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Author:

Hu, Jingyun (Hu, Jingyun.) | Xue, Haibin (Xue, Haibin.) | Zhang, Xinping (Zhang, Xinping.) (Scholars:张新平)

Indexed by:

Scopus SCIE

Abstract:

We report fabrication of large-scale homogeneous crystallization of CH3NH3PbBr3 (MAPbBr(3)) in the patterned substrate by a two-dimensional (2D) grating. This achieves high-quality optotelectronic structures on local sites in the micron scales and a homogeneous thin-film device in a centimeter scale, proposing a convenient technique to overcome the challenge for producing large-area thin-film devices with high quality by spin-coating. Through matching the concentration of the MAPbBr(3)/DMF solutions with the periods of the patterning structures, we found an optimized size of the patterning channels for a specified solution concentration (e.g., channel width of 5 mu m for a concentration of 0.14 mg/mL). Such a design is also an excellent scheme for random lasing, since the crystalline periodic networks of MAPbBr(3) grids are multi-crystalline constructions, and supply strong light-scattering interfaces. Using the random lasing performance, we can also justify the crystallization qualities and reveal the responsible mechanisms. This is important for the design of large-scale optoelectronic devices based on thin-film hybrid halide perovskites.

Keyword:

hybrid halide perovskites two-dimensional patterning periodical grids random lasing large-scale thin-film networks

Author Community:

  • [ 1 ] [Hu, Jingyun]Beijing Univ Technol, Inst Informat Photon Technol, Beijing 100124, Peoples R China
  • [ 2 ] [Zhang, Xinping]Beijing Univ Technol, Inst Informat Photon Technol, Beijing 100124, Peoples R China
  • [ 3 ] [Xue, Haibin]Chinese Peoples Liberat Army, Gen Hosp, Med Ctr 8, Beijing 100091, Peoples R China

Reprint Author's Address:

  • 张新平

    [Zhang, Xinping]Beijing Univ Technol, Inst Informat Photon Technol, Beijing 100124, Peoples R China

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Source :

CRYSTALS

Year: 2021

Issue: 9

Volume: 11

2 . 7 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:116

JCR Journal Grade:2

Cited Count:

WoS CC Cited Count: 6

SCOPUS Cited Count: 5

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 7

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