidation performance as well as sulfur dioxide and water resistance was examined. It was shown that the 0.25Pt-CoOx/TiO2 catalyst exhibited a good catalytic activity and good resistance to sulfur dioxide and water. The T50, T90, and T100 (the temperatures for achieving CO conversions of 50, 90, and 100%) over the 0.25Pt-CoOx/TiO2 catalyst at a space velocity of 47,872 mL/(g h) were 95, 110, and 120 degrees C, which were 70, 57, and 50 degrees C lower than those over the 0.25Pt/TiO2 catalyst, respectively. Meanwhile, CO conversions over 0.25Pt-CoOx/TiO2 were maintained at above 99% within 12 h of reaction in the co-presence of SO2 and H2O. The doping of CoOx to 0.25Pt/TiO2 increased the surface Co3+ species concentration, redox ability, and acid site number of the 0.25Pt-CoOx/TiO2 catalyst, which favored the enhancements in catalytic activity and SO2- and H2O-resistant performance. In addition, it was also found that an appropriate amount of H2O introduction to the reaction system could promote the oxidation of CO and inhibit the negative effect of SO2 addition on CO oxidation over 0.25Pt-CoOx/TiO2, thus making this catalyst show good CO oxidation activity and good sulfur dioxide and water resistance. We are sure that the developed 0.25Pt-CoOx/ TiO2 catalyst has a great application potential in the removal of the flue gas emissions from the iron and steel industries.
Keyword ：
Titania -supported platinum catalyst Titania -supported platinum catalyst Carbon monoxide oxidation Carbon monoxide oxidation Sulfur dioxide resistance Sulfur dioxide resistance Water resistance Water resistance Cobalt oxide doping Cobalt oxide doping
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| GB/T 7714 | Cai, Jianyu , He, Junda , Yu, Zehui et al. Enhanced catalytic activity and stability in CO oxidation of the Pt/TiO2 catalyst by CoOx doping [J]. | SURFACES AND INTERFACES , 2024 , 51 . |
| MLA | Cai, Jianyu et al. "Enhanced catalytic activity and stability in CO oxidation of the Pt/TiO2 catalyst by CoOx doping" . | SURFACES AND INTERFACES 51 (2024) . |
| APA | Cai, Jianyu , He, Junda , Yu, Zehui , Li, Jian , Fan, Xing , Liang, Wenjun et al. Enhanced catalytic activity and stability in CO oxidation of the Pt/TiO2 catalyst by CoOx doping . | SURFACES AND INTERFACES , 2024 , 51 . |
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| GB/T 7714 | Dai, Hongxing , Wang, Junhu . Advances in Catalytic Oxidation of Methane and Carbon Monoxide (2nd Edition) [J]. | CATALYSTS , 2024 , 14 (9) . |
| MLA | Dai, Hongxing et al. "Advances in Catalytic Oxidation of Methane and Carbon Monoxide (2nd Edition)" . | CATALYSTS 14 . 9 (2024) . |
| APA | Dai, Hongxing , Wang, Junhu . Advances in Catalytic Oxidation of Methane and Carbon Monoxide (2nd Edition) . | CATALYSTS , 2024 , 14 (9) . |
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| GB/T 7714 | Dai, Hongxing , Wang, Xiang , Zhu, Yujun et al. Exclusive Papers on Environmentally Friendly Catalysis in China [J]. | CATALYSTS , 2023 , 13 (9) . |
| MLA | Dai, Hongxing et al. "Exclusive Papers on Environmentally Friendly Catalysis in China" . | CATALYSTS 13 . 9 (2023) . |
| APA | Dai, Hongxing , Wang, Xiang , Zhu, Yujun , Huang, Haibao , Zhao, Yunkun . Exclusive Papers on Environmentally Friendly Catalysis in China . | CATALYSTS , 2023 , 13 (9) . |
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Abstract ：
The development of efficient and stable catalysts is of great importance for the elimination of volatile organic pollutants (VOCs). In this work, AuPdx nanoparticles (NPs) were loaded on TiO2 through the electrostatic adsorption approach to generate the yAuPd(x)/TiO2 (i.e., 0.35AuPd(0.46)/TiO2, 0.34AuPd(2.09)/TiO2, and 0.37AuPd(2.72)/TiO2; x and y are Pd/Au molar ratio and AuPdx loading, respectively; x = 0.46-2.72; and y = 0.34-0.37 wt%) catalysts, and their catalytic activities for the oxidation of ethyl acetate were determined. The results showed that the 0.37AuPd(2.72)/TiO2 sample exhibited the best activity (T-50% = 217 degrees C and T-90% = 239 degrees C at SV = 40,000 mL/(g h), E-a = 37 kJ/mol, specific reaction rate at 220 degrees C = 113.8 mu mol/(g(Pd) s), and turnover frequency (TOFNoble metal) at 220 degrees C = 109.7 x 10(-3) s(-1)). The high catalytic performance of the 0.37AuPd(2.72)/TiO2 sample was attributed to the good dispersion of AuPd2.72 NPs, the strong redox ability, the large ethyl acetate adsorption capacity, and the strong interaction between AuPdx and TiO2. Acetaldehyde, ethanol, and acetic acid are the main intermediates in the oxidation of ethyl acetate, and the loading of AuPdx NPs effectively reduces the formation of the toxic by-product acetaldehyde. The oxidation of ethyl acetate over the 0.34AuPd(2.09)/TiO2 sample might occur via the pathway of ethyl acetate -> ethanol -> acetic acid -> acetate -> CO2 and H2O. We believe that the obtained results may provide a useful idea for the design of bimetallic catalysts under industrial conditions and for understanding the VOCs oxidation mechanisms.
Keyword ：
ethyl acetate oxidation ethyl acetate oxidation strong electrostatic adsorption strong electrostatic adsorption sulfur dioxide resistance sulfur dioxide resistance reaction mechanism reaction mechanism supported Au-Pd nanocatalyst supported Au-Pd nanocatalyst
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| GB/T 7714 | Bao, Minming , Liu, Yuxi , Deng, Jiguang et al. Catalytic Performance and Reaction Mechanisms of Ethyl Acetate Oxidation over the Au-Pd/TiO2 Catalysts [J]. | CATALYSTS , 2023 , 13 (4) . |
| MLA | Bao, Minming et al. "Catalytic Performance and Reaction Mechanisms of Ethyl Acetate Oxidation over the Au-Pd/TiO2 Catalysts" . | CATALYSTS 13 . 4 (2023) . |
| APA | Bao, Minming , Liu, Yuxi , Deng, Jiguang , Jing, Lin , Hou, Zhiquan , Wang, Zhiwei et al. Catalytic Performance and Reaction Mechanisms of Ethyl Acetate Oxidation over the Au-Pd/TiO2 Catalysts . | CATALYSTS , 2023 , 13 (4) . |
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Abstract ：
Designing new synthesis routes to fabricate highly thermallydurableprecious metal single-atom catalysts (SACs) is challenging in industrialapplications. Herein, a general strategy is presented that startsfrom dual-metal nanocrystals (NCs), using bimetallic NCs as a facilitatorto spontaneously convert a series of noble metals to single atomson aluminum oxide. The metal single atoms are captured by cation defects in situ formed on the surface of the inversespinel (AB(2)O(4)) structure, which process providesnumerous anchoring sites, thus facilitating generation of the isolatedmetal atoms that contributes to the extraordinary thermodynamic stability.The Pd-1/AlCo2O4-Al2O3 shows not only improved low-temperature activity butalso unprecedented (hydro)thermal stability for CO and propane oxidationunder harsh aging conditions. Furthermore, our strategy exhibits asmall scaling-up effect by the simple physical mixing of commercialmetal oxide aggregates with Al2O3. The goodregeneration between oxidative and reductive atmospheres of theseionic palladium species makes this catalyst system of potential interestfor emissions control.
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| GB/T 7714 | Hou, Zhiquan , Lu, Yue , Liu, Yuxi et al. A General Dual-Metal Nanocrystal Dissociation Strategy to Generate Robust High-Temperature-Stable Alumina-Supported Single-Atom Catalysts [J]. | JOURNAL OF THE AMERICAN CHEMICAL SOCIETY , 2023 , 145 (29) : 15869-15878 . |
| MLA | Hou, Zhiquan et al. "A General Dual-Metal Nanocrystal Dissociation Strategy to Generate Robust High-Temperature-Stable Alumina-Supported Single-Atom Catalysts" . | JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 145 . 29 (2023) : 15869-15878 . |
| APA | Hou, Zhiquan , Lu, Yue , Liu, Yuxi , Liu, Ning , Hu, Jingcong , Wei, Lu et al. A General Dual-Metal Nanocrystal Dissociation Strategy to Generate Robust High-Temperature-Stable Alumina-Supported Single-Atom Catalysts . | JOURNAL OF THE AMERICAN CHEMICAL SOCIETY , 2023 , 145 (29) , 15869-15878 . |
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Abstract ：
Among the developed electrocatalysts, NiCr-layered double hydroxides (NiCr-LDH) are one of the most effective electrocatalytic materials for water oxidation. However, applications of such a kind of materials are practically limited due to their poor electric conductivity. In this work, the single-walled carbon nanotube (SWCNT) was doped to NiCr-LDH, and the LDH-based nanocomposites were synthesized using the one-step ultrasonic-assisted method. Physicochemical properties of the NiCr-LDH/SWCNT composites were characterized by means of X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FTIR), energy dispersive X-ray (EDX) analysis, transmission electron microscopy (TEM), field emission-scanning electron microscopy (FE-SEM), and linear sweep voltammetry (LSV). The NiCr-LDH/SWCNT composites were used as effective nanomaterials for oxygen evolution reaction (OER) at a near neutral medium. The LSV results confirm that the overpotential of the NiCr-LDH/SWCNT-0.006 sample decreased to about 120 mV at pH = 9.5, as compared with that of the NiCr-LDH or NiCr-LDH-SWCNT-0.006 (prepared by the two-step method) sample. The high oxygen evolution activity of NiCr-LDH/SWCNT-0.006 was associated with the co-presence of the homogeneously dispersed NiCr-LDH, good electrochemical activity, and high electrical conductivity. In addition, the as-prepared optimized NiCr-LDH/SWCNT electrocatalyst was highly stable for the OER reaction. (c) 2022 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
Keyword ：
Ni-based-layered double hydroxide Ni-based-layered double hydroxide Ultrasonic method Ultrasonic method Doped carbon nanotube Doped carbon nanotube Water oxidation Water oxidation Electrocatalyst Electrocatalyst
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| GB/T 7714 | Foruzin, Leila Jafari , Nejati, Kamellia , Dai, Hongxing et al. Ultrasonic-assisted synthesis of Ni based-layered double hydroxide doped carbon nanotube and its highly efficient in water oxidation reaction [J]. | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2023 , 48 (9) : 3429-3439 . |
| MLA | Foruzin, Leila Jafari et al. "Ultrasonic-assisted synthesis of Ni based-layered double hydroxide doped carbon nanotube and its highly efficient in water oxidation reaction" . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 48 . 9 (2023) : 3429-3439 . |
| APA | Foruzin, Leila Jafari , Nejati, Kamellia , Dai, Hongxing , Rezvani, Zolfaghar . Ultrasonic-assisted synthesis of Ni based-layered double hydroxide doped carbon nanotube and its highly efficient in water oxidation reaction . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2023 , 48 (9) , 3429-3439 . |
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Abstract ：
The painting and electronics industries simultaneously release aromatic compounds and chlorinated organics. The development of catalysts with synergistic control of these pollutants is of great significance to achieve air purification. However, developing active catalysts while maintaining good chlorine resistance remain a huge challenge due to the difficulty of the trade-off between the redox properties and acidity and the production of polychlorinated byproducts. Herein, we introduce a novel tandem PtSn/CeO2 & Mn/ZSM-5 catalyst and investigate its catalytic performance for multicomponent volatile organic compounds (VOCs) oxidation. The two individual catalysts, PtSn/CeO2 and Mn/ZSM-5, were used to catalyze two distinct sequential reactions. PtSn/CeO2 catalyzed toluene oxidation to produce CO2 and H2O. Meanwhile, the introduction of SnOx favored the adsorption of trichloroethylene (TCE) molecules that prevented Pt sites from chlorine poisoning and possibly converted adsorbed TCE into intermediates, which were subsequently oxidized deeply by the nearby Mn/ZSM-5. This approach resulted in a remarkable oxidation efficiency for toluene (T90 = 296 degrees C) and TCE (T90 = 384 degrees C), with fewer unexpected toxic byproducts (chlorobenzene and 4-chlorotoluene). Furthermore, the tandem catalyst possessed excellent chlorine and water resistances. In conclusion, the above findings provide new insights into the design and/or syntheses of advanced catalysts for widespread VOCs pollution control.
Keyword ：
Catalytic oxidation Catalytic oxidation Polychlorinated byproducts Polychlorinated byproducts Multicomponent volatile organic compound Multicomponent volatile organic compound Supported catalyst Supported catalyst Tandem catalyst Tandem catalyst
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| GB/T 7714 | Li, Zeya , Gao, Ruyi , Hou, Zhiquan et al. Tandem supported Pt and ZSM-5 catalyst with separated catalytic functions for promoting multicomponent VOCs oxidation [J]. | APPLIED CATALYSIS B-ENVIRONMENTAL , 2023 , 339 . |
| MLA | Li, Zeya et al. "Tandem supported Pt and ZSM-5 catalyst with separated catalytic functions for promoting multicomponent VOCs oxidation" . | APPLIED CATALYSIS B-ENVIRONMENTAL 339 (2023) . |
| APA | Li, Zeya , Gao, Ruyi , Hou, Zhiquan , Yu, Xiaohui , Dai, Hongxing , Deng, Jiguang et al. Tandem supported Pt and ZSM-5 catalyst with separated catalytic functions for promoting multicomponent VOCs oxidation . | APPLIED CATALYSIS B-ENVIRONMENTAL , 2023 , 339 . |
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Abstract ：
As typical air pollutants, CO, CH4, and volatile organic compounds (VOCs) have received great attention due to their negative impact on the environment and human health. Heterogeneous catalysts are widely used in the catalytic removal of exhaust emission from industrial and automobile sources but still suffer from deactivation because of various factors. The development of a catalyst with excellent catalytic stability is highly desired. We herein summarized the recent progress for enhancing the catalytic stability of catalysts and tried to obtain an in-depth understanding of the long-term durability, resistance to sinter, and tolerance for multi-impurities. Finally, the current challenges and future perspectives for developing stable and highly efficient catalysts in the fields of synergistic catalytic removal of pollutants or resource utilization of VOCs via the selective catalytic oxidation are proposed.
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| GB/T 7714 | Feng, Yuan , Liu, Yuxi , Dai, Hongxing et al. Review and Perspectives of Enhancement in the Catalytic Stability for the Complete Combustion of CO, CH4, and Volatile Organic Compounds [J]. | ENERGY & FUELS , 2023 . |
| MLA | Feng, Yuan et al. "Review and Perspectives of Enhancement in the Catalytic Stability for the Complete Combustion of CO, CH4, and Volatile Organic Compounds" . | ENERGY & FUELS (2023) . |
| APA | Feng, Yuan , Liu, Yuxi , Dai, Hongxing , Deng, Jiguang . Review and Perspectives of Enhancement in the Catalytic Stability for the Complete Combustion of CO, CH4, and Volatile Organic Compounds . | ENERGY & FUELS , 2023 . |
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Abstract ：
The emission of methane leads to the increase in the methane concentration in the atmosphere, which not only wastes resources but also intensifies the greenhouse effect and brings about serious environmental problems. Catalytic combustion can completely convert methane into carbon dioxide and water at low temperatures. However, the catalytic activities of the conventional supported palladium catalysts (e.g., Pd/Al2O3 and Pd/ZrO2) are easy to decrease or the two catalysts can even be deactivated under actual harsh reaction conditions (high temperatures, steam- and sulfur dioxide-containing atmospheres, etc.). Recently, noble metal catalysts supported on zeolites with ordered pores and good thermal stability have attracted much attention. This review article summarizes the recent progress on the development and characteristics of zeolite-supported noble metal catalysts for the combustion of methane. The effects of framework structures, silica/alumina ratios, acidity, doping of alkali metals or transition metals, particle sizes and distributions, and their locations of/in the zeolites on methane combustion activity are discussed. The importance of developing high-performance catalysts under realistic operation conditions is highlighted. In addition, the related research work on catalytic methane combustion in the future is also envisioned.
Keyword ：
zeolite zeolite supported noble metal catalyst supported noble metal catalyst catalytic oxidation mechanism catalytic oxidation mechanism methane combustion methane combustion palladium-based catalyst palladium-based catalyst
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| GB/T 7714 | Tao, Jinxiong , Liu, Yuxi , Deng, Jiguang et al. Methane Combustion over Zeolite-Supported Palladium-Based Catalysts [J]. | CATALYSTS , 2023 , 13 (9) . |
| MLA | Tao, Jinxiong et al. "Methane Combustion over Zeolite-Supported Palladium-Based Catalysts" . | CATALYSTS 13 . 9 (2023) . |
| APA | Tao, Jinxiong , Liu, Yuxi , Deng, Jiguang , Jing, Lin , Hou, Zhiquan , Wei, Lu et al. Methane Combustion over Zeolite-Supported Palladium-Based Catalysts . | CATALYSTS , 2023 , 13 (9) . |
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