Abstract:
腐殖酸(Humic acid,HA)是水体中常见的膜污染物质和消毒副产物前驱体.通过真空抽滤将碳纳米管(Carbon nanotubes,CNTs)和氧化石墨烯(Graphene oxide,GO)负载于基膜表面,结合聚多巴胺(Polydopamine,PDA)的交联黏合功能,制备了 GO/PDA/CNT双层低压膜.采用ATR-FTIR分析证实了 PDA在GO膜表面的聚合,通过超声破碎验证了双层膜的稳定性.结果表明,GO/PDA/CNT双层膜性能稳定,渗透通量达到1 238 L/(m2·h·MPa),高于GO膜的279 L/(m2·h·MPa).该膜对HA的去除率达到88.5%,均高于GO膜(85.8%)和CNT膜(38.9%).GO膜和CNT膜的比通量在过滤HA过程中分别降至0.314和0.697,GO/PDA/CNT双层膜的比通量下降幅度最小(0.753).提高搅拌速率有利于双层膜对HA的去除并进一步缓解膜污染,但搅拌速率过高会加剧膜污染;酸性条件下双层膜对HA去除率最高(94.5%),膜污染相较于中性和碱性条件更为严重.GO/PDA/CNT双层膜的制备,有助于提高膜滤效率和强化腐殖质类有机物的去除,减少消毒副产物的产生.
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膜科学与技术
ISSN: 1007-8924
Year: 2023
Issue: 6
Volume: 43
Page: 61-70
Cited Count:
WoS CC Cited Count: 0
SCOPUS Cited Count:
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count: -1
Chinese Cited Count:
30 Days PV: 6
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