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Author:

Wu, Zhixing (Wu, Zhixing.) | Deng, Jiguang (Deng, Jiguang.) | Liu, Yuxi (Liu, Yuxi.) | Xie, Shaohua (Xie, Shaohua.) | Jiang, Yang (Jiang, Yang.) | Zhao, Xingtian (Zhao, Xingtian.) | Yang, Jun (Yang, Jun.) | Arandiyan, Hamidreza (Arandiyan, Hamidreza.) | Guo, Guangsheng (Guo, Guangsheng.) | Dai, Hongxing (Dai, Hongxing.) (Scholars:戴洪兴)

Indexed by:

EI Scopus SCIE

Abstract:

Three-dimensionally ordered mesoporous Co3O4 (meso-Co3O4) and its supported Au, Pd, and Au-Pd alloy (xAu(y)Pd/meso-Co3O4; x = 0.43-2.94 wt%; Au/Pd molar ratio (y) = 0.43-0.50) nanocatalysts were prepared using the KIT-6-templating and polyvinyl alcohol-protected reduction methods, respectively. It is found that the meso-Co3O4 with a high surface area of 106 m(2)/g was cubic in crystal structure and the noble metal nanoparticles (NPs) with a size of 2.7-4.5 nm were uniformly dispersed on the surface of meso-Co3O4. The 2.94Au(0.50)Pd/meso-Co3O4 sample performed the best for methane combustion, showing the T-10%, T-50%, and T-90% (temperatures required for achieving methane conversions of 10%, 50%, and 90%) of 230, 280, and 324 degrees C at a space velocity of 20,000 mL/(g h) and the lowest apparent activation energy of 44.4 kJ/mol. Furthermore, the effects of CO2, SO2, and H2O addition on the catalytic stability of 2.94Au(0.50)Pd/meso-Co3O4 were also examined. It is concluded that the excellent catalytic performance of 2.94Au(0.50)Pd/meso-Co3O4 was associated with its porous structure, high adsorbed oxygen species concentration, good low-temperature reducibility, and strong interaction between Au-Pd alloy NPs and meso-Co3O4. (C) 2015 Elsevier Inc. All rights reserved.

Keyword:

Noble metal alloy Mesoporous cobalt oxide Methane combustion Strong metal-support interaction Supported catalyst

Author Community:

  • [ 1 ] [Wu, Zhixing]Beijing Univ Technol, Coll Environm & Energy Engn, Key Lab Adv Funct Mat,Educ Minist China, Key Lab Beijing Reg Air Pollut Control,Beijing Ke, Beijing 100124, Peoples R China
  • [ 2 ] [Deng, Jiguang]Beijing Univ Technol, Coll Environm & Energy Engn, Key Lab Adv Funct Mat,Educ Minist China, Key Lab Beijing Reg Air Pollut Control,Beijing Ke, Beijing 100124, Peoples R China
  • [ 3 ] [Liu, Yuxi]Beijing Univ Technol, Coll Environm & Energy Engn, Key Lab Adv Funct Mat,Educ Minist China, Key Lab Beijing Reg Air Pollut Control,Beijing Ke, Beijing 100124, Peoples R China
  • [ 4 ] [Xie, Shaohua]Beijing Univ Technol, Coll Environm & Energy Engn, Key Lab Adv Funct Mat,Educ Minist China, Key Lab Beijing Reg Air Pollut Control,Beijing Ke, Beijing 100124, Peoples R China
  • [ 5 ] [Jiang, Yang]Beijing Univ Technol, Coll Environm & Energy Engn, Key Lab Adv Funct Mat,Educ Minist China, Key Lab Beijing Reg Air Pollut Control,Beijing Ke, Beijing 100124, Peoples R China
  • [ 6 ] [Zhao, Xingtian]Beijing Univ Technol, Coll Environm & Energy Engn, Key Lab Adv Funct Mat,Educ Minist China, Key Lab Beijing Reg Air Pollut Control,Beijing Ke, Beijing 100124, Peoples R China
  • [ 7 ] [Yang, Jun]Beijing Univ Technol, Coll Environm & Energy Engn, Key Lab Adv Funct Mat,Educ Minist China, Key Lab Beijing Reg Air Pollut Control,Beijing Ke, Beijing 100124, Peoples R China
  • [ 8 ] [Guo, Guangsheng]Beijing Univ Technol, Coll Environm & Energy Engn, Key Lab Adv Funct Mat,Educ Minist China, Key Lab Beijing Reg Air Pollut Control,Beijing Ke, Beijing 100124, Peoples R China
  • [ 9 ] [Dai, Hongxing]Beijing Univ Technol, Coll Environm & Energy Engn, Key Lab Adv Funct Mat,Educ Minist China, Key Lab Beijing Reg Air Pollut Control,Beijing Ke, Beijing 100124, Peoples R China
  • [ 10 ] [Wu, Zhixing]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Chem & Chem Engn, Lab Catalysis Chem & Nanosci, Beijing 100124, Peoples R China
  • [ 11 ] [Deng, Jiguang]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Chem & Chem Engn, Lab Catalysis Chem & Nanosci, Beijing 100124, Peoples R China
  • [ 12 ] [Liu, Yuxi]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Chem & Chem Engn, Lab Catalysis Chem & Nanosci, Beijing 100124, Peoples R China
  • [ 13 ] [Xie, Shaohua]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Chem & Chem Engn, Lab Catalysis Chem & Nanosci, Beijing 100124, Peoples R China
  • [ 14 ] [Jiang, Yang]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Chem & Chem Engn, Lab Catalysis Chem & Nanosci, Beijing 100124, Peoples R China
  • [ 15 ] [Zhao, Xingtian]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Chem & Chem Engn, Lab Catalysis Chem & Nanosci, Beijing 100124, Peoples R China
  • [ 16 ] [Yang, Jun]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Chem & Chem Engn, Lab Catalysis Chem & Nanosci, Beijing 100124, Peoples R China
  • [ 17 ] [Guo, Guangsheng]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Chem & Chem Engn, Lab Catalysis Chem & Nanosci, Beijing 100124, Peoples R China
  • [ 18 ] [Dai, Hongxing]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Chem & Chem Engn, Lab Catalysis Chem & Nanosci, Beijing 100124, Peoples R China
  • [ 19 ] [Arandiyan, Hamidreza]Univ New S Wales, Sch Chem Engn, Particles & Catalysis Res Grp, Sydney, NSW 2052, Australia

Reprint Author's Address:

  • 邓积光

    [Deng, Jiguang]Beijing Univ Technol, Coll Environm & Energy Engn, Key Lab Adv Funct Mat,Educ Minist China, Key Lab Beijing Reg Air Pollut Control,Beijing Ke, Beijing 100124, Peoples R China

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Source :

JOURNAL OF CATALYSIS

ISSN: 0021-9517

Year: 2015

Volume: 332

Page: 13-24

7 . 3 0 0

JCR@2022

ESI Discipline: CHEMISTRY;

ESI HC Threshold:253

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 135

SCOPUS Cited Count: 141

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 11

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