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学者姓名：程水源
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Abstract ：
A variety of methods based on air quality models, including tracer methods, the brute-force method (BFM), decoupled direct method (DDM), high-order decoupled direct method (HDDM), response surface models (RSMs) and so on forth, have been widely used to study the transport of air pollutants. These methods have good applicability for the transport of air pollutants with simple formation mechanisms. However, differences in research conclusions on secondary pollutants with obvious nonlinear characteristics have been reported. For example, the tracer method is suitable for the study of simplified scenarios, while HDDM and RSMs are more suitable for the study for nonlinear pollutants. Multiple observation techniques, including conventional air pollutant observation, lidar observation, air sounding balloons, vehicle-mounted and ship-borne technology, aerial surveys, and remote sensing observations, have been utilized to investigate air pollutant transport characteristics with time resolution as high as 1 sec. In addition, based on a multi-regional input-output model combined with emission inventories, the transfer of air pollutant emissions can be evaluated and applied to study the air pollutant transport characteristics. Observational technologies have advantages in temporal resolution and accuracy, while modeling technologies are more flexible in spatial resolution and research plan setting. In order to accurately quantify the transport characteristics of pollutants, it is necessary to develop a research method for interactive verification of observation and simulation. Quantitative evaluation of the transport of air pollutants from different angles can provide a scientific basis for regional joint prevention and control. (c) 2022 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
Keyword ：
Transport flux Transport flux Air pollutant transport Air pollutant transport Simulation technology Simulation technology Observation technology Observation technology Transport matrix Transport matrix
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| GB/T 7714 | Wang, Xiaoqi , Cheng, Shuiyuan , Zhou, Ying et al. A review of the technology and applications of methods for evaluating the transport of air pollutants [J]. | JOURNAL OF ENVIRONMENTAL SCIENCES , 2023 , 123 : 341-349 . |
| MLA | Wang, Xiaoqi et al. "A review of the technology and applications of methods for evaluating the transport of air pollutants" . | JOURNAL OF ENVIRONMENTAL SCIENCES 123 (2023) : 341-349 . |
| APA | Wang, Xiaoqi , Cheng, Shuiyuan , Zhou, Ying , Zhang, Hanyu , Guan, Panbo , Zhang, Zhida et al. A review of the technology and applications of methods for evaluating the transport of air pollutants . | JOURNAL OF ENVIRONMENTAL SCIENCES , 2023 , 123 , 341-349 . |
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Abstract ：
利用核壳型的CdSe@CdS量子点作为发光物质，并用壳聚糖（CS）、类石墨烯氮化碳（gC_3N_4）与CdSe@CdS量子点合成了CdSe@CdS/CS/gC_3N_4复合物，将该复合物修饰至玻碳电极（GCE）表面，将适配体（Apt）的互补DNA链（cDNA）通过化学反应连接到量子点上，Apt与cDNA发生杂交反应而被修饰至电极表面。将辣根过氧化物酶（HRP）固定到该修饰电极表面，构建了检测卡那霉素（Kana）的电化学发光（ECL）适配体传感器。通过生物催化沉淀（BCP）方法实现Kana的检测，溶液中无Kana时，在H_2O_2的存在下，修饰在电极上的HRP可以催化氧化4-氯-1-萘酚（4-CN），在电极表面产生不导电的苯并-4-氯己二烯酮沉淀，导致电化学发光信号明显降低。溶液中存在Kana时，Kana会与Apt特异性结合，部分dsDNA解旋，导致部分HRP从电极表面脱落，BCP反应减弱，导致ECL信号增强，实现目标物质的特异性检测。计算适配体传感器在Kana溶液中的ECL强度（I）与传感器在空白溶液中的ECL强度（I_0）的差值ΔI (I-I_0)，并以此作为响应信号。结果显示，ΔI与Kana浓度的对数值在1.0×10~(-8)～1.0×10~(-4) g/L范围呈良好的线性关系，检出限为5 ng/L。该传感器在实际样品测定中具有较好的应用前景。
Keyword ：
电化学发光 电化学发光 卡那霉素 卡那霉素 量子点 量子点 适配体 适配体 生物催化沉淀 生物催化沉淀
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| GB/T 7714 | 高会莲 , 康天放 , 鲁理平 et al. 基于CdSe@CdS/壳聚糖/gC_3N_4复合物的卡那霉素电化学发光适配体传感器 [J]. | 分析试验室 , 2023 , 42 (03) : 305-311 . |
| MLA | 高会莲 et al. "基于CdSe@CdS/壳聚糖/gC_3N_4复合物的卡那霉素电化学发光适配体传感器" . | 分析试验室 42 . 03 (2023) : 305-311 . |
| APA | 高会莲 , 康天放 , 鲁理平 , 程水源 . 基于CdSe@CdS/壳聚糖/gC_3N_4复合物的卡那霉素电化学发光适配体传感器 . | 分析试验室 , 2023 , 42 (03) , 305-311 . |
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Abstract ：
制备了硫化镉量子点-壳聚糖(CdS-CS)复合物修饰的玻碳电极(GCE),记作CdS-CS/GCE.以卡那霉素为模板分子,3-氨基苯硼酸(APBA)为功能单体,采用循环伏安法在CdS-CS/GCE表面电聚合得到了分子印迹聚合物(MIP)膜,所制备的传感器记作MIP/CdS-CS/GCE.卡那霉素可与传感器表面的MIP特异性结合,占据印迹孔穴,阻断共反应剂K2 S2 O8扩散到电极表面的通路,使电化学发光强度减弱.以传感器在空白溶液中的电化学发光强度(I0)与传感器在卡那霉素标准溶液中的电化学发光强度(I)的差值ΔI(ΔI=I0-I)作为响应信号,在优化的试验条件下,响应信号ΔI与卡那霉素浓度的对数值在1.0×10-11～1.0×10-7 mol·L-1内呈线性关系,相关系数为0.9990,检出限(3S/N)为5×10-12 mol·L-1.按标准加入法对实际样品进行回收试验,回收率为99.9％～103％,测定值的相对标准偏差(n=5)为2.5％～4.3％.
Keyword ：
分子印迹聚合物 分子印迹聚合物 传感器 传感器 卡那霉素 卡那霉素 电化学发光法 电化学发光法 CdS-CS复合物 CdS-CS复合物
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| GB/T 7714 | 孙晨阳 , 康天放 , 鲁理平 et al. 分子印迹电化学发光传感器的制备及其对卡那霉素的测定应用 [J]. | 理化检验（化学分册） , 2023 , 59 (3) : 249-256 . |
| MLA | 孙晨阳 et al. "分子印迹电化学发光传感器的制备及其对卡那霉素的测定应用" . | 理化检验（化学分册） 59 . 3 (2023) : 249-256 . |
| APA | 孙晨阳 , 康天放 , 鲁理平 , 程水源 . 分子印迹电化学发光传感器的制备及其对卡那霉素的测定应用 . | 理化检验（化学分册） , 2023 , 59 (3) , 249-256 . |
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Abstract ：
Great changes occurred in the physical and chemical properties of the atmosphere in the North China Plain (NCP) in summer caused by PM2.5 dropping from 58 mu g/m(3) in 2015 to 36.0 mu g/m(3) in 2019. In this study, we first applied the WRF-Chem model to quantify the impact of PM2.5 reduction on shortwave radiation reaching the ground (SWDOWN), planetary boundary layer height (PBLH), and the surface concentration of air pollutants (represented by CO). Simulation results obtained an increase of 15.0% in daytime SWDOWN and 9.9% in daytime PBLH, and a decrease of -5.0% in daytime CO concentration. These changes were induced by the varied PM2.5 levels. Moreover, the variation in SWDOWN further led to a rise in the NO2 photolysis rate (JNO(2)) over this region, by 1.82 x 10(-4)similar to 1.91 x 10(-4) s(-1) per year. Afterwards, we employed MCM chemical box model to explore how the JNO(2) increase and the precursor decrease (CO, VOCs, and NOx) influenced O-3 and HO2 radicals. The results revealed that the photolysis rate U) increase would individually cause a change on daytime surface O-3, OH, and HO2 radicals by +9.0%, +18.9%, and +23.7%; the corresponding change induced by the precursor decrease was -2.5%, +1.9%, and -2.3%. At the same time, the integrated impacts of the change in J and precursors cause an increase of +6.3%, +21.1%, and +20.9% for daytime surface O-3, OH, and HO2. Generally, the atmospheric oxidation capacity significantly enhanced during summer in NCP due to the PM2.5 dropping in recent years. This research can help understand atmosphere changes caused by PM2.5 reduction comprehensively.
Keyword ：
chemical box model chemical box model atmospheric oxidation capacity atmospheric oxidation capacity WRF-Chem WRF-Chem photolysis rates photolysis rates
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| GB/T 7714 | Ou, Shengju , Wei, Wei , Cai, Bin et al. The Independent Impacts of PM2.5 Dropping on the Physical and Chemical Properties of Atmosphere over North China Plain in Summer during 2015-2019 [J]. | SUSTAINABILITY , 2022 , 14 (7) . |
| MLA | Ou, Shengju et al. "The Independent Impacts of PM2.5 Dropping on the Physical and Chemical Properties of Atmosphere over North China Plain in Summer during 2015-2019" . | SUSTAINABILITY 14 . 7 (2022) . |
| APA | Ou, Shengju , Wei, Wei , Cai, Bin , Chen, Saisai , Guan, Panbo , Cheng, Shuiyuan . The Independent Impacts of PM2.5 Dropping on the Physical and Chemical Properties of Atmosphere over North China Plain in Summer during 2015-2019 . | SUSTAINABILITY , 2022 , 14 (7) . |
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Abstract ：
本文合成了La~(3+)掺杂的CdS量子点(CdS:La QDs),以其作为发光材料。将量子点吸附于玻碳电极(GCE)表面。采用卡那霉素(Kana)的适配体(apt)及其互补链(cDNA)制备传感器，使apt与cDNA在电极表面杂交形成双链DNA(dsDNA),然后用氯化血红素(hemin)溶液孵育该修饰电极，使hemin嵌入至dsDNA中，制得Kana电化学发光适配体传感器，记作hemin-dsDNA/CdS:La/GCE。建立了简便、灵敏的检测Kana的电化学发光(ECL)方法，当不存在Kana时，电极表面的hemin作为模拟过氧化物酶会催化溶液中的H_2O_2还原为OH~-,使作为量子点...
Keyword ：
La~(3+)离子 La~(3+)离子 CdS量子点 CdS量子点 适配体传感器 适配体传感器 电化学发光 电化学发光 卡那霉素 卡那霉素
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| GB/T 7714 | 高会莲 , 康天放 , 鲁理平 et al. La~(3+)掺杂CdS 量子点的卡那霉素电化学发光适配体传感器研究 [J]. | 化学研究与应用 , 2022 , 34 (03) : 525-532 . |
| MLA | 高会莲 et al. "La~(3+)掺杂CdS 量子点的卡那霉素电化学发光适配体传感器研究" . | 化学研究与应用 34 . 03 (2022) : 525-532 . |
| APA | 高会莲 , 康天放 , 鲁理平 , 程水源 . La~(3+)掺杂CdS 量子点的卡那霉素电化学发光适配体传感器研究 . | 化学研究与应用 , 2022 , 34 (03) , 525-532 . |
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Abstract ：
Ammonia (NH3) discharged from agricultural activities to the atmosphere plays a crucial role in the formation of secondary inorganic aerosols. This study analyzed the temporal-spatial development of agricultural NH3 emissions from 2000 to 2018 in the Beijing-Tianjin-Hebei (BTH) region and assessed the effects of reducing PM2.5 by removing agricultural NH3 using an air quality model. The results showed that the interannual agricultural NH3 emissions in the BTH region exhibited a stairs trend from 2000 to 2018, with an average of 971.63 Gg. In particular, agricultural NH3 emissions in the BTH region reached a maximum in summer when the temperature was high and were more concentrated in the southern plains compared to the northern areas. Under the reduction scenario (RS), the agricultural NH3 emissions in the BTH region in 2015, 2016, 2017, and 2018 were reduced by 2.95%, 4.10%, 18.75%, and 10.21%, resulting in a reduction of 0.5%, 0.5%, 2.5%, and 1.2% of annual mean PM2.5 concentration, respectively, compared with the baseline scenario (BS). Furthermore, agricultural NH3 emissions contributed 12.6, 12.1, 11.9, and 11.3 mu g m(-3) to PM2.5 concentrations in 2015, 2016, 2017, and 2018 under the zero-emission scenario (ZS), respectively. However, the contribution rates exhibited a slightly increasing trend from 20.5% in 2015 to 24.6% in 2018. These findings could provide a new understanding of agricultural NH3 emission trends and their impacts on PM2.5 concentration based on actual NH3 mitigation ratios in recent years, thereby guiding the formulation of future control strategies.
Keyword ：
PM2.5 PM2.5 Ammonia Ammonia Reduction effects Reduction effects Emission trends Emission trends
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| GB/T 7714 | Cheng, Long , Ye, Zhilan , Cheng, Shuiyuan et al. Agricultural ammonia emissions and its impact on PM2.5 concentrations in the Beijing-Tianjin-Hebei region from 2000 to 2018 [J]. | ENVIRONMENTAL POLLUTION , 2021 , 291 . |
| MLA | Cheng, Long et al. "Agricultural ammonia emissions and its impact on PM2.5 concentrations in the Beijing-Tianjin-Hebei region from 2000 to 2018" . | ENVIRONMENTAL POLLUTION 291 (2021) . |
| APA | Cheng, Long , Ye, Zhilan , Cheng, Shuiyuan , Guo, Xiurui . Agricultural ammonia emissions and its impact on PM2.5 concentrations in the Beijing-Tianjin-Hebei region from 2000 to 2018 . | ENVIRONMENTAL POLLUTION , 2021 , 291 . |
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Abstract ：
A significant technique of combining simulation experiments with a long-term real-time field measurement was first deployed to explore impacts of various environmental factors on formations of sulfate aerosol on the surface of mineral aerosols as MgO in the different reaction systems, and synergistic impacts of these environmental factors on the formation of sulfate aerosols in the different seasonal systems, especially in haze days. Meanwhile, a new correction technique was developed to estimate the effective reaction area and initial uptake coefficient of SO2 on the MgO aerosol surfaces. The significant results showed that the reactions of SO2 on the MgO aerosol surfaces in the system of SO2-MgO-dark could produce a small amount of sulfate and a large amount of sulfite and bisulfite, while in the systems of SO2-MgO-h? and SO2-MgO-O3 produce a large amount of sulfate and a small amount of sulfite and bisulfite. The impacts of temperature T and relative humidity RH on the sulfate formation on MgO aerosol surfaces showed a single-peak mode under the UV light condition, respectively. The sensitivities of these environmental factors to the sulfate aerosol formation were found to follow the order of RH > UV >T > O3 > SO2. The revised initial uptake coefficient ?0.REV of SO2 on the MgO aerosols was always between ?0.BET and ?0.GEO, and much closer to actual value. The heterogeneous reaction mechanisms of SO2 on the MgO aerosol surfaces in the different reaction systems were obviously different. In the presence of water, light irradiation and O3 exerted crucially significant roles in promoting sulfate heterogeneous formation. The various environmental factors in the different seasonal systems, especially in haze days, showed different synergistic effects on sulfate aerosol formations. The sulfate aerosol formations in haze days were mostly impacted by RH, T, O3, and SO2 in spring, RH in summer, RH, T, and SO2 in autumn, and RH and SO2 in winter. The study will provide significant scientific bases for understanding and controlling haze pollution formation.
Keyword ：
Uptake coefficient Uptake coefficient Synergistic effect Synergistic effect Sensitive factors Sensitive factors Mineral aerosol Mineral aerosol Sulfate aerosol Sulfate aerosol Haze days Haze days
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| GB/T 7714 | Han, Lihui , Liu, Xinhang , Chen, Yuanyuan et al. Key factors influencing the formation of sulfate aerosol on the surface of mineral aerosols: Insights from laboratory simulations and ACSM measurements [J]. | ATMOSPHERIC ENVIRONMENT , 2021 , 253 . |
| MLA | Han, Lihui et al. "Key factors influencing the formation of sulfate aerosol on the surface of mineral aerosols: Insights from laboratory simulations and ACSM measurements" . | ATMOSPHERIC ENVIRONMENT 253 (2021) . |
| APA | Han, Lihui , Liu, Xinhang , Chen, Yuanyuan , Xiang, Xin , Cheng, Shuiyuan , Wang, Haiyan . Key factors influencing the formation of sulfate aerosol on the surface of mineral aerosols: Insights from laboratory simulations and ACSM measurements . | ATMOSPHERIC ENVIRONMENT , 2021 , 253 . |
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Abstract ：
武安市是以钢铁立市的典型重工业城市.为研究武安市PM2.5的污染特征和区域来源解析,对武安非采暖期(2018年10月)和采暖期(2019年1月)进行大气PM2.5样品的采集和组分测试,并利用CAMx-PSAT模型模拟结果分析区域源排放对武安PM2.5及其二次水溶性无机离子(SO2-4、NO3-、NH4+)的质量浓度贡献.测试结果表明,武安PM2.5污染严重,平均质量浓度为113.5μg/m3,采暖期PM2.5污染水平高于非采暖期;SO2-4、NO3-和NH4+的平均质量浓度占PM2.5总质量浓度的41.1％,是PM2.5重要组成部分;SO2-4、NO3-和NH4+质量浓度表现为采暖期高于非采暖期;NO3-与SO2-4质量浓度比值在采暖期和非采暖期均小于1,表明燃煤烟尘等固定源贡献相对较大;随着PM2.5污染等级的升高,SO2-4、NO3-和NH4+质量浓度明显增大,达到重污染天时,SO2-4、NO3-和NH4+质量浓度增至最高.模拟结果显示,武安城区PM2.5污染是由本地污染源排放和外来污染物区域传输共同作用的结果,本地污染源排放占主导地位;冶金源排放对PM2.5、NO3-和SO2-4质量浓度贡献影响最大;农业源排放是NH4+质量浓度的主要污染来源;采暖期的居民源排放对PM2.5和SO2-4、NO3-、NH4+质量浓度贡献率相比于非采暖期出现大幅度增加.外来工业源和机动车源对武安PM2.5质量浓度贡献较为突出.
Keyword ：
二次水溶性无机离子 二次水溶性无机离子 武安市 武安市 PM2.5 PM2.5 重工业城市 重工业城市 CAMx-PSAT模型 CAMx-PSAT模型 区域来源解析 区域来源解析
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| GB/T 7714 | 姚诗音 , 韩力慧 , 郭改仲 et al. 武安市PM2.5及其二次水溶性无机离子污染特征和区域来源解析 [J]. | 北京工业大学学报 , 2021 , 47 (6) : 644-654 . |
| MLA | 姚诗音 et al. "武安市PM2.5及其二次水溶性无机离子污染特征和区域来源解析" . | 北京工业大学学报 47 . 6 (2021) : 644-654 . |
| APA | 姚诗音 , 韩力慧 , 郭改仲 , 程水源 , 王传达 . 武安市PM2.5及其二次水溶性无机离子污染特征和区域来源解析 . | 北京工业大学学报 , 2021 , 47 (6) , 644-654 . |
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Abstract ：
In this paper, a regional emissions inventory of anthropogenic VOCs was established based on the traditional emissions factor method for the Beijing-Tianjin-Hebei (BTH) region, followed by a multidimensional calibration study based on regional satellite remote sensing information for formaldehyde and typical urban ground VOCs. Inventory calculations showed that the VOCs emissions in BTH in 2013, 2015, and 2017 were 2026700, 2073400, and 1934200 tons, respectively, comprising alkanes (29.83% to 30.72%), unsaturated hydrocarbons (16.54% to 17.68%), aromatic hydrocarbons (27.14% to 27.51%), aldehydes (8.75% to 9.52%), ketones (8.13% to 9.04%), and aldehydes and ketones lipids (5.13% to 6.60%). During 2013-2017, the emission of VOCs in Zhangjiakou, Qinhuangdao, and Hengshui increased slightly (1.10% to 1.66% per year); emissions in Xingtai and Handan decreased slightly (-1.46% to -1.12% per year); and emissions in Chengde, Tangshan, Baoding, and Cangzhou were stable. There trends were consistent with the inter-annual trend of satellite-derived HCHO column concentrations. However, in Beijing, Tianjin, Langfang, and Shijiazhuang, annual variations in VOCs emissions (-6.51%, -3.30%, 2.16%, and 0.11% per year) and HCHO column concentrations (-1.17%, 7.19%, -0.24%, and 6.68% per year) were observed, respectively. In the regional VOCs inventory, a good linear correlation (R>0.5) was achieved between the grid emissions of VOCs and HCHO column concentrations in urban areas, while the correlation was only 0.33 in suburban areas. This is mainly due to the important influence of secondary conversion of VOCs originating from natural sources to HCHO in suburban areas. In addition, ground-level VOCs concentrations were observed in the urban areas of Beijing and Handan, where the emission ratios (ERs) of VOCs and CO were regressed. The ERs of most hydrocarbons were in good agreement with the regressed ERs, but the ERs of ethane were significantly lower (-156% to -73%) and the ERs of aromatic hydrocarbons above C8 were relatively high (54% to 74%). In general, the regional anthropogenic VOCs emissions inventory established in this paper offers high accuracy and reliability.
Keyword ：
volatile organic compounds(VOCs) volatile organic compounds(VOCs) emission inventory verification emission inventory verification satellite remote sensing satellite remote sensing ground observation ground observation species inventory species inventory
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| GB/T 7714 | Wang Yue , Wei Wei , Ren Yun-Ting et al. [Multidimensional Verification of Anthropogenic VOCs Emissions Inventory Through Satellite Retrievals and Ground Observations]. [J]. | Huanjing kexue , 2021 , 42 (6) : 2713-2720 . |
| MLA | Wang Yue et al. "[Multidimensional Verification of Anthropogenic VOCs Emissions Inventory Through Satellite Retrievals and Ground Observations]." . | Huanjing kexue 42 . 6 (2021) : 2713-2720 . |
| APA | Wang Yue , Wei Wei , Ren Yun-Ting , Wang Xiao-Qi , Chen Sai-Sai , Cheng Shui-Yuan . [Multidimensional Verification of Anthropogenic VOCs Emissions Inventory Through Satellite Retrievals and Ground Observations]. . | Huanjing kexue , 2021 , 42 (6) , 2713-2720 . |
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Abstract ：
Ozone pollution in Handan has become severe in recent years and in the summer of 2018, the average maximum daily 8-hour average ozone concentration in Handan was 175 μg·m-3 with a maximum of 257 μg·m-3. Ozone concentrations exceeded the National Air Quality Grade Ⅱ Standard in 59% of cases. In this study, the H2O2/HNO3 indicator was applied to analyze summertime ozone sensitivity in Handan using the WRF-CMAQ modeling system. The results showed that H2O2/HNO3 was more appropriate than other ozone indicators, both theoretically and based on simulation outputs. The good simulation effect of CMAQ on H2O2 and HNO3 was attributed to fine emission inventory and grid resolution. The H2O2/HNO3 simulation results showed that the relative importance of a VOCs-limited regime decreased month by month; a VOCs-NO x -mixed-limited regime was dominant in June; and a NO x -limited regime was more dominant in July and August than in June. The remarkable spatial difference in VOCs and NO x emission ratios among the counties of Handan led to differences in ozone sensitivity. The VOCs-limited regime was concentrated in counties where VOCs/NO x emission ratios were lower than 1.7. Southern counties had a NO x -limited regime, where VOCs/NO x emission ratios were higher than 6.9. Counties with VOCs/NO x emission ratios varying from 1.7 to 6.9 were more susceptible to both VOCs and NO x . According to these results, the transition range of HCHO/NO2, O3/HNO3, and O3/NO x ratios were adjusted to 0.35-0.6, 20-35, and 10-25 respectively. Adjusting the transition range of H2O2/(O3+NO2) was not effective, indicating that this indicator may not be applicable to Handan.
Keyword ：
WRF-CMAQ WRF-CMAQ photochemical indicator photochemical indicator sensitivity sensitivity ozone ozone Handan City Handan City
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| GB/T 7714 | Niu Yuan , Cheng Shui-Yuan , Ou Sheng-Ju et al. [Applying Photochemical Indicators to Analyze Ozone Sensitivity in Handan]. [J]. | Huanjing kexue , 2021 , 42 (6) : 2691-2698 . |
| MLA | Niu Yuan et al. "[Applying Photochemical Indicators to Analyze Ozone Sensitivity in Handan]." . | Huanjing kexue 42 . 6 (2021) : 2691-2698 . |
| APA | Niu Yuan , Cheng Shui-Yuan , Ou Sheng-Ju , Yao Shi-Yin , Shen Ze-Ya , Guan Pan-Bo . [Applying Photochemical Indicators to Analyze Ozone Sensitivity in Handan]. . | Huanjing kexue , 2021 , 42 (6) , 2691-2698 . |
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