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学者姓名：陈莎
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Abstract ：
Tetrabromobisphenol A (TBBPA) is a kind of widely used brominated flame retardant (BFR), which is proven to be harmful to ecological systems and public health. It is very important to remove TBBPA from the environment. In our study, a magnetic composite named Fe3O4/GO/ZIF-67 was synthesized by a coprecipitation method and applied in the highly efficient adsorption of TBBPA from water. Static adsorption experiments demonstrated that the adsorption capacity could reach 232 mgg-1 within 120 min, which is much higher than those reported in the other literature. The experimental results show that the adsorption of TBBPA on Fe3O4/GO/ZIF-67 followed Langmuir and pseudo-second-order kinetic adsorption models. The main mechanisms for these adsorptions were identified as hydrogen bonds between OH groups in TBBPA and COOHs of Fe3O4/GO/ZIF-67, and pi-pi stacking between Fe3O4/GO/ZIF-67 and TBBPA. This study provides a method with great promise for the design and synthesis of better adsorbents for the removal of TBBPA from the water environment.
Keyword ：
metal-organic frameworks metal-organic frameworks magnetic separation magnetic separation adsorption adsorption Fe3O4/GO/ZIF-67 Fe3O4/GO/ZIF-67 TBBPA TBBPA
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| GB/T 7714 | Li, Sumei , Ji, Jian , Shan, Saisai et al. Efficient Adsorption Removal of Tetrabromobisphenol A from Water by Using a Magnetic Composite Fe3O4/GO/ZIF-67 [J]. | CRYSTALS , 2024 , 14 (6) . |
| MLA | Li, Sumei et al. "Efficient Adsorption Removal of Tetrabromobisphenol A from Water by Using a Magnetic Composite Fe3O4/GO/ZIF-67" . | CRYSTALS 14 . 6 (2024) . |
| APA | Li, Sumei , Ji, Jian , Shan, Saisai , Chen, Sha , Li, Hanbing , Xu, Qian et al. Efficient Adsorption Removal of Tetrabromobisphenol A from Water by Using a Magnetic Composite Fe3O4/GO/ZIF-67 . | CRYSTALS , 2024 , 14 (6) . |
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Abstract ：
Synergetic energy-water-carbon pathways are key issues to be tackled under carbon-neutral target and high-quality development worldwide, especially in ecologically vulnerable regions (EVRs). In this study, to explore the synergistic pathways in an EVR, a water-energy-carbon assessment (WECA) model was built, and the synergistic effects of water-energy-carbon were comprehensively and quantitatively analyzed under various scenarios of regional transition. Shaanxi Province was chosen as the representative EVR, and Lower challenge (LEC) and Greater challenge (GER) scenarios of zero-carbon transition were set considering the technological maturity and regional energy characteristics. The results showed that there were limited effects under the zero-carbon transition of the entire region on reducing water withdrawals and improving the water quality. In the LEC scenario, the energy demand and CO2 emissions of Shaanxi in 2060 will decrease by 70.9% and 99.4%, respectively, whereas the water withdrawal and freshwater aquatic ecotoxicity potential (FAETP) will only decrease by 8.9% and 1.6%, respectively. This could be attributed to the stronger demand for electricity in the energy demand sector caused by industrial transition measures. The GER scenario showed significant growth in water withdrawals (16.0%) and FAETP (36.0%) because of additional biomass demand. To promote the synergetic development of regional transition, EVRs should urgently promote zero-carbon technologies (especially solar and wind power technologies) between 2020 and 2060 and dry cooling technology for power generation before 2030. In particular, a cautious attitude toward the biomass energy with carbon capture and storage technology in EVRs is strongly recommended.
Keyword ：
Water environment quality Water environment quality Water withdrawals Water withdrawals Ecologically vulnerable region Ecologically vulnerable region Typical regional transition Typical regional transition Carbon neutrality Carbon neutrality
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| GB/T 7714 | Liu, Yingying , Li, Hanbing , Chen, Sha et al. Synergetic pathways of water-energy-carbon in ecologically vulnerable regions aiming for carbon neutrality: a case study of Shaanxi, China [J]. | FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING , 2024 , 18 (9) . |
| MLA | Liu, Yingying et al. "Synergetic pathways of water-energy-carbon in ecologically vulnerable regions aiming for carbon neutrality: a case study of Shaanxi, China" . | FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING 18 . 9 (2024) . |
| APA | Liu, Yingying , Li, Hanbing , Chen, Sha , Zhang, Lantian , Li, Sumei , Lv, He et al. Synergetic pathways of water-energy-carbon in ecologically vulnerable regions aiming for carbon neutrality: a case study of Shaanxi, China . | FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING , 2024 , 18 (9) . |
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Abstract ：
Quantitatively analysing the impacts on regional water sustainability under the energy transition is vital to regional water management and specific technology selection, which is also relevant to dealing with climate change. This study proposed a new multi-indicator evaluation framework for regional water sustainability under local energy transition to quantitatively evaluate the water withdrawal and water environment during the energy transition from a lifecycle perspective. An integrated regional energy-water evaluation model was also developed based on the Low Emissions Analysis Platform with a combination of lifecycle assessment and water footprint analysis. Shaanxi province in China was then taken as a case study, and the impacts of its energy transition on regional water environmental sustainability, including quantity and quality, were investigated under five scenarios. Results showed that the large-scale application of carbon capture, utilisation and storage technology and bioenergy equipped with carbon capture and storage technology could have additional advantages regarding CO2 emissions. However, such technologies exhibit a minimal effect on improving water environmental quality and reducing water demand for the first time due to the leakage of absorbents, CO2 and other risky substances during capture, transportation and storage from a lifecycle perspective. This finding drives the innovation of related breakthrough technologies with the promotion of water and end-treatment technologies in the future.
Keyword ：
Transition path Transition path Water sustainability Water sustainability Energy-water nexus Energy-water nexus Spatial and temporal analyses Spatial and temporal analyses
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| GB/T 7714 | Zhang, Lan-Tian , Liu, Ying-Ying , Chen, Sha et al. Quantitative evaluation framework and application for regional water sustainability under local energy transition [J]. | ADVANCES IN CLIMATE CHANGE RESEARCH , 2023 , 14 (6) : 976-987 . |
| MLA | Zhang, Lan-Tian et al. "Quantitative evaluation framework and application for regional water sustainability under local energy transition" . | ADVANCES IN CLIMATE CHANGE RESEARCH 14 . 6 (2023) : 976-987 . |
| APA | Zhang, Lan-Tian , Liu, Ying-Ying , Chen, Sha , Li, Han-Bing , Li, Su-Mei , Jiang, Ke-Jun et al. Quantitative evaluation framework and application for regional water sustainability under local energy transition . | ADVANCES IN CLIMATE CHANGE RESEARCH , 2023 , 14 (6) , 976-987 . |
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Abstract ：
Purpose A three-way catalytic converter (TWC) is a type of pollution control product (PCP) that has been widely used to reduce the emission of carbon monoxide (CO), total hydrocarbon (THC), and nitrogen oxides (NOx) from vehicles. TWC's decreasing removal efficiency as a result of their aging condition can have a substantial impact on their environmental benefits. The goal of this paper is to evaluate the dynamic environmental impacts of TWC during its whole life cycle. Methods Dynamic emission factors of pollutants from the rapid aging (RA) test and the real vehicle aging (RVA) test were firstly analyzed. Then, the dynamic environmental benefits and dynamic environmental burdens of TWC during its whole life cycle were evaluated by a dynamic life cycle assessment (DLCA) method. Impact categories assessed included global warming potentials (GWP), acidification potentials (AP), human toxicity potentials (HTP), photochemical smog potentials (POCP), and abiotic resource depletion potentials (ADPs). Results and discussion Dynamic emission factors of vehicle pollutants collected from the rapid aging (RA) test and the real vehicle aging (RVA) test indicate that CO had the highest emission amounts compared to NOx and THC. Results in AP, HTP, and POCP showed that the environmental benefits of TWC in the RVA test were 76.24, 1.03, and 2743 times greater than its burdens. The difference in AP, HTP, and POCP between RVA and RA tests was 0.39%, 0.39%, and 0.97%, showing no significant variations from these two tests to evaluate the environmental benefits. Dynamic environmental burdens allowed for a 51.36% increase in HTP compared to static environmental burdens of TWC. Conclusions Both RVA and RA tests are suitable methods to acquire the dynamic data in the dynamic life cycle assessment of TWC. Our results proved the more precise evaluation of dynamic environmental burdens in reflecting the performance of TWC in real driving circumstances.
Keyword ：
Pollution control products Pollution control products Dynamic emission factors Dynamic emission factors Environmental benefits Environmental benefits Dynamic life cycle assessment Dynamic life cycle assessment Real vehicle aging test Real vehicle aging test Rapid aging test Rapid aging test
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| GB/T 7714 | Liu, Yingying , Li, Hanbing , Chen, Sha et al. Dynamic evaluation of environmental impact for three-way catalytic converter with temporal variation life cycle method [J]. | INTERNATIONAL JOURNAL OF LIFE CYCLE ASSESSMENT , 2022 , 27 (9-11) : 1170-1179 . |
| MLA | Liu, Yingying et al. "Dynamic evaluation of environmental impact for three-way catalytic converter with temporal variation life cycle method" . | INTERNATIONAL JOURNAL OF LIFE CYCLE ASSESSMENT 27 . 9-11 (2022) : 1170-1179 . |
| APA | Liu, Yingying , Li, Hanbing , Chen, Sha , Zhang, Yana , Lv, He , Yan, Shuqi et al. Dynamic evaluation of environmental impact for three-way catalytic converter with temporal variation life cycle method . | INTERNATIONAL JOURNAL OF LIFE CYCLE ASSESSMENT , 2022 , 27 (9-11) , 1170-1179 . |
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Abstract ：
本发明公开了一种综合环境和营养效益的新型食物当量的计算方法及应用，通过一次计算需要营养素修正系数和限制营养素修正系数、食物的热量评分和营养评分、营养修正系数，得出新型食物当量，可以评价食物领域温室气体排放量、水足迹等环境影响，也可以新型食物当量为方法学基础，计算基于生命周期的食物的全球变暖潜势、酸化潜势、富营养化潜势、臭氧消耗潜势、非生物性消耗(元素)、非生物性消耗(化石)、水生态毒性潜势、人体生态毒性潜势、光化学臭氧生成潜势和陆地生态毒性潜势等环境影响，能有效的对比各类食物的环境和健康效益，对于食物的温室气体排放核算、碳减排路径和健康效益的分析对比十分有效，应用价值较高。
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| GB/T 7714 | 陈莎 , 张孟蓉 , 李素梅 et al. 一种综合环境和营养效益的新型食物当量的计算方法及应用 : CN202211217352.3[P]. | 2022-10-03 . |
| MLA | 陈莎 et al. "一种综合环境和营养效益的新型食物当量的计算方法及应用" : CN202211217352.3. | 2022-10-03 . |
| APA | 陈莎 , 张孟蓉 , 李素梅 , 李寒冰 , 刘影影 , 麦兴宇 . 一种综合环境和营养效益的新型食物当量的计算方法及应用 : CN202211217352.3. | 2022-10-03 . |
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Abstract ：
As anthropogenic antibiotics, quinolones, e.g., ofloxacin have adverse impacts on ecological systems and human heaths. The removal of quinolones is of great importance, and adsorption techniques have been widely used to remove this hazardous contaminant. However, a robust and easy-operating adsorbent is still emergently required due to the complex chemical structure of quinolones. In this study, we successfully synthesized the promising metallic carbons (MCs) containing carbon nanotubes and cobalt nanoparticles by carbonizing Zn/Co-ZIF at 900 degrees C. Three different molar ratios of Co and Zn were applied to optimize the adsorption capacity on ofloxacin (OFL). Results showed MC with molar ratio of Co and Zn at 3:1 (Co-CNT/NPC3/1) achieved the maximal adsorption capacity to 118.3 mg g-1. Its adsorption performance was satisfied in the pH range from 5 to 9 and ionic strengths at 0.01 M. The main mechanisms for these adsorptions were identified as electrostatic attraction, metal coordination and pi-pi EDA. Removal efficiencies of quinolones higher than 68 mg g-1 indicated the strong feasibility of this adsorbent for wastewater treatments. The regeneration of Co-CNT/NPC3/1 at 600 degrees C allowed its at least 4-time reusability and its magnetic property enabled external magnets to recycle it from real environments.
Keyword ：
Magnetic separation Magnetic separation Adsorption Adsorption Zn Zn Co zeolitic imidazolate frameworks Co zeolitic imidazolate frameworks Metallic carbides Metallic carbides
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| GB/T 7714 | Liang, Yixuan , Zhang, Qiyu , Li, Sumei et al. Highly efficient removal of quinolones by using the easily reusable MOF derived-carbon [J]. | JOURNAL OF HAZARDOUS MATERIALS , 2022 , 423 . |
| MLA | Liang, Yixuan et al. "Highly efficient removal of quinolones by using the easily reusable MOF derived-carbon" . | JOURNAL OF HAZARDOUS MATERIALS 423 (2022) . |
| APA | Liang, Yixuan , Zhang, Qiyu , Li, Sumei , Fei, Jiaying , Zhou, Jian , Shan, Saisai et al. Highly efficient removal of quinolones by using the easily reusable MOF derived-carbon . | JOURNAL OF HAZARDOUS MATERIALS , 2022 , 423 . |
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Abstract ：
Around 6.6 million tons of spent coffee is produced per year, resulting in resources loss and potential environmental risks. Hence, a green technique is required to reuse the spent coffee grains. In this study, coffee grounds were burnt at 900 degrees C to generate the biochar (BC) for the synthesis of the porous adsorbent (ZIF-8 @BC) by growing ZIF-8 on the surface of BC. We applied the well-prepared ZIF-8 @BC to remove Congo red (CR) in water. The maximum adsorption capacity of ZIF-8 @BC on Congo red in water was up to 1080.4 mg/g, which was significantly higher than that of many different types of BCs reported in previous studies. The reasons for its highly efficient adsorption of CR probably was attributed to metal ions and coordinatively unsaturated sites in the material. Also, BC enabled the less aggregation of ZIF-8 to provide sufficient specific surface area for CR adsorption. From the analysis of the pseudo-second-order kinetic model and Langmuir model, the adsorption of ZIF-8 @BC on CR was a homogeneously chemical adsorption process regulated by electrostatic interaction, pi-pi stacking and metal coordination.
Keyword ：
Congo red Congo red Spent coffee grounds Spent coffee grounds Adsorption Adsorption Metal-organic framework Metal-organic framework
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| GB/T 7714 | Liang, Yixuan , Li, Hanbing , Li, Xiaotong et al. Using recycled coffee grounds for the synthesis of ZIF-8@BC to remove Congo red in water [J]. | ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY , 2022 , 236 . |
| MLA | Liang, Yixuan et al. "Using recycled coffee grounds for the synthesis of ZIF-8@BC to remove Congo red in water" . | ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY 236 (2022) . |
| APA | Liang, Yixuan , Li, Hanbing , Li, Xiaotong , Zhang, Qiyu , Fei, Jiaying , Li, Sumei et al. Using recycled coffee grounds for the synthesis of ZIF-8@BC to remove Congo red in water . | ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY , 2022 , 236 . |
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Abstract ：
Cities play critical roles in achieving carbon-neutrality, and the pathways to the carbon-neutral goal are different because of cities' various developmental levels. On the basis of the industrial structure and energy intensity, "2 thorn 26" cities were classified firstly. With LEAP-city model built, the gaps and pathways to carbon neutrality for different city types (SCJ, CCL, CCX, and ICZ) are analyzed under the policy (PO) and low-carbon (LC) scenarios. Results show that CCL and CCX would be carbon-neutral without carbon capture and storage (CCS) technology in the LC scenario. If SCJ and ICZ apply the CCS for the power and heating plants, they can be carbon neutral in 2049 and 2050, respectively. Regarding CO2 emissions, the industry sector in all energy demand sectors is always the most key sector for CCX and ICZ from 2016 to 2030, which means optimizing production processes and reducing surplus output are very important. After high energy-consuming industries are moved out CCL and SCJ, CO2 emissions from transportation and buildings are the challenges. Therefore, instead of fuel vehicles, zero-carbon vehicles are the first option. Electrification and zero-carbon energy used in buildings are the priorities combined with the decarbonization of electricity, which would also be a highly efficient measure in the industry sector after 2030.
Keyword ：
CO 2 emissions CO 2 emissions Scenario analysis Scenario analysis LEAP-city model LEAP-city model Carbon neutrality Carbon neutrality
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| GB/T 7714 | Liu, Yingying , Chen, Sha , Jiang, Kejun et al. The gaps and pathways to carbon neutrality for different type cities in China [J]. | ENERGY , 2022 , 244 . |
| MLA | Liu, Yingying et al. "The gaps and pathways to carbon neutrality for different type cities in China" . | ENERGY 244 (2022) . |
| APA | Liu, Yingying , Chen, Sha , Jiang, Kejun , Kaghembega, Wendkuuni Steve-Harold . The gaps and pathways to carbon neutrality for different type cities in China . | ENERGY , 2022 , 244 . |
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Abstract ：
The evaluation of the efficiency and feasibility of energy transition and air pollution control at the city level is one of the key points in addressing environmental problems and achieving the goals of CO2 emission reduction and carbon neutrality in China. In this study, an integrated method is developed on the basis of the Low Emissions Analysis Platform (LEAP) and life cycle assessment (LCA). The energy demands and environmental co-benefits in Jinan, one of the low-carbon city pilots in China, are quantitatively evaluated under three policy scenarios: low-carbon (LC) policy scenario, pollution control (PC) policy scenario, and deep-level cut of CO2 emissions (DCC) scenario from 2016 to 2050. From 2016 to 2030, the PC policies would be more powerful than the LC policies in terms of energy demand decrease. From 2030 to 2050, the LC policies would be more efficient than all the other policies. Promoting energy-saving buildings in the LC scenario would contribute to the continual decline in energy demands. In the DCC scenario, CO2, PM2.5, PM10, CO, NOX and SO2 emissions would decline by more than 71.4% relative to the records in 2016. Global warming potential, human toxicity potential, photochemical ozone creation potential, particulate matter formation potential, and acidification potential would also decrease by 81.8%-88.5%. On the basis of the integrated city-level LEAP and LCA method, this study quantifies the various environmental impacts of urban decarbonization policies and provides science-based references for urban low-carbon transformation.
Keyword ：
Coordinated emission reduction Coordinated emission reduction Jinan Jinan LEAP-LCA LEAP-LCA Environmental co-benefits Environmental co-benefits
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| GB/T 7714 | Chen Sha , Liu Ying-Ying , Lin Jin et al. Coordinated reduction of CO2 emissions and environmental impacts with integrated city-level LEAP and LCA method: A case study of Jinan, China [J]. | ADVANCES IN CLIMATE CHANGE RESEARCH , 2021 , 12 (6) : 848-857 . |
| MLA | Chen Sha et al. "Coordinated reduction of CO2 emissions and environmental impacts with integrated city-level LEAP and LCA method: A case study of Jinan, China" . | ADVANCES IN CLIMATE CHANGE RESEARCH 12 . 6 (2021) : 848-857 . |
| APA | Chen Sha , Liu Ying-Ying , Lin Jin , Shi Xiao-Dan , Jiang Ke-Jun , Zhao Guang-Lin . Coordinated reduction of CO2 emissions and environmental impacts with integrated city-level LEAP and LCA method: A case study of Jinan, China . | ADVANCES IN CLIMATE CHANGE RESEARCH , 2021 , 12 (6) , 848-857 . |
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Abstract ：
欧盟在2019年提出2050年碳中和目标,这一目标不只是一个长期目标,很多行业已经开始制定短期的具体行动方案和对策,并启动了实际行动。2020年9月中国在联大会议上宣布,力争在2060年前实现碳中和。碳中和目标会明显影响未来一些产业的生产工艺。对于工业中难以减排的行业,如钢铁、水泥、合成氨、乙烯、苯、甲醇等,为实现深度减排,氢基产业将是一个重要选项。绿氢的供应将会明显影响这些产业采用氢工艺的成本,进而影响产业的区域布局。通过本研究可以看出,未来中国主要基础产业的布局将出现明显变化,在考虑多种实现产业深度减排技术选择(如碳捕集与封存)的情况下,不少产业都将转向可再生能源富集和低成本地区,特别是光...
Keyword ：
巴黎协定目标 巴黎协定目标 电力 电力 经济布局 经济布局 碳中和 碳中和 中国 中国
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| GB/T 7714 | 姜克隽 , 向翩翩 , 贺晨旻 et al. 零碳电力对中国工业部门布局影响分析 [J]. | 全球能源互联网 , 2021 , 4 (01) : 5-11 . |
| MLA | 姜克隽 et al. "零碳电力对中国工业部门布局影响分析" . | 全球能源互联网 4 . 01 (2021) : 5-11 . |
| APA | 姜克隽 , 向翩翩 , 贺晨旻 , 冯升波 , 刘昌义 , 谭新 et al. 零碳电力对中国工业部门布局影响分析 . | 全球能源互联网 , 2021 , 4 (01) , 5-11 . |
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