• Complex
  • Title
  • Keyword
  • Abstract
  • Scholars
  • Journal
  • ISSN
  • Conference
搜索

Author:

Liu, Lisha (Liu, Lisha.) | Song, Yong (Song, Yong.) | Fu, Zhidan (Fu, Zhidan.) | Ye, Qing (Ye, Qing.) (Scholars:叶青) | Cheng, Shuiyuan (Cheng, Shuiyuan.) (Scholars:程水源) | Kang, Tianfang (Kang, Tianfang.) (Scholars:康天放) | Dai, Hongxing (Dai, Hongxing.) (Scholars:戴洪兴)

Indexed by:

EI Scopus SCIE

Abstract:

The cryptomelane-type manganese oxide octahedral molecular sieve (OMS-2)-supported Pd (0.5 wt% Pd/OMS-2-DP, 0.5 wt% Pd/OMS-2-PI, and 0.5 wt% Pd/OMS-2-EX) catalysts were prepared by the deposition-precipitation, pre-incorporation, and ion-exchanging strategies, respectively. It is shown that the preparation method exerted an important effect on the physicochemical property of the sample. Among the OMS-2-supported Pd catalysts, 0.5 wt% Pd/OMS-2-DP possessed the highest surface (Mn2+ + Mn3+)/Mn4+ atomic ratio and the highest surface Pd loading and acid sites. The 0.5 wt% Pd/OMS-2 catalysts outperformed the Pd-free counterpart, among which 0.5 wt% Pd/OMS-2-DP presented the best catalytic activity (T-50% and T-90% were 25 and 55 degrees C for CO oxidation, 240 and 285 degrees C for toluene oxidation, and 160 and 200 degrees C for ethyl acetate oxidation, respectively). We believe that the high Pd surface loading, high surface atomic ratio of (Mn2+ + Mn3+)/Mn4+, and good low-temperature reducibility, good oxygen mobility, and high acidity were responsible for the excellent performance of the 0.5 wt% Pd/OMS-2-DP catalyst. (C) 2016 Elsevier B.V. All rights reserved.

Keyword:

Supported Pd catalyst Cryptomelane-type manganese oxide octahedral molecular sieve Carbon monoxide oxidation Oxygen mobility Volatile organic compound combustion

Author Community:

  • [ 1 ] [Liu, Lisha]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Environm Sci, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 2 ] [Song, Yong]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Environm Sci, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 3 ] [Fu, Zhidan]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Environm Sci, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 4 ] [Ye, Qing]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Environm Sci, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 5 ] [Cheng, Shuiyuan]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Environm Sci, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 6 ] [Kang, Tianfang]Beijing Univ Technol, Coll Environm & Energy Engn, Dept Environm Sci, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
  • [ 7 ] [Dai, Hongxing]Beijing Univ Technol, Key Lab Beijing Reg Air Pollut Control, Beijing Key Lab Green Catalysis & Separat, Dept Chem & Chem Engn,Coll Environm & Energy Engn, Beijing 100124, Peoples R China

Reprint Author's Address:

  • 叶青 戴洪兴

    [Ye, Qing]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China;;[Dai, Hongxing]Beijing Univ Technol, Coll Environm & Energy Engn, Beijing 100124, Peoples R China

Show more details

Related Keywords:

Source :

APPLIED SURFACE SCIENCE

ISSN: 0169-4332

Year: 2017

Volume: 396

Page: 599-608

6 . 7 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:287

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 60

SCOPUS Cited Count: 62

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 4

Online/Total:638/10516311
Address:BJUT Library(100 Pingleyuan,Chaoyang District,Beijing 100124, China Post Code:100124) Contact Us:010-67392185
Copyright:BJUT Library Technical Support:Beijing Aegean Software Co., Ltd.