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Abstract:
We report dependence of random lasing performance of directly spin-coated multicrystalline thin films of an organic-inorganic hybrid, halide perovskite CH3NH3PbBr3 (MAPbBr(3)), on different substrates. It was discovered that random lasing performance is strongly dependent on the surface energy properties of the substrate, which determine the morphology and crystallization properties of the spin-coated film, and will consequently determine its optical scattering and emission properties. Using indium-tin oxide (ITO)-coated glass, fused silica, and tricyclo[5.2.1.0(2,6)] decanedimethanol diacrylate (ADCP)-coated fused silica as the substrate materials, we compared the spectroscopic response of the random lasers and thus justified the photophysical mechanisms involved. The modification of the surface properties of the substrate enables controlling of the MAPbBr(3) crystallization and leads to the changing of the random lasing properties. The discoveries herein are also important for the construction of other types of laser devices, where the substrate effects should be considered during the design and preparation of the micro-/nano structures.
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CRYSTALS
Year: 2022
Issue: 3
Volume: 12
2 . 7
JCR@2022
2 . 7 0 0
JCR@2022
ESI Discipline: MATERIALS SCIENCE;
ESI HC Threshold:66
JCR Journal Grade:2
CAS Journal Grade:3
Cited Count:
WoS CC Cited Count: 2
SCOPUS Cited Count: 2
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 5
Affiliated Colleges: