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Author:

Lang, Jianlei (Lang, Jianlei.) (Scholars:郎建垒) | Zhou, Ying (Zhou, Ying.) | Chen, Dongsheng (Chen, Dongsheng.) (Scholars:陈东升) | Xing, Xiaofan (Xing, Xiaofan.) | Wei, Lin (Wei, Lin.) | Wang, Xiaotong (Wang, Xiaotong.) | Zhao, Na (Zhao, Na.) | Zhang, Yanyun (Zhang, Yanyun.) | Guo, Xiurui (Guo, Xiurui.) | Han, Lihui (Han, Lihui.) | Cheng, Shuiyuan (Cheng, Shuiyuan.) (Scholars:程水源)

Indexed by:

EI Scopus SCIE PubMed

Abstract:

Many studies have been conducted focusing on the contribution of land emission sources to PM2.5 in China; however, little attention had been paid to other contributions, especially the secondary contributions from shipping emissions to atmospheric PM2.5. In this study, a combined source apportionment approach, including principle component analysis (PCA) and WRF-CMAQ simulation, was applied to identify both primary and secondary contributions from ships to atmospheric PM2.5. An intensive PM2.5 observation was conducted from April 2014 to January 2015 in Qinhuangdao, which was close to the largest energy output port of China. The chemical components analysis results showed that the primary component was the major contributor to PM2.5, with proportions of 483%, 48.9%, 55.1% and 55.4% in spring, summer, autumn and winter, respectively. The secondary component contributed higher fractions in summer (48.2%) and winter (36.8%), but had lower percentages in spring (30.1%) and autumn (32.7%). The hybrid source apportionment results indicated that the secondary contribution (SC) of shipping emissions to PM2.5 could not be ignored. The annual average SC was 2.7%, which was comparable to the primary contribution (2.9%). The SC was higher in summer (5.3%), but lower in winter (1.1%). The primary contributions to atmospheric PM2.5 were 3.0%, 2.5%, 3.4% and 2.7% in spring, summer, autumn and winter, respectively. As for the detailed chemical components, the contributions of shipping emissions were 23%, 0.5%, 0.1%, 1.0%, 1.7% and 0.1% to elements & sea salt, primary organic aerosol (POA), element carbon (EC), nitrate, sulfate and secondary organic carbon (SOA), respectively. The results of this study will further the understanding of the implications of shipping emissions in PM2.5 pollution. (C) 2017 Elsevier Ltd. All rights reserved.

Keyword:

Shipping emissions Fine particle WRF-CMAQ Qinhuangdao Source apportionment PCA

Author Community:

  • [ 1 ] [Lang, Jianlei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 2 ] [Zhou, Ying]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 3 ] [Chen, Dongsheng]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 4 ] [Xing, Xiaofan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 5 ] [Wei, Lin]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 6 ] [Wang, Xiaotong]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 7 ] [Zhao, Na]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 8 ] [Zhang, Yanyun]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 9 ] [Guo, Xiurui]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 10 ] [Han, Lihui]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China
  • [ 11 ] [Cheng, Shuiyuan]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China

Reprint Author's Address:

  • 郎建垒 陈东升

    [Lang, Jianlei]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China;;[Chen, Dongsheng]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Coll Environm & Energy Engn, Beijing 100124, Peoples R China

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Source :

ENVIRONMENTAL POLLUTION

ISSN: 0269-7491

Year: 2017

Volume: 229

Page: 557-566

8 . 9 0 0

JCR@2022

ESI Discipline: ENVIRONMENT/ECOLOGY;

ESI HC Threshold:228

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 46

SCOPUS Cited Count: 58

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 7

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