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Author:

Liang, Wen-Jun (Liang, Wen-Jun.) (Scholars:梁文俊) | Fang, Hong-Ping (Fang, Hong-Ping.) | Li, Jian (Li, Jian.) | Zheng, Feng (Zheng, Feng.) | Li, Jing-Xin (Li, Jing-Xin.) | Jin, Yu-Quan (Jin, Yu-Quan.)

Indexed by:

EI Scopus SCIE

Abstract:

Destruction of hydrogen sulfide using dielectric barrier discharge plasma in a coaxial cylindrical reactor was carried out at atmospheric pressure and room temperature. Three types of DBD reactor were compared in terms of specific energy density (SED), equivalent capacitances of the gap (Cg) and the dielectric barrier (Cd), energy yield (EY), and H2S decomposition. In addition, byproducts during the decomposition of H2S and destruction mechanism were also investigated. SED for all the reactors depended almost linearly on the voltage. In general, Cg decreased with increasing voltage and with the existence of pellet material, while Cd displayed the opposite trend. The removal efficiency of H2S increased substantially with increasing AC frequency and applied voltage. Longer gas residence times also contributed to higher H2S removal efficiency. The choice of pellet material was an important factor influencing the H2S removal. The reactor filled with ceramic Raschig rings had the best H2S removal performance, with an EY of 7.30 g/kWh. The likely main products in the outlet effluent were H2O, SO2, and SO3. (C) 2011 Elsevier B.V. All rights reserved.

Keyword:

Lissajous diagram Dielectric barrier discharge Hydrogen sulfide Specific energy density Non-thermal plasma

Author Community:

  • [ 1 ] [Liang, Wen-Jun]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 2 ] [Fang, Hong-Ping]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 3 ] [Li, Jian]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 4 ] [Zheng, Feng]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 5 ] [Li, Jing-Xin]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 6 ] [Jin, Yu-Quan]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China

Reprint Author's Address:

  • 梁文俊

    [Liang, Wen-Jun]Beijing Univ Technol, Coll Environm & Energy Engn, 100 Ping Le Yuan, Beijing 100124, Peoples R China

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Source :

JOURNAL OF ELECTROSTATICS

ISSN: 0304-3886

Year: 2011

Issue: 3

Volume: 69

Page: 206-213

1 . 8 0 0

JCR@2022

ESI Discipline: ENGINEERING;

JCR Journal Grade:2

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count: 55

SCOPUS Cited Count: 61

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 10

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