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Treatment of volatile ethanol gas emitted by pharmaceutical manufacturing industry in a combination process of spraying absorption and wastewater biological treatment SCIE
期刊论文 | 2024 , 12 (6) | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
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Abstract :

The pharmaceutical industry is a significant emission source of water-soluble volatile organic compounds (VOCs). However, these VOCs are primarily treated through adsorption on activated carbon or combustion methods, leading to high the generation of hazardous solid waste or energy consumption. This study proposed an innovative approach to address these issues by integrating spray absorption with biological treatment in sequencing batch reactors (SBRs). The results indicated that after spray absorption, more than 90 % of ethanol could be removed in SBRs, while 1-6 % of ethanol was emitted into the atmosphere, depending on aeration intensity and ethanol concentration. Although the intermittent emissions of ethanol gas resulted in a high variation in loading into the activated sludge system, stable and efficient treatment of ethanol was achieved. Amaricoccus was predominated as the primary bacterium responsible for ethanol degradation, indicating a robust microbial community capable of adapting to fluctuating ethanol levels. This study provides an environment-friendly and efficient solution to treating water-soluble VOCs. The proposed method utilizes existing infrastructure such as spray towers and biological treatment facilities commonly found in pharmaceutical enterprises, making it a cost-effective and easily implementable technology. This study contributes to the advancement of understanding in the field of VOCs treatment.

Keyword :

Volatile ethanol gas Volatile ethanol gas Spraying absorption Spraying absorption Ethanol shock loads Ethanol shock loads Biological treatment Biological treatment Ethanol emissions Ethanol emissions

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GB/T 7714 Zhu, Wen-Jie , Cui, You-Wei , Yang, Hou-Jian . Treatment of volatile ethanol gas emitted by pharmaceutical manufacturing industry in a combination process of spraying absorption and wastewater biological treatment [J]. | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING , 2024 , 12 (6) .
MLA Zhu, Wen-Jie 等. "Treatment of volatile ethanol gas emitted by pharmaceutical manufacturing industry in a combination process of spraying absorption and wastewater biological treatment" . | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING 12 . 6 (2024) .
APA Zhu, Wen-Jie , Cui, You-Wei , Yang, Hou-Jian . Treatment of volatile ethanol gas emitted by pharmaceutical manufacturing industry in a combination process of spraying absorption and wastewater biological treatment . | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING , 2024 , 12 (6) .
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Spontaneous granulation of moderately halophilic sludge inoculated with saltern sediments from single granule into multi-granule aggregation SCIE
期刊论文 | 2023 , 216 | ENVIRONMENTAL RESEARCH
WoS CC Cited Count: 6
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Abstract :

There is very limited research on the application of moderate halophiles for biotreatment of hypersaline wastewater widely generated from some industries. This study demonstrated the development of moderate halophiles inoculated from saltern sediments into aerobic granule sludge (AGS) to treat hypersaline wastewater with a salinity of 100 g/L. The granulation of moderate halophiles can occur without applying the settling ve-locity selective pressure. The saltern sediment initially aggregated into single small granules and finally devel-oped into 1200 +/- 50 mu m multiparticle granules. The halophiles affiliated in Halomonas was dominant in the granular bacterial community, with a relative abundance of 94.52%. Halomonas ventosae secreted sulfated polysaccharides. The sulfated polysaccharides content accounted for 63.95 +/- 2.10% in the polysaccharides (PS), having an adhesive role in connecting single granules. Multiparticle granules showed the clear stratified struc-ture, with alpha-D-glucopyranose polysaccharides in the inner bounders and beta-D-glucopyranose polysaccharides in the outer. The moderately granular sludge showed the stable chemical oxygen demand (COD) removal efficiency of >90% and the aerobic total inorganic nitrogen (TIN) removal efficiency (equal to ammonia removal) of 70 +/- 5.00%. This paper contributes new insight into the formation of moderately halophilic granular sludge and accelerates the application of moderately halophilic granular sludge to treat hypersaline wastewater.

Keyword :

Saltern sediments Saltern sediments Hypersaline wastewater Hypersaline wastewater Moderately halophilic granular sludge Moderately halophilic granular sludge Sulfated polysaccharides Sulfated polysaccharides Halomonas sp Halomonas sp

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GB/T 7714 Wang, Ling , Cui, You -Wei , Jian, Li et al. Spontaneous granulation of moderately halophilic sludge inoculated with saltern sediments from single granule into multi-granule aggregation [J]. | ENVIRONMENTAL RESEARCH , 2023 , 216 .
MLA Wang, Ling et al. "Spontaneous granulation of moderately halophilic sludge inoculated with saltern sediments from single granule into multi-granule aggregation" . | ENVIRONMENTAL RESEARCH 216 (2023) .
APA Wang, Ling , Cui, You -Wei , Jian, Li , Yao, Jia-Lin . Spontaneous granulation of moderately halophilic sludge inoculated with saltern sediments from single granule into multi-granule aggregation . | ENVIRONMENTAL RESEARCH , 2023 , 216 .
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A novel Pseudomonas aeruginosa strain performs simultaneous heterotrophic nitrification-aerobic denitrification and aerobic phosphate removal SCIE
期刊论文 | 2022 , 221 | WATER RESEARCH
WoS CC Cited Count: 48
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Abstract :

Nitrogen and phosphate removal from wastewater relies on different functional bacteria. In this study, a novel strain affiliated with Pseudomonas aeruginosa was isolated from activated sludge by gradient dilution and per-formed heterotrophic nitrification-aerobic denitrification and aerobic phosphate removal (HNADPR). The strain showed an ammonium removal efficiency of 87% and a phosphate removal efficiency of 97% under optimal conditions, such as C/N ratio of 10, P/N ratio of 0.1, temperature of 30C, and pH of 7.5-8.5. The modified Gompertz model could fit well the heterotrophic ammonium nitrification, aerobic nitrite/nitrate denitrification, and aerobic phosphate removal processes. Functional gene amplification indicated that ammonium removal followed the complete HN-AD pathway (NH4+ -> NH2OH -> NO2- -> NO3? -> NO2- -> NO -> N2O -> N-2). Phosphate removal only occurred under aerobic conditions and ceased under anaerobic conditions. In successive aerobic cycles, the strain persistently took up phosphate. In wastewater, phosphate was aerobically converted into cell membrane, intracellular and extracellular polymeric substrates (EPS). Phosphorus in the form of phosphate monoester was pooled in EPS. A hypothetic aerobic phosphate removal model for strain SNDPR-01 is proposed to improve our understanding of the novel bacterial function of HNADPR.

Keyword :

Aerobic phosphate removal model Aerobic phosphate removal model Phosphorus species Phosphorus species Heterotrophic nitrification-aerobic denitrification Heterotrophic nitrification-aerobic denitrification Simultaneous nitrogen and phosphate removal Simultaneous nitrogen and phosphate removal Nitrogen removal pathway Nitrogen removal pathway

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GB/T 7714 Huang, Mei-Qi , Cui, You -Wei , Huang, Ji-Lin et al. A novel Pseudomonas aeruginosa strain performs simultaneous heterotrophic nitrification-aerobic denitrification and aerobic phosphate removal [J]. | WATER RESEARCH , 2022 , 221 .
MLA Huang, Mei-Qi et al. "A novel Pseudomonas aeruginosa strain performs simultaneous heterotrophic nitrification-aerobic denitrification and aerobic phosphate removal" . | WATER RESEARCH 221 (2022) .
APA Huang, Mei-Qi , Cui, You -Wei , Huang, Ji-Lin , Sun, Feng-Long , Chen, Si . A novel Pseudomonas aeruginosa strain performs simultaneous heterotrophic nitrification-aerobic denitrification and aerobic phosphate removal . | WATER RESEARCH , 2022 , 221 .
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Sludge retention time effects on recovery of soluble organic matters via polyhydroxyalkanoate storage in contact stabilization process under feast/famine regime SCIE
期刊论文 | 2022 , 97 (12) , 3534-3543 | JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY
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BACKGROUND Contact stabilization (CS) can be used to capture organic matters from wastewater. However, CS is less efficient in capturing soluble organic matters (SOMs). Recovery of SOMs is required to minimize carbon emission and to maximize organic recovery from wastewater. RESULTS SOMs were recovered by applying a feast/famine (F/F) regime in a CS process. Sludge retention time (SRT) was found to regulate the recovery efficiency of SOMs. At a SRT of 4 d, 44.7% of the removed soluble chemical oxygen demand (SCOD) in wastewater was recovered and stored into intracellular polyhydroxyalkanoates (PHA), leading to 12.8% decrease of CO2 emission in comparison with the conventional activated sludge process. The storage of PHA in waste sludge harvested at a SRT of 4 d significantly increased the methane yield (187.3 +/- 5.9 mL (g VSS)(-1)). The dominant bacteria performing SOM recovery in CS belonged to the genera Tessaracoccus, norank_f__Caldilineaceacea, unclassified_f__Microbacteriaceae and Flavobacterium. CONCLUSIONS The study demonstrated that applying F/F regime in a CS process can recover SOMs via PHA storage. The regulation of SRT can enhance SCOD recovery. The study provides a solution to enhance SOM recovery from wastewater instead of being oxidized into CO2. (c) 2022 Society of Chemical Industry (SCI).

Keyword :

polyhydroxyalkanoate polyhydroxyalkanoate contact stabilization contact stabilization organic recovery organic recovery feast feast famine regime famine regime methane yield methane yield

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GB/T 7714 Sun, Feng-Long , Cui, You-Wei , Jian, Li et al. Sludge retention time effects on recovery of soluble organic matters via polyhydroxyalkanoate storage in contact stabilization process under feast/famine regime [J]. | JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY , 2022 , 97 (12) : 3534-3543 .
MLA Sun, Feng-Long et al. "Sludge retention time effects on recovery of soluble organic matters via polyhydroxyalkanoate storage in contact stabilization process under feast/famine regime" . | JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY 97 . 12 (2022) : 3534-3543 .
APA Sun, Feng-Long , Cui, You-Wei , Jian, Li , Yao, Jia-Lin . Sludge retention time effects on recovery of soluble organic matters via polyhydroxyalkanoate storage in contact stabilization process under feast/famine regime . | JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY , 2022 , 97 (12) , 3534-3543 .
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Coupling Magnetic Field and Salinity Upshock to Improve Polyhydroxyalkanoate Productivity by Haloferax mediterranei Feeding on Molasses Wastewater Scopus
期刊论文 | 2022 , 88 (13) | Applied and Environmental Microbiology
SCOPUS Cited Count: 4
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Abstract :

Low polyhydroxyalkanoate (PHA) volumetric productivity from wastewater limits low-cost PHA production. To resolve this problem, an external magnetic field (MF) coupled with upshock salinity was applied to PHA production by Haloferax mediterranei (family Halobacteriaceae). Elevating the fermentation salinity over the optimal growth salinity (200 g/L) increased the PHA cell content while inhibiting cell proliferation, decreasing volumetric productivity. When a MF of 50 mT in 300 g/L salinity was applied, H. mediterranei proliferation and PHA cell content were promoted, leading to a 7.95% increase in PHA volumetric productivity in synthetic molasses wastewater and a 13.82% increase in glucose feeding compared with those in 200 g/L salinity. Under the MF, osmotic pressure regulation was activated by accumulating K1 and increasing betaine synthesis. The maximum betaine content increased by 74.33% in 300 g/L salinity with a 50-mT MF compared with that in 200 g/L salinity. When a 50-mT MF in 300 g/L salinity was applied, the malondialdehyde (MDA) content decreased by 32.66% and the activity of superoxide dismutase (SOD) increased by 46.89%, which reduced the oxidative damage. This study provides a new solution to enhance PHA volumetric productivity by MF and an insight into the magnetic effects of H. mediterranei. IMPORTANCE The obstacle to replacing petroplastics with PHA is its high production cost. To increase the fermentation economy, a novel strategy of coupling a MF with salinity upshock was applied, which enhanced the PHA volumetric productivity of H. mediterranei in fermenting molasses wastewater. The magnetic effect of H. mediterranei was found at a MF of 50 mT, which improved the salt tolerance of H. mediterranei and reduced the oxidative damage induced by the elevated salinity, thereby promoting proliferation and PHA cell content. This is the first time a technical method for enhancing PHA volumetric productivity by means of a MF has been proposed. Such a strategy can advance the utilization of H. mediterranei for the industrial production of PHA using organic wastewater. Copyright © 2022 American Society for Microbiology. All Rights Reserved.

Keyword :

Haloferax mediterranei; magnetic field; microbial magnetic effect; polyhydroxyalkanoate volumetric productivity; salinity upshock Haloferax mediterranei; magnetic field; microbial magnetic effect; polyhydroxyalkanoate volumetric productivity; salinity upshock

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GB/T 7714 Chen, S. , Cui, Y.-W. , Huang, M.-Q. . Coupling Magnetic Field and Salinity Upshock to Improve Polyhydroxyalkanoate Productivity by Haloferax mediterranei Feeding on Molasses Wastewater [J]. | Applied and Environmental Microbiology , 2022 , 88 (13) .
MLA Chen, S. et al. "Coupling Magnetic Field and Salinity Upshock to Improve Polyhydroxyalkanoate Productivity by Haloferax mediterranei Feeding on Molasses Wastewater" . | Applied and Environmental Microbiology 88 . 13 (2022) .
APA Chen, S. , Cui, Y.-W. , Huang, M.-Q. . Coupling Magnetic Field and Salinity Upshock to Improve Polyhydroxyalkanoate Productivity by Haloferax mediterranei Feeding on Molasses Wastewater . | Applied and Environmental Microbiology , 2022 , 88 (13) .
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Occurrence of heterotrophic nitrification-aerobic denitrification induced by decreasing salinity in a halophilic AGS SBR treating hypersaline wastewater SCIE
期刊论文 | 2022 , 431 | CHEMICAL ENGINEERING JOURNAL
WoS CC Cited Count: 33
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Abstract :

Heterotrophic nitrification-aerobic denitrification (HN-AD) is a novel alternative for nitrogen removal due to simultaneous nitrification and denitrification that occurs under aerobic conditions. Until now, ways in which to achieve aerobic nitrogen removal from wastewater via the HN-AD process have not been fully explored. In this study, autotrophic nitrification was converted into HN-AD in a halophilic aerobic granular sludge (HAGS) system when the wastewater salinity decreased from 30 to 20 g/L. Bacteria affiliated to the genus Paracoccus were dominant in the HAGS with a relative abundance of 56%, functioning with HN-AD. Accordingly, the indicative gene napA encoding for HN-AD was 5.1 x 10(9) copies/g HAGS. HAGS performing HN-AD exhibited a stable total inorganic nitrogen (TIN) removal efficiency performance in response to salinity variations of 10-40 g/L, owing to the stable HN-AD functional community. The significant inhibition of HN-AD was observed in both low salinity (& LE;5 g/L) and high salinity (& GE;50 g/L) conditions, accompanied by the disintegration of granules. Granular disintegration was triggered by the lower secretion of extracellular polymeric substances and alginate-like exopolysaccharides. HAGS performing HN-AD could simultaneously remove chemical oxygen demand and TIN from saline wastewater in a single aerobic tank, thus reducing the construction and operation costs.

Keyword :

Halophilic AGS Halophilic AGS Paracoccus Paracoccus Salinity shock Salinity shock Heterotrophic nitrification-aerobic denitrification Heterotrophic nitrification-aerobic denitrification Species succession Species succession

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GB/T 7714 Huang, Ji-Lin , Cui, You-Wei , Yan, Jin-Lei et al. Occurrence of heterotrophic nitrification-aerobic denitrification induced by decreasing salinity in a halophilic AGS SBR treating hypersaline wastewater [J]. | CHEMICAL ENGINEERING JOURNAL , 2022 , 431 .
MLA Huang, Ji-Lin et al. "Occurrence of heterotrophic nitrification-aerobic denitrification induced by decreasing salinity in a halophilic AGS SBR treating hypersaline wastewater" . | CHEMICAL ENGINEERING JOURNAL 431 (2022) .
APA Huang, Ji-Lin , Cui, You-Wei , Yan, Jin-Lei , Cui, Yuan . Occurrence of heterotrophic nitrification-aerobic denitrification induced by decreasing salinity in a halophilic AGS SBR treating hypersaline wastewater . | CHEMICAL ENGINEERING JOURNAL , 2022 , 431 .
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Promoting enrichment of sulfur-oxidizing autotrophic denitrifiers via static magnetic fields: Performance and mechanism of magnetic biological effects SCIE
期刊论文 | 2022 , 347 | BIORESOURCE TECHNOLOGY
WoS CC Cited Count: 23
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Abstract :

Sulfur-driven autotrophic denitrification (SADN) is a promising technology for nitrogen removal from wastewater. In this study, different-strength SMFs (0, 5, 20, 50, 70 mT) were evaluated to investigate the potential of external static magnetic field (SMF) for enriching sulfur-oxidizing autotrophic denitrifiers (SOAD). 50-mT and 70-mT SMFs were most suitable to accelerate the growth of SOAD and the elimination of non-SOAD. The relative abundance of Thiobacillus significantly increased (p < 0.01) from 6.26% in control reactor to 36.15% under 50 mT and 52.51% under 70 mT. Under 50 mT, Thiobacillus denitrificans accumulated most rapidly, with the largest population. Furthermore, functional gene forecast by high-throughput and metagenomic sequencing indicated that SMF changed the two-component system, the adenosine 5'-monophosphate-activated protein kinase (AMPK) signaling system, the phosphotransferase system (PTS), as well as N/S-related enzymes to regulate stress response and promote the growth of SOAD. The findings indicated that SMF accelerated the start-up of SADN.

Keyword :

Magnetic biological effect Magnetic biological effect Magnetic induction mechanism Magnetic induction mechanism Magnetic field Magnetic field Enrichment of functional bacteria Enrichment of functional bacteria Sulfur-driven autotrophic denitrification Sulfur-driven autotrophic denitrification

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GB/T 7714 Yan, Hui-Juan , Cui, You-Wei , Han, Shi-Cai . Promoting enrichment of sulfur-oxidizing autotrophic denitrifiers via static magnetic fields: Performance and mechanism of magnetic biological effects [J]. | BIORESOURCE TECHNOLOGY , 2022 , 347 .
MLA Yan, Hui-Juan et al. "Promoting enrichment of sulfur-oxidizing autotrophic denitrifiers via static magnetic fields: Performance and mechanism of magnetic biological effects" . | BIORESOURCE TECHNOLOGY 347 (2022) .
APA Yan, Hui-Juan , Cui, You-Wei , Han, Shi-Cai . Promoting enrichment of sulfur-oxidizing autotrophic denitrifiers via static magnetic fields: Performance and mechanism of magnetic biological effects . | BIORESOURCE TECHNOLOGY , 2022 , 347 .
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A~2/O硫自养反硝化处理低碳氮比废水计量学研究 CSCD
期刊论文 | 2021 , 47 (07) , 118-122 | 水处理技术
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针对日益提升的污水处理氮排放标准使低碳氮比污水的深度脱氮遇到严峻考验的问题,以实际生活污水为处理对象,通过长期的实验研究硫自养反硝化滤池(简称硫池)脱氮性能和对TN去除的贡献。结果表明,当硫池的水力停留时间不低于1.4 h时,NO_x~--N的去除率能达到100%,硫池的NO_x~--N最高去除负荷为0.25 kg/(m~3·d)。硫池的硫酸根生成量和硝酸氮去除量的质量浓度比(Δρ(SO_4~(2-))/Δρ(NO_3~--N))为6.50,低于理论的7.54,表明硫池还存在着部分异养反硝化或异养硫酸盐还原作用,或硫的不完全氧化。可为低碳氮比实际污水的深度脱氮提供现实依据。

Keyword :

硫自养反硝化 硫自养反硝化 去除负荷 去除负荷 深度脱氮 深度脱氮 贡献率 贡献率 硫酸盐 硫酸盐

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GB/T 7714 徐康康 , 闫慧娟 , 崔有为 . A~2/O硫自养反硝化处理低碳氮比废水计量学研究 [J]. | 水处理技术 , 2021 , 47 (07) : 118-122 .
MLA 徐康康 et al. "A~2/O硫自养反硝化处理低碳氮比废水计量学研究" . | 水处理技术 47 . 07 (2021) : 118-122 .
APA 徐康康 , 闫慧娟 , 崔有为 . A~2/O硫自养反硝化处理低碳氮比废水计量学研究 . | 水处理技术 , 2021 , 47 (07) , 118-122 .
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一株异养硝化-好氧反硝化嗜盐菌及其在环境保护中的应用 incoPat
专利 | 2021-01-29 | CN202110120552.6
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本发明属于微生物技术领域。菌株于2020年11月18日保藏于中国微生物菌种保藏管理委员会普通微生物中心,保藏编号为CGMCC No.21200。墨西哥微小杆菌SND‑01是一株异养硝化‑好氧反硝化嗜盐菌株,在温度20‑40℃、盐度10‑100g/L、C/N=4‑20、溶解氧3‑5mg/L下,利用有机碳源将水中的无机氮转化成氮气,实现含盐废水的同步硝化反硝化脱氮。将本发明提供的菌株接种到含盐废水中,对氨氮、硝酸盐氮和亚硝酸盐氮的去除率分别为93%、100%和100%;同步去除氨氮、硝酸盐氮和亚硝酸盐氮时,氮去除率达到100%。该菌株可以应用在水体修复、河道治理、污水处理等环境保护领域。

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GB/T 7714 崔有为 , 崔媛 . 一株异养硝化-好氧反硝化嗜盐菌及其在环境保护中的应用 : CN202110120552.6[P]. | 2021-01-29 .
MLA 崔有为 et al. "一株异养硝化-好氧反硝化嗜盐菌及其在环境保护中的应用" : CN202110120552.6. | 2021-01-29 .
APA 崔有为 , 崔媛 . 一株异养硝化-好氧反硝化嗜盐菌及其在环境保护中的应用 : CN202110120552.6. | 2021-01-29 .
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一种促进好氧颗粒污泥快速形成的连续流运行方法 incoPat
专利 | 2021-01-25 | CN202110093244.9
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本发明公开一种促进好氧颗粒污泥快速形成的连续流反应器装置及运行方法,装置包括反应器主体、进水系统、曝气系统、沉淀系统、污泥回流系统,反应器主体可放置若干个可移动挡板,沉淀系统由中部可移动挡板分隔。可移动挡板的设置使得曝气盘曝出的气体定向流动,使泥水混合物被迫在曝气区做纵向往复的“S”型流态,为污泥提供了更强的和更规则的水力剪切力,促进微生物碰撞聚集,并分泌大量胞外聚合物,促进好氧颗粒污泥的形成。位于双沉淀池的中部可移动挡板的高度决定了沉淀时间,其可在颗粒化过程中灵活调整沉淀时间,选择性排泥。本发明结构简单且灵活多变,能在连续不间歇的进水和出水条件下快速形成好氧颗粒污泥。

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GB/T 7714 崔有为 , 闫金磊 . 一种促进好氧颗粒污泥快速形成的连续流运行方法 : CN202110093244.9[P]. | 2021-01-25 .
MLA 崔有为 et al. "一种促进好氧颗粒污泥快速形成的连续流运行方法" : CN202110093244.9. | 2021-01-25 .
APA 崔有为 , 闫金磊 . 一种促进好氧颗粒污泥快速形成的连续流运行方法 : CN202110093244.9. | 2021-01-25 .
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