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Author:

Han, Weina (Han, Weina.) | Jiang, Lan (Jiang, Lan.) | Li, Xiaowei (Li, Xiaowei.) | Wang, Qingsong (Wang, Qingsong.) | Wang, Shaojun (Wang, Shaojun.) | Hu, Jie (Hu, Jie.) | Lu, Yongfeng (Lu, Yongfeng.)

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Scopus SCIE PubMed

Abstract:

We demonstrated an abnormal double-peak (annular shaped) energy deposition through dual-wavelength synthesis of the fundamental frequency (omega) and the second-harmonic frequency (2 omega) of a femtosecond (fs) Ti: sapphire laser. The annular shaped distribution of the dual-wavelength fs laser was confirmed through real beam shape detection. This uniquely simple and flexible technique enables the formation of functional plasmonic nanostructures. We applied this double-peak fs-laser-induced dewetting effect to the controlled fabrication and precise deposition of Au nanostructures, by using a simple, lithography-free, and single-step process. In this process, the double-peak energy-shaped fs laser pulse induces surface patterning of a thin film followed by nanoscale hydrodynamic instability, which is highly controllable under specific irradiation conditions. Nanostructure morphology (shape, size, and distribution) modulation can be achieved by adjusting the laser irradiation parameters, and the subsequent ion-beam polishing enables further dimensional reduction and removal of the surrounding film. The unique optical properties of the resulting nanostructure are highly sensitive to the shape and size of the nanostructure. In contrast to a nanoparticle, the resonance-scattering spectrum of an Au nanobump exhibites two resonance peaks. These suggest that the dual-wavelength fs laser-based dewetting of thin films can be an effective means for the scalable manufacturing of patterned-functional nanostructures.

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Author Community:

  • [ 1 ] [Han, Weina]Beijing Univ Technol, Beijing Engn Res Ctr Appl Laser Technol, Inst Laser Engn, Beijing 100124, Peoples R China
  • [ 2 ] [Han, Weina]Beijing Inst Technol, Laser Micro Nano Fabricat Lab, Sch Mech Engn, Beijing 100081, Peoples R China
  • [ 3 ] [Jiang, Lan]Beijing Inst Technol, Laser Micro Nano Fabricat Lab, Sch Mech Engn, Beijing 100081, Peoples R China
  • [ 4 ] [Li, Xiaowei]Beijing Inst Technol, Laser Micro Nano Fabricat Lab, Sch Mech Engn, Beijing 100081, Peoples R China
  • [ 5 ] [Wang, Qingsong]Beijing Inst Technol, Laser Micro Nano Fabricat Lab, Sch Mech Engn, Beijing 100081, Peoples R China
  • [ 6 ] [Wang, Shaojun]Beijing Inst Technol, Laser Micro Nano Fabricat Lab, Sch Mech Engn, Beijing 100081, Peoples R China
  • [ 7 ] [Hu, Jie]Beijing Inst Technol, Laser Micro Nano Fabricat Lab, Sch Mech Engn, Beijing 100081, Peoples R China
  • [ 8 ] [Jiang, Lan]Tsinghua Univ, Laser Micro Nanofabricat Lab, Dept Mech Engn, Beijing 100084, Peoples R China
  • [ 9 ] [Lu, Yongfeng]Univ Nebraska, Dept Elect & Comp Engn, Lincoln, NE 68588 USA

Reprint Author's Address:

  • [Jiang, Lan]Beijing Inst Technol, Laser Micro Nano Fabricat Lab, Sch Mech Engn, Beijing 100081, Peoples R China;;[Jiang, Lan]Tsinghua Univ, Laser Micro Nanofabricat Lab, Dept Mech Engn, Beijing 100084, Peoples R China

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Source :

SCIENTIFIC REPORTS

ISSN: 2045-2322

Year: 2017

Volume: 7

4 . 6 0 0

JCR@2022

ESI Discipline: Multidisciplinary;

ESI HC Threshold:283

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count: 16

SCOPUS Cited Count: 17

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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