Patterning　of　luminescent　nanomaterials　is　critical　in　the　fields　of　display　and　information　encryption,　and　inkjet　printing　technology　have　shown　remarkable　significance　with　the　advantage　of　fast,　large-scalable　and　integrative.　However,　inkjet　printing　nanoparticle　deposits　with　high-resolution　and　well　controlled　morphology　from　nonpolar　solvent　droplets　is　still　challenging.　Herein,　a　facile　approach　of　nonpolar　solvent　modulated　inkjet　printing　of　nanoparticles　self-assembly　patterns　driven　by　the　shrinkage　of　the　droplet　and　inner　solutal　convection　is　proposed.　Through　regulating　the　solvent　composition　and　nanoparticle　concentration,　multicolor　light-emissive　upconversion　nanoparticle　self-assembly　microarrays　with　tunable　morphologies　are　achieved,　showing　the　integration　of　designable　microscale　morphologies　and　photoluminescences　for　multimodal　anti-counterfeit.　Furthermore,　inkjet　printing　of　nanoparticles　self-assembled　continuous　lines　with　adjustable　morphologies　by　controlling　the　coalescence　and　drying　of　the　ink　droplets　is　achieved.　The　high　resolution　of　inkjet　printing　microarrays　and　continuous　lines＇　width　＜　5　and　10　mu　m　is　realized,　respectively.　This　nonpolar　solvent-modulated　inkjet　printing　of　nanoparticle　deposits　approach　facilitates　the　patterning　and　integration　of　different　nanomaterials,　and　is　expected　to　provide　a　versatile　platform　for　fabricating　advanced　devices　applied　in　photonics　integration,　micro-LED,　and　near-field　display.