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Author:

Wang, Ce (Wang, Ce.) | Zhu, Jiahao (Zhu, Jiahao.) | Jin, Yuhong (Jin, Yuhong.) | Liu, Jingbing (Liu, Jingbing.) | Wang, Hao (Wang, Hao.) (Scholars:汪浩) | Zhang, Qianqian (Zhang, Qianqian.)

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EI Scopus SCIE

Abstract:

Homogeneous ion transport during Li+ plating/stripping plays a significant role in the stability of Li metal anodes (LMAs) and the electrochemical performance of Li metal batteries (LMBs). Controlled ion transport with uniform Li+ distribution is expected to suppress notorious Li dendrite growth while stabilizing the susceptible solid electrolyte interfacial (SEI) film and optimizing the electrochemical stability. Here, we are committed to rendering a comprehensive study of Li+ transport during the Li plating/stripping process related to the interactions between the Li dendrites and SEI film. Moreover, rational ion modulation strategies based on functional separators, artificial SEI films, solid-state electrolytes and structured anodes are introduced to homogenize Li+ flux and stabilize the lithium metal surface. Finally, the current issues and potential opportunities for ion transport regulation to boost the high energy density of LMBs are described.

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Author Community:

  • [ 1 ] [Wang, Ce]Beijing Univ Technol, Fac Mat & Mfg, Key Lab New Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 2 ] [Zhu, Jiahao]Beijing Univ Technol, Fac Mat & Mfg, Key Lab New Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 3 ] [Jin, Yuhong]Beijing Univ Technol, Fac Mat & Mfg, Key Lab New Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 4 ] [Liu, Jingbing]Beijing Univ Technol, Fac Mat & Mfg, Key Lab New Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 5 ] [Wang, Hao]Beijing Univ Technol, Fac Mat & Mfg, Key Lab New Funct Mat, Minist Educ, Beijing 100124, Peoples R China
  • [ 6 ] [Zhang, Qianqian]Beijing Univ Technol, Fac Mat & Mfg, Key Lab New Funct Mat, Minist Educ, Beijing 100124, Peoples R China

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Source :

MATERIALS HORIZONS

ISSN: 2051-6347

Year: 2023

Issue: 9

Volume: 10

Page: 3218-3236

1 3 . 3 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:26

Cited Count:

WoS CC Cited Count: 6

SCOPUS Cited Count: 6

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 5

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