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学者姓名：王湛
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Abstract ：
在本研究中,将不同孔径的超滤膜用于过滤活性污泥悬浮液,以探究不同孔径膜的超滤膜过滤性能.结果表明:渗透滤液的累积体积随孔径的增大而减小.过滤初期,膜的渗透通量随着孔径的增大而增大.过滤后期,膜的渗透通量随着孔径的增大而减小.膜孔径越大,有效膜面积下降得越快,达到稳定有效膜面积的时间越短.同时,通过计算孔堵塞阻力和膜的有效膜面积可以很好地评估超滤膜过滤性能,孔径小的膜孔内阻力占比小、受污染程度低和抗污性能好.
Keyword ：
膜孔径 膜孔径 污染机理 污染机理 膜污染 膜污染
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| GB/T 7714 | 刘鑫森 , 王湛 . 膜孔径大小对超滤膜过滤性能影响的研究 [J]. | 当代化工研究 , 2023 , (15) : 23-25 . |
| MLA | 刘鑫森 等. "膜孔径大小对超滤膜过滤性能影响的研究" . | 当代化工研究 15 (2023) : 23-25 . |
| APA | 刘鑫森 , 王湛 . 膜孔径大小对超滤膜过滤性能影响的研究 . | 当代化工研究 , 2023 , (15) , 23-25 . |
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Abstract ：
<正>北京工业大学王湛教授编写的‘Modelling of the Microfiltration Process’一书，在Springer出版社出版．购书链接：https：//www.amazon.com/Modelling-Microfiltration-Process-Zhan-Wang/dp/9819904706/ref=sr＿1＿1?crid=16A38H0VFX4Z0&keywords=Modelling+of+the+microfiltration+process&qid=1674185669&sprefix=%2Caps%2C1899&sr=8-1内容简介在城市污水资源化、工业废水回用、海水和苦咸水淡化过程中，膜技术及其应用发挥着重要作用．
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| GB/T 7714 | 王湛 . 好书推荐 [J]. | 膜科学与技术 , 2023 , 43 (03) : 53 . |
| MLA | 王湛 . "好书推荐" . | 膜科学与技术 43 . 03 (2023) : 53 . |
| APA | 王湛 . 好书推荐 . | 膜科学与技术 , 2023 , 43 (03) , 53 . |
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Abstract ：
This study describes the preparation of graphitic carbon nitride (g-C3N4), hematite (alpha-Fe2O3), and their g-C3N4/alpha-Fe2O3 heterostructure for the photocatalytic removal of methyl orange (MO) under visible light illumination. The facile hydrothermal approach was utilized for the preparation of the nanomaterials. Powder X-ray diffraction (XRD), Scanning electron microscopy (SEM), Energy dispersive X-ray (EDX), and Brunauer-Emmett-Teller (BET) were carried out to study the physiochemical and optoelectronic properties of all the synthesized photocatalysts. Based on the X-ray photoelectron spectroscopy (XPS) and UV-visible diffuse reflectance (DRS) results, an energy level diagram vs. SHE was established. The acquired results indicated that the nanocomposite exhibited a type-II heterojunction and degraded the MO dye by 97%. The degradation ability of the nanocomposite was higher than that of pristine g-C3N4 (41%) and alpha-Fe2O3 (30%) photocatalysts under 300 min of light irradiation. The formation of a type-II heterostructure with desirable band alignment and band edge positions for efficient interfacial charge carrier separation along with a larger specific surface area was collectively responsible for the higher photocatalytic efficiency of the g-C3N4/alpha-Fe2O3 nanocomposite. The mechanism of the nanocomposite was also studied through results obtained from UV-vis and XPS analyses. A reactive species trapping experiment confirmed the involvement of the superoxide radical anion (O-2(& BULL;-)) as the key reactive oxygen species for MO removal. The degradation kinetics were also monitored, and the reaction was observed to be pseudo-first order. Moreover, the sustainability of the photocatalyst was also investigated.
Keyword ：
alignment of energy levels alignment of energy levels g-C3N4/alpha-Fe2O3 nanocomposite g-C3N4/alpha-Fe2O3 nanocomposite MO photodegradation MO photodegradation g-C3N4 g-C3N4 heterostructure (type-II) heterostructure (type-II)
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| GB/T 7714 | Khurram, Rooha , Nisa, Zaib Un , Javed, Aroosa et al. Synthesis and Characterization of an alpha-Fe2O3-Decorated g-C3N4 Heterostructure for the Photocatalytic Removal of MO [J]. | MOLECULES , 2022 , 27 (4) . |
| MLA | Khurram, Rooha et al. "Synthesis and Characterization of an alpha-Fe2O3-Decorated g-C3N4 Heterostructure for the Photocatalytic Removal of MO" . | MOLECULES 27 . 4 (2022) . |
| APA | Khurram, Rooha , Nisa, Zaib Un , Javed, Aroosa , Wang, Zhan , Hussien, Mostafa A. . Synthesis and Characterization of an alpha-Fe2O3-Decorated g-C3N4 Heterostructure for the Photocatalytic Removal of MO . | MOLECULES , 2022 , 27 (4) . |
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Abstract ：
Recently, rising distress over ecological pollution owing to water contamination by coloring effluents primarily due to dyes is of growing concern. The development of semiconductor/magnetic oxide-based nanomaterials has verified to be a potent remediation means for water pollution. In the present article, the fabrication of nanocomposites was carried out by the facile hydrothermal method. The ZnO and ZnSe nanoparticles were in situ formed on the α-Fe2O3 layer, thereby forming a heterojunction. The prepared α-Fe2O3/ZnSe nanocomposite possessed a degradation of 98.9% for a Congo red aqueous solution of 100 ppm. The α-Fe2O3/ZnO nanocomposite showed only 26% degradation of 100 ppm dye solution depicting a poor photocatalytic performance. This is attributed to the formation of recombination-enhanced configuration (type-I heterostructure) in the α-Fe2O3/ZnO nanocomposite (NC). In contrast, α-Fe2O3/ZnSe NC accomplished a higher and enhanced photocatalytic response. The key rationale for elevated photocatalytic response is the establishment of a recombination-free configuration (type-II heterostructure). Thus, α-Fe2O3/ZnSe NC known as one of outstanding nanoparticle-nanocomposite photocatalysts was synthesized under mild conditions exclusive of some multifaceted post-treatment, for dye abatement process.
Keyword ：
ZnSe ZnSe α-Fe2O3 α-Fe2O3 Mechanism Mechanism ZnO ZnO Hydrothermal process Hydrothermal process Textile wastewater treatment Textile wastewater treatment Alignment of energy levels Alignment of energy levels Photocatalysis Photocatalysis
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| GB/T 7714 | Khurram Rooha , Wang Zhan , Ehsan Muhammad Fahad . α-Fe2O3-based nanocomposites: synthesis, characterization, and photocatalytic response towards wastewater treatment. [J]. | Environmental science and pollution research international , 2021 , 28 (14) : 17697-17711 . |
| MLA | Khurram Rooha et al. "α-Fe2O3-based nanocomposites: synthesis, characterization, and photocatalytic response towards wastewater treatment." . | Environmental science and pollution research international 28 . 14 (2021) : 17697-17711 . |
| APA | Khurram Rooha , Wang Zhan , Ehsan Muhammad Fahad . α-Fe2O3-based nanocomposites: synthesis, characterization, and photocatalytic response towards wastewater treatment. . | Environmental science and pollution research international , 2021 , 28 (14) , 17697-17711 . |
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Abstract ：
Photocatalysis and membrane technology in a single unit is an ideal strategy for the development of wastewater treatment systems. In this work, novel GO (x wt%)/TiO2-CA hybrid membranes have been synthesized via a facile non-solvent induced phase inversion technique. The strategy aimed to address the following dilemmas: (1) Effective utilization of visible light and minimize e(-)/h(+) recombination; (2) Enhanced separation capability and superior anti-fouling and self-cleaning ability. The experimental results reveal that the integration of nano-composite (GO/TiO2) boosts the membrane properties when compared to pristine CA and single photocatalyst employed membrane (GO-CA and TiO2-CA). The effect of GO content on the properties of the photocatalytic membrane has been determined by utilizing three different ratios of GO, viz. 0.5 wt%, 1 wt%, and 2 wt% designated as NC(1)-CA, NC(2)-CA, and NC(3)-CA, respectively. Amongst them, NC(3)-CA membrane showed state-of-the-art performance with an elevated photocatalytic response (four times higher than pristine CA membrane) toward methyl orange. Moreover, the water flux of NC(3)-CA membrane is 613 L/m(2)h, approximately three times higher than bare CA membrane (297 L/m(2)h), while keeping the MO rejection high (96.6%). Besides, fouling experiments presented the lowest total and fouling resistance ratios and a higher flux recovery ratio (91.78%) for the NC(3)-CA membrane, which endows the membrane with higher anti-fouling and self-cleaning properties. Thus, NC(3)-CA membrane outperforms the other as synthesized membranes in terms of separation efficiency, visible light photo-degradation of pollutant, anti-fouling and self-cleaning ability. Therefore, NC(3)-CA membrane is considered as the next generation membrane for exhibiting great potential for the wastewater treatment applications.
Keyword ：
environmental science environmental science Titania (TiO2) Titania (TiO2) self-cleaning and anti-fouling ability self-cleaning and anti-fouling ability Photocatalytic membranes Photocatalytic membranes clean technology and engineering clean technology and engineering photo-degradation of MO photo-degradation of MO Graphene oxide (GO) Graphene oxide (GO)
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| GB/T 7714 | Khurram, Rooha , Javed, Aroosa , Ke, Ruihua et al. Visible Light-Driven GO/TiO2-CA Nano-Photocatalytic Membranes: Assessment of Photocatalytic Response, Antifouling Character and Self-Cleaning Ability [J]. | NANOMATERIALS , 2021 , 11 (8) . |
| MLA | Khurram, Rooha et al. "Visible Light-Driven GO/TiO2-CA Nano-Photocatalytic Membranes: Assessment of Photocatalytic Response, Antifouling Character and Self-Cleaning Ability" . | NANOMATERIALS 11 . 8 (2021) . |
| APA | Khurram, Rooha , Javed, Aroosa , Ke, Ruihua , Lena, Cheng , Wang, Zhan . Visible Light-Driven GO/TiO2-CA Nano-Photocatalytic Membranes: Assessment of Photocatalytic Response, Antifouling Character and Self-Cleaning Ability . | NANOMATERIALS , 2021 , 11 (8) . |
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Abstract ：
Homogeneous electrocatalytic reaction has been extensively applied in electrochemical flow sensors especially for the detection of non-electroactive species. Herein, homogeneous electrocatalytic reaction is studied on a rotating disc electrode (RDE) system to mimic the forced convection in flow sensors in both experiments and theory. The experimental RDE voltammogram reveals a pre plateau feature under the rotation frequency of 25 rpm and the corresponding theoretical current–potential curves generated by 2D axisymmetric electrochemical analysis model is in good consistency with the experimental voltammetric responses. Based on the same model, mediator and substrate concentration distributions and the diffusion layer thicknesses are discussed in detail. Moreover, the interference of direct electrochemical oxidation of the substrate is investigated via the homogeneous electrocatalytic reaction between 1,1′-ferrocenedicarboxylic acid and L-cysteine and the corresponding second-order rate constant (372 (mol m−3)−1 s−1) is shown by the modified model. Also, the influence of substrate diffusion coefficients in homogeneous electrocatalytic reaction is analyzed and the obtained transition point indicates the specific critical second-order rate constant for both ferroceneacetic acid (106.02 (mol m−3)−1 s−1) and 1,1′-ferrocenedicarboxylic acid (105.36 (mol m−3)−1 s−1) as the mediator. At last, the design principle of homogeneous electrocatalytic flow sensor is summarized. © 2021 The Author(s)
Keyword ：
Rate constants Rate constants Electrocatalysis Electrocatalysis Mass transfer Mass transfer Rotating disks Rotating disks Electrochemical oxidation Electrochemical oxidation Electrochemical electrodes Electrochemical electrodes Amino acids Amino acids
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| GB/T 7714 | Song, Peng , Yin, Shuang , Wang, Zhan . Insights into the design of homogeneous electrocatalytic flow sensor via a rotating disc electrode system [J]. | Materials and Design , 2021 , 206 . |
| MLA | Song, Peng et al. "Insights into the design of homogeneous electrocatalytic flow sensor via a rotating disc electrode system" . | Materials and Design 206 (2021) . |
| APA | Song, Peng , Yin, Shuang , Wang, Zhan . Insights into the design of homogeneous electrocatalytic flow sensor via a rotating disc electrode system . | Materials and Design , 2021 , 206 . |
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Abstract ：
A new model based on the removal mechanism of loose/compact cake and the re-deposition mechanism of foulants was proposed to predict the instantaneous fouling resistance (Rf(t)) in the rinsing process of 0.1 mu m PAN membrane fouled with activated sludge. The variation trend of Rf(t) was also analyzed by the removal rate of loose/compact cake (rr-ose/rr-compact) and the re-deposition rate of foulants (rre-deposition). Moreover, the model was validated by using other foulants (yeast, actual activated sludge, HA and SA) and membranes (0.1 mu m PES and PVDF membranes). The results showed that the model predictions had good agreements with experimental data at different cross-flow velocities (1.0, 1.5, 2.0 and 2.5 m/s) or temperatures (25, 30, 35 and 40 degrees C) (R2 0.9900). Besides, the variation trend of Rf(t) could be divided into three stages: (i) Rf(t) quickly decreased and the removal of loose cake was almost completed at rinsing time of t1 (first transition point) (rrose = 0); (ii) Rf(t) slowly decreased and Rf(t) reached to minimum (rr-compact = rre-deposition) at t2 (second transition point); (iii) Rf(t) slightly increased after t2 (rr-compact(t)<rre-deposition(t)). This model would provide an accurate method to analyze the variation trend of Rf(t) in the rinsing process and a theoretical basis for the optimization of rinsing conditions.
Keyword ：
Mechanism Mechanism Desorption energy Desorption energy Rinsing model Rinsing model ose ose compact cake compact cake Transition point Transition point
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| GB/T 7714 | Qiao, Zhaoyu , Wang, Zhan , Guo, Yangyang . A new model based on the cake removal and the re-deposition mechanism in the rinsing process [J]. | JOURNAL OF MEMBRANE SCIENCE , 2021 , 636 . |
| MLA | Qiao, Zhaoyu et al. "A new model based on the cake removal and the re-deposition mechanism in the rinsing process" . | JOURNAL OF MEMBRANE SCIENCE 636 (2021) . |
| APA | Qiao, Zhaoyu , Wang, Zhan , Guo, Yangyang . A new model based on the cake removal and the re-deposition mechanism in the rinsing process . | JOURNAL OF MEMBRANE SCIENCE , 2021 , 636 . |
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Abstract ：
Electroactive species modified electrodes are extensively studied as the mediator donor in homogeneous electrocatalytic reaction for electrochemical sensing purpose. In this paper, homogeneous electrocatalytic reaction within a thin layer modified electrode is investigated theoretically and experimentally to illustrate the electroactive species distribution on ferrocenedicarboxylic acid modified carbon black paste electrodes (FDACBPE). The voltammetric analysis of the fabricated FDACBPE reveals that the electrode is in diffusional control at the scan rate lower than 50 mV s-1 while a surface control electrode reaction is observed at a higher scan rate. Based on the experimental results, three finite element models including thin layer model, fixed mediator model and combined model are established to evaluate the homogeneous electrocatalytic reaction with FDACBPE. The numerical results show that the anodic peak gap order of 3 models is as follows: fixed mediator model > combined model > thin layer model. As validation of the proposed model, the comparison between experimental results and numerical data on both polished and unpolished FDACBPE indicates that the combined model data are more suitable for the description of experimental voltammograms compared with the other two models. Also, the comparison between these models suggests that both surface confined and diffusional FDA exist when FDACBPE is employed.
Keyword ：
Electrocatalytic reaction Electrocatalytic reaction Numerical simulation Numerical simulation Surface modified electrode Surface modified electrode Electroactive layer Electroactive layer Ferrocenedicarboxylic acid Ferrocenedicarboxylic acid
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| GB/T 7714 | Song, Peng , Li, Yan , Yin, Shuang et al. Simulation-based evaluation of homogeneous electrocatalytic reaction within a thin layer modified electrode [J]. | JOURNAL OF ELECTROANALYTICAL CHEMISTRY , 2021 , 901 . |
| MLA | Song, Peng et al. "Simulation-based evaluation of homogeneous electrocatalytic reaction within a thin layer modified electrode" . | JOURNAL OF ELECTROANALYTICAL CHEMISTRY 901 (2021) . |
| APA | Song, Peng , Li, Yan , Yin, Shuang , Tang, Yang , Wang, Zhan . Simulation-based evaluation of homogeneous electrocatalytic reaction within a thin layer modified electrode . | JOURNAL OF ELECTROANALYTICAL CHEMISTRY , 2021 , 901 . |
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Abstract ：
Extracellular polymeric substances (EPSs) in activated sludge suspensions are the key substances leading to the membrane fouling. In order to understand the effect of EPSs on the membrane fouling, the actual EPSs solution extracted from activated sludge suspensions was used as the feed solution to conduct dead-end microfiltration experiment under different pressures by using different membranes. The flux (J), fouling resistances (Rm, Rp, Rc and Rtotal) and the available membrane area (A/A0) were used to describe the membrane fouling. The results showed that with the increase of pressure, J and Rtotal increased. Rp firstly increased and then kept constant, Rc always increased and became the dominant resistance. A/A0 decreased from 1 to a constant. Rc plays a key role on Rtotal for different membranes under the same pressure. The sequence of the steady available membrane area (Asteady/A0) for different pressures was: 63.0% (0.05MPa)> 56.5% (0.08MPa)> 53.6% (0.10MPa), and that for different membranes was: 80.1% (0.2μm PES) > 79.9% (0.1μm PES) > 78.4% (0.1μm PAN) > 53.6% (0.1μm PVDF). © Content from this work may be used under the terms of the Creative Commons Attribution 3.0 licence.
Keyword ：
Membranes Membranes Polymers Polymers Microfiltration Microfiltration Energy resources Energy resources Membrane fouling Membrane fouling
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| GB/T 7714 | Li, Qiang , Hu, Ge , Song, Peng et al. Membrane fouling of actual extracellular polymeric substances [C] . 2021 . |
| MLA | Li, Qiang et al. "Membrane fouling of actual extracellular polymeric substances" . (2021) . |
| APA | Li, Qiang , Hu, Ge , Song, Peng , Khaliunaa, Natsagdorj , Khurram, Rooha , Zhang, Hu et al. Membrane fouling of actual extracellular polymeric substances . (2021) . |
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Abstract ：
This study systematically investigated the fouling behavior and mechanism of PAN Microfiltration (MF) membrane fouled with the model binary mixture (bovine serum albumin (BSA) and sodium alginate (SA)) of extracellular polymer substance (EPS) solution under different concentration and transmembrane pressure (TMP). The result showed that the fouling mechanism of the model binary mixture was the pore blocking and cake formation. Moreover, the SA plays a dominant role in the model binary mixture (BSA/SA). The higher SA concentration could cause the more serious membrane fouling (both the flux (J) and the available membrane area (A/A0) decreased), and the total resistance increased and caused the fouling mechanism changing from combined complete blocking and cake filtration into individual cake filtration appeared earlier. In addition, increasing of the TMP can also aggravate membrane fouling and it could be accurately described by the cake-complete model. This studied offered insight into the model binary mixture in the fouling behavior and mechanism, which can be used as guidance for practical application. © Content from this work may be used under the terms of the Creative Commons Attribution 3.0 licence.
Keyword ：
Binary mixtures Binary mixtures Energy resources Energy resources Mammals Mammals Sodium alginate Sodium alginate Membrane fouling Membrane fouling Microfiltration Microfiltration
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| GB/T 7714 | Gao, Shujuan , Liu, Xinsen , Zhang, Hu et al. The study of fouling behavior for the model binary mixture [C] . 2021 . |
| MLA | Gao, Shujuan et al. "The study of fouling behavior for the model binary mixture" . (2021) . |
| APA | Gao, Shujuan , Liu, Xinsen , Zhang, Hu , Liu, Xuguo , Wang, Zhan , Wang, Xi . The study of fouling behavior for the model binary mixture . (2021) . |
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