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学者姓名：周志伟
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Abstract ：
Evaporation has been one of the most classic desalination processes on the Earth. When we try to use the power of water flow itself, the evaporation process can perform even better. Here, we report a hydrodynamic solardriven interfacial evaporation process which water evaporation rate can achieve 6.58 kg & sdot;m(-2)& sdot;h(-1) (over 100 times higher than natural evaporation). A waterwheel-structure solar interfacial evaporator was designed and assembled by printed filter papers. The evaporator can both rapidly distribute solution on the evaporation interface and be hydraulically driven to rotate continuously to improve the evaporation rate by water flow. The hydrodynamic solar-driven interfacial evaporation process successfully overcomes the problem of slow diffusion of water vapor, but also realizes the day-and-night operation of process and the self-cleaning of salt fouling. Apart from the application in solar desalination, the developed evaporator has great potentials in vapor production and salt recovery for industrial use.
Keyword ：
Salt fouling removal Salt fouling removal Day-and-night operation Day-and-night operation Hydrodynamic evaporation system Hydrodynamic evaporation system Ultra-high evaporation rate Ultra-high evaporation rate Dynamic solar-driven interfacial evaporation Dynamic solar-driven interfacial evaporation Waterwheel evaporator Waterwheel evaporator
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| GB/T 7714 | Ren, Jiawei , Xu, Jia , Tian, Shuangchao et al. Hydrodynamic solar-driven interfacial evaporation - Gone with the flow [J]. | WATER RESEARCH , 2024 , 266 . |
| MLA | Ren, Jiawei et al. "Hydrodynamic solar-driven interfacial evaporation - Gone with the flow" . | WATER RESEARCH 266 (2024) . |
| APA | Ren, Jiawei , Xu, Jia , Tian, Shuangchao , Shi, Ke , Gu, Tianyu , Zhao, Jiaheng et al. Hydrodynamic solar-driven interfacial evaporation - Gone with the flow . | WATER RESEARCH , 2024 , 266 . |
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Abstract ：
Biofouling is a major challenge limiting the practical application of biofiltration-facilitated gravity-driven membrane (GDM) systems in drinking water treatment. In this study, ultraviolet irradiation, including ultraviolet (UV) and vacuum ultraviolet (VUV) irradiation, was used for in-situ purification of membrane tanks to control membrane biofouling. After using UV and VUV, the permeate flux increased significantly by 26.1% and 78.3%, respectively, which was mainly due to the decreased cake layer resistance (Rc). The permeability of the biofouling layer improved after UV and VUV application, as evidenced by the increased surface porosity and decreased thickness. The contents of loosely bound extracellular proteins (LB-PN) and tightly bound extracellular proteins (TB-PN) in the biofouling layer were reduced after UV and VUV irradiation. The decreased LB-PN and TB-PN improved the interfacial free energy between the fouling itself and between the fouling and the membrane, which contributed to the reduction of interfacial cohesion and adhesion, resulting in a looser and thinner biofouling layer and a cleaner membrane. The concentration of protein-like material in the membrane tank decreased after UV and VUV irradiation, significantly altering the bacterial community structure on the membrane surface (Mantel's r > 0.7, p < 0.05). The changes in the metabolic state were responsible for the differences in the LB-PN and TB-PN contents. The inhibition of "Alanine, aspartate and glutamate metabolism" and "Glycine, serine and threonine metabolism" reduced amino acid biosynthesis, which restricted the secretion of LB-PN and TB-PN. Critical genera in the Proteobacteria phylum, such as Hirschia, Rhodobacter, Nordella, Candidatus_Berkiella, and Limnohabitans, were involved in metabolite transformation. Overall, the in-situ application of UV and VUV can be an effective alternative strategy to mitigate membrane biofouling, which would facilitate the practical application of biofiltration-facilitated GDM systems in drinking water treatment.
Keyword ：
Metabolic pathway Metabolic pathway Gravity-driven membrane (GDM) Gravity-driven membrane (GDM) Ultraviolet (UV) Ultraviolet (UV) Interface free energy Interface free energy Extracellular polymeric substances (EPS) Extracellular polymeric substances (EPS) Vacuum ultraviolet (VUV) Vacuum ultraviolet (VUV)
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| GB/T 7714 | Feng, Jianyong , Li, Xing , Lu, Zedong et al. Enhanced permeation performance of biofiltration-facilitated gravity-driven membrane (GDM) systems by in-situ application of UV and VUV: Comprehensive insights from thermodynamic and multi-omics perspectives [J]. | WATER RESEARCH , 2023 , 242 . |
| MLA | Feng, Jianyong et al. "Enhanced permeation performance of biofiltration-facilitated gravity-driven membrane (GDM) systems by in-situ application of UV and VUV: Comprehensive insights from thermodynamic and multi-omics perspectives" . | WATER RESEARCH 242 (2023) . |
| APA | Feng, Jianyong , Li, Xing , Lu, Zedong , Yang, Yanling , Zhou, Zhiwei , Liang, Heng . Enhanced permeation performance of biofiltration-facilitated gravity-driven membrane (GDM) systems by in-situ application of UV and VUV: Comprehensive insights from thermodynamic and multi-omics perspectives . | WATER RESEARCH , 2023 , 242 . |
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Abstract ：
This study investigated the ultrasonic-thermal regeneration of powdered activated carbon (PAC) spent using 4-chlorophenol (4-CP). Similarly, a thermal regeneration process was also studied and the reaction conditions (i.e., regeneration temperature, heating rate, regeneration time) were tested. Fourier transform infrared spectroscopy (FT-IR), thermogravimetric analysis (TGA), scanning electron microscopy (SEM), X-ray photoelectron spectroscopy (XPS) and X-ray diffraction (XRD) analysis were applied to characterize the regenerated PACs under different treatments (thermal, ultrasonic and ultrasonic-thermal) and also compare them with the fresh and exhausted PACs. According to our regeneration observations, the ideal regeneration parameters were determined to be a 40 kHz frequency, 0.18 W/mL sonication power, 0.1 M NaOH and 50% (v/v) ethyl alcohol as the regeneration solution, and 1 g/L of saturated PAC mass with thermal regeneration as the second stage at 500 ?, desorbed for 30 min with a heating rate of 20 ? min(-1). Under these conditions, the RE value achieved 90.99% and the ? value reached 5.6%. The results of FTIR, XPS and XRD revealed that the oxygen functional group content of ultrasonic-thermal regenerated PAC significantly increased. These oxygenous groups exerted a positive effect on the adsorption process of the regenerated PAC and the subsequent adsorption-regeneration process.
Keyword ：
characteristic characteristic powdered activated carbon powdered activated carbon thermal thermal ultrasonic ultrasonic regeneration regeneration
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| GB/T 7714 | Zhang, Tingting , Yang, Yanling , Li, Xing et al. Ultrasonic-Thermal Regeneration of Spent Powdered Activated Carbon [J]. | SUSTAINABILITY , 2023 , 15 (11) . |
| MLA | Zhang, Tingting et al. "Ultrasonic-Thermal Regeneration of Spent Powdered Activated Carbon" . | SUSTAINABILITY 15 . 11 (2023) . |
| APA | Zhang, Tingting , Yang, Yanling , Li, Xing , Zhou, Zhiwei , Wei, Bigui . Ultrasonic-Thermal Regeneration of Spent Powdered Activated Carbon . | SUSTAINABILITY , 2023 , 15 (11) . |
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Abstract ：
In this study, a novel composite based on bismuth oxide, reduced graphene oxide and titanium dioxide (labeled as BRGT) was utilized for visible light photocatalysis to mitigate ultrafiltration membrane fouling caused by natural organic matter (NOM). The results show that the coexistence of NOM and the BRGT composite (without photocatalysis) did not aggravate membrane fouling, and the membrane preferentially retained a high molecular weight, hydrophobic component of NOM that formed a dense cake layer with BRGT composite. As the photo-catalysis time increased, the extent of membrane fouling was alleviated. The maximum specific flux recovered from 0.21 to 0.73 at 60 min, and the hydraulic reversible and irreversible resistances ere 1.15 x 1010 and 4.23 x 1010 m-1, respectively. The reduction of NOM in the feed water, especially the removal of UV254, played a significant role in the alleviation of membrane fouling. Additionally, the changes in the properties of NOM, including the reduction of fluorescent humic and protein/polyphenol components corresponding to reversible and irreversible fouling, respectively, the photo-degradation of high molecular weight NOM into low molecular weight NOM (such as low molecular weight-acids), and the conversion of hydrophobic fractions into hydrophilic fractions, contributed to the mitigation of membrane fouling. We also found a strong negative correlation be-tween the roughness of the cake layer and irreversible fouling. Overall, the changes in the properties of NOM in feed water can hinder or even inhibit the formation of the cake layer, and the use of visible light photocatalysis of the BRGT composite has great potential to alleviate ultrafiltration membrane fouling caused by natural organic matter.
Keyword ：
Mechanism of fouling development Mechanism of fouling development Fouling mitigation Fouling mitigation Ultrafiltration Ultrafiltration Natural organic matter Natural organic matter Visible light photocatalysis Visible light photocatalysis
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| GB/T 7714 | Yu, Rui , Yang, Yanling , Zhou, Zhiwei et al. Role of visible light photocatalysis in alleviation and mechanism transformation of ultrafiltration membrane fouling caused by natural organic matter [J]. | SEPARATION AND PURIFICATION TECHNOLOGY , 2023 , 324 . |
| MLA | Yu, Rui et al. "Role of visible light photocatalysis in alleviation and mechanism transformation of ultrafiltration membrane fouling caused by natural organic matter" . | SEPARATION AND PURIFICATION TECHNOLOGY 324 (2023) . |
| APA | Yu, Rui , Yang, Yanling , Zhou, Zhiwei , Li, Xing , Liu, Chunjiao , Sun, Tianjie . Role of visible light photocatalysis in alleviation and mechanism transformation of ultrafiltration membrane fouling caused by natural organic matter . | SEPARATION AND PURIFICATION TECHNOLOGY , 2023 , 324 . |
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Abstract ：
Natural organic matter (NOM) can impede the removal of organic micro-pollutants (OMPs) through several mechanisms, including inner filter effect, competition with the target OMP, and radical scavenging, during synchronous adsorption/photocatalysis of multi-functional composites. In this study, the fate and inhibitory mechanisms of sulfamerazine (SMZ, a model OMP) that occurred in presence of seven different NOM samples (i.e. three standard NOM surrogates, a river water sample, a carbon filter effluent and two different sand filter effluents) during the adsorption/photocatalysis by a composite of Bi2O3-TiO2 supported on powdered activated carbon (Bi2O3-TiO2/PAC, abbreviated as BTP) when exposed to visible light irradiation were revealed. The results indicated that adsorption played a greater attribution than photocatalysis on SMZ removal. The primary impediment to the adsorption and photocatalytic degradation of SMZ was attributed to the presence of terrestrial-derived, humic-like NOM fractions with high aromaticity. The adsorption efficacy of SMZ was weakened by the absorption of NOM and its degradation products onto the BTP surface. The inner filter effect, competition between NOM and SMZ, and radical scavenging were responsible for the reduced photocatalysis of SMZ. In the cases of real water matrices, the presence of inorganic anion and co-existed NOM reduced the removal of SMZ. In summary, the findings of this work offer a comprehensive comprehension of the impact of NOM fractions on photocatalysis, emphasizing the necessity to examine the interplay between NOM and background inorganic constituents in the degradation of OMP via adsorption/photocatalysis.
Keyword ：
inhibition inhibition Bi2O3-TiO2 Bi2O3-TiO2 PAC composite PAC composite multi-functional composite multi-functional composite natural organic matter natural organic matter adsorption and photocatalysis adsorption and photocatalysis
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| GB/T 7714 | Zhou, Zhiwei , Zhang, Ruixin , Yang, Yanling et al. Fate of sulfamerazine by synchronous adsorption and photocatalysis dependent on natural organic matter properties [J]. | ENVIRONMENTAL TECHNOLOGY , 2023 , 45 (18) : 3635-3647 . |
| MLA | Zhou, Zhiwei et al. "Fate of sulfamerazine by synchronous adsorption and photocatalysis dependent on natural organic matter properties" . | ENVIRONMENTAL TECHNOLOGY 45 . 18 (2023) : 3635-3647 . |
| APA | Zhou, Zhiwei , Zhang, Ruixin , Yang, Yanling , Li, Xing , Ren, Jiawei . Fate of sulfamerazine by synchronous adsorption and photocatalysis dependent on natural organic matter properties . | ENVIRONMENTAL TECHNOLOGY , 2023 , 45 (18) , 3635-3647 . |
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Abstract ：
In this study, persulphate and nanoscale zero-valent iron were activated by ultraviolet irradiation (PS/nZVI/UV), followed by formation of dynamic flocs with AlCl3-TiCl4 coagulant directly injected into a gravity-driven membrane (GDM) tank. Membrane fouling caused by typical organic matter fractions including humic acid (HA), HA together with bovine serum albumin (HA-BSA), HA combined with polysaccharide (HA-SA) and the HA-BSA-SA mixture at pH of 6.0, 7.5 and 9.0 were evaluated by specific flux and fouling resistance distribution. The results showed that GDM pre-layered with AlCl3-TiCl4 flocs exhibited the maximum specific flux, followed by AlCl3 and TiCl4. Pre-oxidation with 0.5 mM PS and 0.1 g nZVI under UV radiation for 20 min was beneficial to degrade HA and SA fraction with molecular weight >100 kDa and <30 kDa, and BSA fraction with <30 kDa. The presence of BSA attributed mostly to irreversible fouling, SA together with BAS could exacerbate irreversible fouling, while HA caused the least fouling. The irreversible resistance of a PS/nZVI/UV-GDM system was 62.79%, 27.27%, 58.03% and 49.68% lower than that of control GDM in the treatment of HA, HA-BSA, HA-SA and HA-BSA-SA, respectively. The PS/nZVI/UV-GDM system could achieve the highest foulants removal efficiency at pH of 6.0. Morphological observations confirmed the differences in biofouling layers in different water types. Over 30-day operation, the bacterial genera on the biofouling layer could affect the organic removals, while the type of organic matter that was present influenced the relative abundance of bacterial genera.
Keyword ：
Gravity-driven membrane Gravity-driven membrane nanoscale zero-valent iron nanoscale zero-valent iron flocs layer flocs layer biofouling layer biofouling layer ultraviolet (PS ultraviolet (PS nZVI nZVI persulphate persulphate NOM fractions NOM fractions UV) UV)
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| GB/T 7714 | Zhao, Fuwang , Zhou, Zhiwei , Du, Peng et al. Reduction of fouling of gravity-driven membrane by combined treatment of persulphate/nanoscale zero-valent iron/ultraviolet and dynamic dual coagulant flocs layer [J]. | ENVIRONMENTAL TECHNOLOGY , 2023 , 45 (17) : 3405-3417 . |
| MLA | Zhao, Fuwang et al. "Reduction of fouling of gravity-driven membrane by combined treatment of persulphate/nanoscale zero-valent iron/ultraviolet and dynamic dual coagulant flocs layer" . | ENVIRONMENTAL TECHNOLOGY 45 . 17 (2023) : 3405-3417 . |
| APA | Zhao, Fuwang , Zhou, Zhiwei , Du, Peng , Li, Xing , Lu, Qingxuan . Reduction of fouling of gravity-driven membrane by combined treatment of persulphate/nanoscale zero-valent iron/ultraviolet and dynamic dual coagulant flocs layer . | ENVIRONMENTAL TECHNOLOGY , 2023 , 45 (17) , 3405-3417 . |
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Abstract ：
This study evaluated a long-term impact of biological activated carbon (BAC) filter that was employed in a fullscale drinking water treatment plant to enhance the removal of contaminants by the ultrafiltration (UF) process. The results showed that BAC enhanced UF performance by increasing the flux by 18.5% and extending the filtration run by 45%. The presence of BAC improved the removal of primary contaminants, including dissolved organic carbon (4-40%), UV254 (10-57.7%), geosmin and 2-methylisoborneol (80%). BAC was also effective in decreasing the concentration of biopolymers, humic substances, (semi-)volatile organics, chlorite and halonitromethanes, thereby lowering contaminant load on the UF unit. The changes in primary water quality parameters in the combined process showed that the humic substances in dissolved organic nitrogen, low molecular weight substances in UV254, and fluorescence protein-like substances could be useful indicators for DBPs as these organic fractions had strong correlation with DBPs. Obvious spatio-temporal characteristics of GAC grain and microbial communities in BAC filter were observed with operation time and filter depth. The bacterial community in BAC filter was highly diverse and was less influenced by influent quality with an increase in filter depth, while the communities in UF cake layer correlated with organic removal in the UF system.
Keyword ：
Ultrafiltration Ultrafiltration Bacterial community Bacterial community Biological activated carbon (BAC) Biological activated carbon (BAC) Disinfection byproduct formation potential (DBPFP) Disinfection byproduct formation potential (DBPFP) Organic fractions Organic fractions
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| GB/T 7714 | Chang, Haiqing , Yu, Haikuan , Li, Xing et al. Role of biological granular activated carbon in contaminant removal and ultrafiltration membrane performance in a full-scale system [J]. | JOURNAL OF MEMBRANE SCIENCE , 2022 , 644 . |
| MLA | Chang, Haiqing et al. "Role of biological granular activated carbon in contaminant removal and ultrafiltration membrane performance in a full-scale system" . | JOURNAL OF MEMBRANE SCIENCE 644 (2022) . |
| APA | Chang, Haiqing , Yu, Haikuan , Li, Xing , Zhou, Zhiwei , Liang, Heng , Song, Wuchang et al. Role of biological granular activated carbon in contaminant removal and ultrafiltration membrane performance in a full-scale system . | JOURNAL OF MEMBRANE SCIENCE , 2022 , 644 . |
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Abstract ：
It is a critical challenge for drinking water production when treating algae-contaminated surface water. In this study, the impact of in situ coagulation (C), activated alumina filtration (AA) and their combination (CAA) on the performance of gravity-driven membrane (GDM) was systematically assessed during 105-day operation. The results indicated that pretreatments in particular CAA could effectively enhance GDM flux, and the stable fluxes were increased to 3.1, 4.9 and 8.3 L/(m(2).h) (LMH) for CGDM, AA/GDM and CAA/GDM, respectively when compared to the control GDM (2.0 LMH). Coagulation was beneficial to formation of thick but loose biofouling layer, while AA filtration was effective to retain foulants including extracellular polymeric substances (EPS), organics, total nitrogen and total phosphorus. The CAA/GDM could mostly remove these foulants, and facilitate the proliferation of bacterial genera that could consume EPS, further alleviating membrane fouling. The dif-ference in loosely bound EPS and tightly bound EPS of biofouling layer attributed to the difference of reversible fouling and irreversible fouling, respectively. Morphological observations, variation in functional groups or el-ements further confirmed the difference in biological layers in different GDM systems. The occurrence of specific bacterial genera involving the potential to degrade protein, chitin and other high molecular weight organics was responsible for contaminant removals.
Keyword ：
In situ coagulation In situ coagulation Biofouling layer Biofouling layer Gravity-driven membrane (GDM) Gravity-driven membrane (GDM) Flux stabilization Flux stabilization Bacterial community Bacterial community Extracellular polymeric substances (EPS) Extracellular polymeric substances (EPS)
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| GB/T 7714 | Du, Peng , Li, Xing , Yang, Yanling et al. Regulated-biofilms enhance the permeate flux and quality of gravity-driven membrane (GDM) by in situ coagulation combined with activated alumina filtration [J]. | WATER RESEARCH , 2022 , 209 . |
| MLA | Du, Peng et al. "Regulated-biofilms enhance the permeate flux and quality of gravity-driven membrane (GDM) by in situ coagulation combined with activated alumina filtration" . | WATER RESEARCH 209 (2022) . |
| APA | Du, Peng , Li, Xing , Yang, Yanling , Zhou, Zhiwei , Fan, Xiaoyan , Chang, Haiqing et al. Regulated-biofilms enhance the permeate flux and quality of gravity-driven membrane (GDM) by in situ coagulation combined with activated alumina filtration . | WATER RESEARCH , 2022 , 209 . |
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Abstract ：
本实用新型公开了一种基于高梯度磁分离的含藻水源水处理系统，所述水处理系统含有包括旋流分离器及电磁场发生装置的高梯度磁旋流分离装置(9)，其中，旋流分离器包括筒体(901)，位于筒体(901)底部的污泥出口管(902)，位于筒体(901)顶部的液体出口管(903)，位于筒体(901)上部一侧的入口管(904)，位于筒体(901)下部一侧的反冲洗管(905)和与其连通的反冲洗泵，电磁场发生装置(906)包括筒体(901)内的、含芯铁的可通电螺线管。本实用新型结构简单，不仅提高了磁性光催化剂的回收率，同时可显著促进后续的絮凝效果、节省絮凝剂的投加量，提高沉后水质。
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| GB/T 7714 | 田立平 , 王晓波 , 周志伟 et al. 基于高梯度磁分离的含藻水源水处理系统 : CN202221801015.4[P]. | 2022-07-12 . |
| MLA | 田立平 et al. "基于高梯度磁分离的含藻水源水处理系统" : CN202221801015.4. | 2022-07-12 . |
| APA | 田立平 , 王晓波 , 周志伟 , 刘春娇 , 于瑞 . 基于高梯度磁分离的含藻水源水处理系统 : CN202221801015.4. | 2022-07-12 . |
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Abstract ：
A Fe-doped graphite-like carbon nitride (g-C3N4) nanocomposites containing various Fe contents (5 wt.%, 10 wt. % and 15 wt.%) were prepared via two-step calcination thermal polymerization, and were employed as efficient heterogeneous photo-Fenton composites towards rhodamine B (RhB) removal in visible-light/H2O2 system. The sheet structure of g-C3N4 was refined down to nano-scale and less densely packed by the increasing Fe-doping ratio. X-ray diffraction (XRD), Fourier transform infrared (FTIR) and X-ray photoelectron spectroscopy (XPS) spectra indicated that Fe was doped completely into the g-C3N4 lattice. Over 90 %RhB was degraded in photo-Fenton system within 45 min under the optimal Fe-doping ratio of 10 wt.% (10 % Fe-g-C3N4). The degradation efficiency of photo-Fenton was superior in comparison with photocatalysis and Fenton reaction. The as-prepared composite exhibited excellent performance (similar to 90 % removal) and high stability in a wide range of pH value (3 similar to 9), and the degradation data well fitted with the pseudo-first-order kinetics model. The enhanced photo-Fenton catalytic activity benefited from the Z-scheme heterojunctions of Fe-g-C3N4, which improved the separation ability of photo-generated charge carriers and increased the electrons that participated in Fe2+/Fe3+ cycle. The main active oxygen species of Fe-g-C3N4 were hydroxyl radicals, followed by superoxide radicals and electron holes. The effect of Fe-doping was revealed by density functional theory calculation. The excellent recyclability and stability of Fe-g-C3N4 catalyst was also observed. Such photo-Fenton system was also effective to degrade other organic pollutants. The findings reported here offer promising implications in developing the utilization of Fe-g-C3N4 composite in photo-Fenton system for treatment of wastewater.
Keyword ：
RhB RhB Photo-Fenton Photo-Fenton Fe doped g-C3N4 Fe doped g-C3N4 Density functional theory (DFT) Density functional theory (DFT)
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| GB/T 7714 | Ji, Siyang , Yang, Yanling , Zhou, Zhiwei et al. Photocatalysis-Fenton of Fe-doped g-C3N4 catalyst and its excellent degradation performance towards RhB [J]. | JOURNAL OF WATER PROCESS ENGINEERING , 2021 , 40 . |
| MLA | Ji, Siyang et al. "Photocatalysis-Fenton of Fe-doped g-C3N4 catalyst and its excellent degradation performance towards RhB" . | JOURNAL OF WATER PROCESS ENGINEERING 40 (2021) . |
| APA | Ji, Siyang , Yang, Yanling , Zhou, Zhiwei , Li, Xing , Liu, Yuankun . Photocatalysis-Fenton of Fe-doped g-C3N4 catalyst and its excellent degradation performance towards RhB . | JOURNAL OF WATER PROCESS ENGINEERING , 2021 , 40 . |
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