Abstract:
研究了重稀土元素铒[Er(Ⅲ)]对短程硝化工艺的短期和长期脱氮效能影响,并进行了相关动力学分析.短期实验表明,0~10mg/L的Er(Ⅲ)对AOB菌活性呈现促进作用,20~60mg/L的Er(Ⅲ)对AOB菌活性呈现轻度抑制,80~120mg/L的Er(Ⅲ)则对AOB菌活性呈现重度抑制.AOB菌会吸附大量Er(Ⅲ),在进水Er(Ⅲ)浓度低于60mg/L时,Er(Ⅲ)去除率均大于90%,高于60mg/L后Er(Ⅲ)去除率逐渐降低.ICP-MS和EDS分析结果表明,Er(Ⅲ)可被AOB菌胞外吸附和胞内摄取,其中又以胞外吸附为主.分别采用Vadivelu模型、Hellinga模型、Michaelis-Menten模型和Hill模型对实验结果进行拟合,结果表明通过分段拟合(0~60mg/L和60~120mg/L)Hill模型能较好的描述Er(Ⅲ)对AOB菌的抑制动力学过程,拟合得到的R2分别为0.9879和0.9999,最大基质去除速率qmax(ΔSNPR)分别为2.59mg/(g·h)和7.15mg/(g·h).长期试验表明,10mg/L的Er(Ⅲ)将使短程硝化系统性能逐渐消失,停止添加Er(Ⅲ)后,反应系统性能也不能恢复.
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Source :
化工进展
ISSN: 1000-6613
Year: 2023
Issue: 3
Volume: 42
Page: 1659-1668
Cited Count:
WoS CC Cited Count: 0
SCOPUS Cited Count:
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count: -1
Chinese Cited Count:
30 Days PV: 0
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