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学者姓名：魏佳
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Abstract ：
Peracetic acid (PAA) as emerging oxidant in advanced oxidation processes (AOPs) has attracted widespread attention in purifying water pollution. In this research, the removal of target contaminant (sulfamethoxazole, SMX) was investigated through PAA activation by a facile catalyst (Co@C), and the active sites of catalyst were identified as sp(3)-C, O-ads, and Co-0 by correlation analysis. Especially, different pH adjustment strategies were designed, including System A (adjusting pH after adding PAA) and System B (adjusting pH before adding PAA), to investigate the impact of oxidant acidity and alkalinity on solution microenvironment as well as effect and mechanism of pollutant removal. The results showed that HO and CH3C(O)OO dominated in System A, while Co(IV)O2+ was also observed in System B. Both systems showed optimal SMX degradation (98 %). However, System A exhibited excellent water quality tolerance (efficiency > 78 %), superior sustained catalyst activation (efficiency > 80 % in 40 h), less ion leaching (41 mu g L-1), and lower products toxicity. Moreover, the pH of solution after reaction in System B was intensely acidic, requiring costly pH adjustments for discharge. This study unveils the strategy of adjusting pH after adding PAA is preferable for water purification, enriching the emerging research of PAA-based AOPs for the remediation of environments.
Keyword ：
Peracetic acid Peracetic acid Emerging contaminants Emerging contaminants pH -dependent removal pH -dependent removal Radical oxidation process Radical oxidation process Co -based catalyst Co -based catalyst
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| GB/T 7714 | Niu, Xiruo , Wei, Jia , Jiang, Zijian et al. New insights into the pH-dependent removal of sulfamethoxazole in peracetic acid activation systems: From mechanistic exploration to practical application potentials [J]. | JOURNAL OF HAZARDOUS MATERIALS , 2024 , 474 . |
| MLA | Niu, Xiruo et al. "New insights into the pH-dependent removal of sulfamethoxazole in peracetic acid activation systems: From mechanistic exploration to practical application potentials" . | JOURNAL OF HAZARDOUS MATERIALS 474 (2024) . |
| APA | Niu, Xiruo , Wei, Jia , Jiang, Zijian , Cui, Xueru , Li, Yanan , Cui, Nan et al. New insights into the pH-dependent removal of sulfamethoxazole in peracetic acid activation systems: From mechanistic exploration to practical application potentials . | JOURNAL OF HAZARDOUS MATERIALS , 2024 , 474 . |
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Abstract ：
The pervasive presence of antibiotics in the environment poses ecological risks and jeopardizes human health. Herein, a simple one-step hydrothermal method was used to prepare a boron-doped (B-doped) bimetallic carbon felt as a cathode for the heterogeneous electro-Fenton (HEF) system. In the HEF process, the modified electrode (B-Co/Fe@CF) demonstrated exceptional efficiency in degrading the target pollutant doxycycline (DOX), owing to its maximal degree of defect and minimal electrochemical impedance. In addition, XPS and structure-activity relationship analysis results revealed that the superior performance of the modified electrode stemmed from the predominant influence of sp(3)/sp(2), C=O and metal-boron (M-B) groups in initiating the production of H2O2 and the consequent formation of reactive oxygen species (ROS). Meanwhile, the introduction of non-metallic boron species significantly accelerated the sustainable cycling of Co(II)/Co(III) and Fe(II)/Fe(III). The quenching and probe experiments suggested that the radicals center dot O-2(-) and center dot OH significantly contributed to the elimination of DOX. Moreover, the advanced B-Co/Fe@CF-HEF system exhibited remarkable versatility, stability and effectiveness throughout the degradation process. Three pathways for the degradation of the pollutants were identified using density functional theory (DFT) calculations and LC-MS detection. Additionally, the treated DOX solution significantly reduced the toxicity to the growth of E. coli and mung bean in actual toxicity experiments. This research presented a novel outlook on developing the B-doped metal catalysts for efficient degradation of pollutants and showcased promising applications in organic wastewater treatment.
Keyword ：
Heterogeneous electro-Fenton Heterogeneous electro-Fenton Organic contaminants Organic contaminants Degradation Degradation Bimetal Bimetal Boron-doped Boron-doped
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| GB/T 7714 | Ji, Wei , Wei, Jia , Xu, Mengdie et al. Enhanced organic contaminant eradication using boron-doped bimetallic cathodes in electro-Fenton: Unveiling structure-activity relationship [J]. | CHEMICAL ENGINEERING JOURNAL , 2024 , 496 . |
| MLA | Ji, Wei et al. "Enhanced organic contaminant eradication using boron-doped bimetallic cathodes in electro-Fenton: Unveiling structure-activity relationship" . | CHEMICAL ENGINEERING JOURNAL 496 (2024) . |
| APA | Ji, Wei , Wei, Jia , Xu, Mengdie , Wang, Linhao , Huo, Jiangkai , Li, Yanan et al. Enhanced organic contaminant eradication using boron-doped bimetallic cathodes in electro-Fenton: Unveiling structure-activity relationship . | CHEMICAL ENGINEERING JOURNAL , 2024 , 496 . |
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Abstract ：
Recently, atomically dispersed dual-metal sites carbocatalysts (DMSCs) make a wave in the field of persulfate-based advanced oxidation processes (PS-AOPs) in light of their approximate to 100% atomic utilization efficiency, high density of active sites, and superior catalytic activity. This review aims to provide a state-of-the-art overview on the development of DMSCs for activating PS. Initially, the types and properties of DMSCs are summarized, as well as the role of doping different heteroatoms is discussed. Subsequently, the properties of different carbon carriers and the methods for the synthesis of DMSCs are outlined. After that, the mechanism and application of DMSCs for the activation of PS toward organic contaminants degradation are revealed. Particularly, the mechanism of nonradical pathway is described, and the necessity of coupling DMSCs-based PS-AOPs to other processes for practical water treatment is emphasized. Finally, the formidable challenges and future research directions of DMSCs are proposed. This review is expected to provide insight into the preparation of DMSCs in the field of nanomaterials and to broaden the path for their environmental applications.
Keyword ：
dual-metal sites dual-metal sites persulfate persulfate organic contaminants organic contaminants advanced oxidation processes advanced oxidation processes carbocatalysts carbocatalysts
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| GB/T 7714 | Li, Yanan , Wei, Jia , Cui, Nan et al. Recent Advance of Atomically Dispersed Dual-Metal Sites Carbocatalysts: Properties, Synthetic Materials, Catalytic Mechanisms, and Applications in Persulfate-Based Advanced Oxidation Process [J]. | ADVANCED FUNCTIONAL MATERIALS , 2023 , 33 (30) . |
| MLA | Li, Yanan et al. "Recent Advance of Atomically Dispersed Dual-Metal Sites Carbocatalysts: Properties, Synthetic Materials, Catalytic Mechanisms, and Applications in Persulfate-Based Advanced Oxidation Process" . | ADVANCED FUNCTIONAL MATERIALS 33 . 30 (2023) . |
| APA | Li, Yanan , Wei, Jia , Cui, Nan , Li, Jiamei , Xu, Mengdie , Pan, Guoping et al. Recent Advance of Atomically Dispersed Dual-Metal Sites Carbocatalysts: Properties, Synthetic Materials, Catalytic Mechanisms, and Applications in Persulfate-Based Advanced Oxidation Process . | ADVANCED FUNCTIONAL MATERIALS , 2023 , 33 (30) . |
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Abstract ：
In recent years, metal-free catalysts for persulfate-mediated oxidation processes have been widely applied to remove contaminants in the aquatic environment. Herein, a simple pyrolysis approach was used to synthesize the boron doped biochars (B@TBCs) derived from boric acid mixed with tea seed shells powders. The obtained B@TBCs exhibited fantastic capability to boost PMS (0.5 mM) activation for 90%~ removal of oxytetracycline (OTC) within 20 min. Through the correlation analysis and DFT calculations, it was concluded that the apparent rate constant of pollutants removal was greatly related to the-O-B -O-groups on the biochars, which could improve the electron-donating capacity of the biochar. In addition, the degradation process of OTC was pH -dependent because of the changed roles of ROSs under different pH. Finally, according to the DFT calcula-tion, LC-MS and toxicological analysis, the degradation pathways of pollutants and the toxicity changes during the degradation process were obtained. These findings consolidated the theoretical basis for further boosting the catalytic activity of B-doped biochars and expanded the imagination for the modification of other metal-free biochar catalysts for PMS activation.
Keyword ：
-O-B-O-moieties -O-B-O-moieties Density function theory Density function theory Antibiotic Antibiotic Peroxymonosulfate activation Peroxymonosulfate activation Boron doped biochar Boron doped biochar
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| GB/T 7714 | Pan, Guoping , Wei, Jia , Xu, Mengdie et al. Insight into boron-doped biochar as efficient metal-free catalyst for peroxymonosulfate activation: Important role of-O-B-O- moieties [J]. | JOURNAL OF HAZARDOUS MATERIALS , 2023 , 445 . |
| MLA | Pan, Guoping et al. "Insight into boron-doped biochar as efficient metal-free catalyst for peroxymonosulfate activation: Important role of-O-B-O- moieties" . | JOURNAL OF HAZARDOUS MATERIALS 445 (2023) . |
| APA | Pan, Guoping , Wei, Jia , Xu, Mengdie , Li, Jiamei , Wang, Linhao , Li, Yanan et al. Insight into boron-doped biochar as efficient metal-free catalyst for peroxymonosulfate activation: Important role of-O-B-O- moieties . | JOURNAL OF HAZARDOUS MATERIALS , 2023 , 445 . |
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Abstract ：
Electro-Fenton is one of the promising clean and renewable technologies for refractory pollutants control. Herein, a ternary metal-layered double hydroxide (CoFeCe-LDH) nanoparticle in situ growth on carbon felt (CF) was prepared to fabricate heterogeneous electro-Fenton (HEF) cathode via one-pot hydrothermal strategy. The optimal CoFeCe-LDH@CF cathode demonstrated high oxygen reduction activity, low resistance and efficient degradation of DOX over a wide pH range (pH = 1-9). On one hand, the introduction of Ce resulted in the generation of plenty of oxygen vacancies (O-alpha) on the electrode surface. On the other hand, the coexistence of Co2+/Co3+, Fe2+/Fe3+ and Ce3+/Ce4+ redox pairs significantly enhanced interfacial electron transfer and promoted the generation and decomposition of in situ H2O2, which in turn boosted the production of reactive radicals ((OH)-O-center dot, O-2(center dot-) and O-1(2)). The Estimation Program Interface (EPI) certificated that intermediates resulted from DOX degradation in the system were relatively low in toxicity to typical aquatic organisms. Meanwhile, the effect experiments of various ions, types of wastewater and pollutants were carried out in the CoFeCe-LDH@CFs-HEF system and all showed excellent pollutant degradation, proving that the developed cathode had special applicability and reusability. Thus, this paper gave a global contribution to develop the high-performance cathode by exploring the synergistic effects of trimetals in LDH and proposed a reliable strategy for enhanced degradation of contaminant by HEF system.
Keyword ：
Heterogeneous electro-Fenton Heterogeneous electro-Fenton Oxygen vacancies Oxygen vacancies Antibiotic Antibiotic Layered double hydroxide Layered double hydroxide Cerium Cerium
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| GB/T 7714 | Xu, Mengdie , Wei, Jia , Cui, Xueru et al. High-efficiency electro-Fenton process based on in-situ grown CoFeCe-LDH@CFs free-standing cathodes: Correlation of cerium and oxygen vacancies with H2O2 [J]. | CHEMICAL ENGINEERING JOURNAL , 2022 , 455 . |
| MLA | Xu, Mengdie et al. "High-efficiency electro-Fenton process based on in-situ grown CoFeCe-LDH@CFs free-standing cathodes: Correlation of cerium and oxygen vacancies with H2O2" . | CHEMICAL ENGINEERING JOURNAL 455 (2022) . |
| APA | Xu, Mengdie , Wei, Jia , Cui, Xueru , Li, Jiamei , Pan, Guoping , Li, Yanan et al. High-efficiency electro-Fenton process based on in-situ grown CoFeCe-LDH@CFs free-standing cathodes: Correlation of cerium and oxygen vacancies with H2O2 . | CHEMICAL ENGINEERING JOURNAL , 2022 , 455 . |
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Abstract ：
Metal sulfides have been found to be effective in removing organic pollutants from water in environmental catalysis. In this study, a porous graphitic biochar wrapped Co9S8 core-shell composite (Co9S8@N-O-BC) was designed for efficient activation of peroxymonosulfate (PMS) and degradation of sulfamethoxazole in an aqueous environment. Based on complementary characterizations and reactive oxygen species (ROS) quenching experiments, we proposed that boosted Co(ii) regeneration by various existing S species along with formed N and O active sites in Co9S8@N-O-BC facilitated the cleavage of the O-O bond of PMS, thus resulting in a high-efficiency non-radical pathway. Consequently, Co9S8@N-O-BC/PMS achieved an outstanding degradation of sulfamethoxazole (100%) within 4 min in a wide pH range (3-11) and its turnover frequency (TOF) value was 11.96 min(-1), up to 117 times higher than other reported catalysts as far as we know. The superior stability and wide applicability in sulfamethoxazole degradation with a series of inorganic ions, especially the production of very few harmless intermediates and the exceptional mineralization efficiency, also further demonstrated that the obtained catalyst possessed excellent potential for practical wastewater treatment.
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| GB/T 7714 | Li, Jiamei , Wei, Jia , Xu, Mengdie et al. A porous graphitic biochar wrapped Co9S8 core-shell composite enables pH-universal activation of peroxymonosulfate for highly efficient and rapid antibiotics degradation [J]. | ENVIRONMENTAL SCIENCE-NANO , 2022 , 9 (9) : 3629-3645 . |
| MLA | Li, Jiamei et al. "A porous graphitic biochar wrapped Co9S8 core-shell composite enables pH-universal activation of peroxymonosulfate for highly efficient and rapid antibiotics degradation" . | ENVIRONMENTAL SCIENCE-NANO 9 . 9 (2022) : 3629-3645 . |
| APA | Li, Jiamei , Wei, Jia , Xu, Mengdie , Pan, Guoping , Zhang, Yifei , Xing, Luyi et al. A porous graphitic biochar wrapped Co9S8 core-shell composite enables pH-universal activation of peroxymonosulfate for highly efficient and rapid antibiotics degradation . | ENVIRONMENTAL SCIENCE-NANO , 2022 , 9 (9) , 3629-3645 . |
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Abstract ：
Metal organic frameworks (MOFs) have been widely concerned by researchers as catalytic materials. In this work, nitrogen doped Fe, Co bimetallic MOF named FeCo/N-MOF was prepared by "one-pot" hydrothermal method as a catalyst for activating persulfate to degrade tetracycline. The hexagonal spindle crystals morphology and porous structure were observed on the FeCo/N-MOF. The X-ray photoelectron spectroscopy (XPS) showed that Fe(III) and Co(II) were the main active sites and the presence of pyrrole N was positive to the catalysis. The different conditions of catalyst dosage, pH and persulfate concentration were discussed to further understand the mechanism of FeCo/N-MOF on tetracycline (TC) degradation. The results revealed that about 99% of tetracycline was degraded in 150 min when FeCo/N-MOF was 0.4 g/L and persulfate was 5 mmol/L in a wide range of pH from 3 to 9. Moreover, the reaction stoichiometric efficiency of persulfate was 6.13%. There were radicals and non-radical pathways in the process of TC degradation and the superoxide radical was the main active sub-stances. This study suggested that FeCo/N-MOF was of great potential in persulfate activation for water puri-fication, which also provided a platform for MOF-derived catalysts in the field of advanced oxidation.
Keyword ：
MOF MOF Persulfate Persulfate Nitrogen -doped Nitrogen -doped Tetracycline Tetracycline Bimetal Bimetal
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| GB/T 7714 | Zhang, Yifei , Wei, Jia , Xing, Luyi et al. Superoxide radical mediated persulfate activation by nitrogen doped bimetallic MOF (FeCo/N-MOF) for efficient tetracycline degradation [J]. | SEPARATION AND PURIFICATION TECHNOLOGY , 2022 , 282 . |
| MLA | Zhang, Yifei et al. "Superoxide radical mediated persulfate activation by nitrogen doped bimetallic MOF (FeCo/N-MOF) for efficient tetracycline degradation" . | SEPARATION AND PURIFICATION TECHNOLOGY 282 (2022) . |
| APA | Zhang, Yifei , Wei, Jia , Xing, Luyi , Li, Jiamei , Xu, Mengdie , Pan, Guoping et al. Superoxide radical mediated persulfate activation by nitrogen doped bimetallic MOF (FeCo/N-MOF) for efficient tetracycline degradation . | SEPARATION AND PURIFICATION TECHNOLOGY , 2022 , 282 . |
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Abstract ：
To address the current water pollution issues, one of the most important technologies is the development of efficient and environmental-friendly catalysts for the treatment of organic pollutants in water. In this study, a nitrogen-enriched biochar encapsulated cobalt nanoparticles composite (Co@N-BC) was synthesized using a one- step pyrolysis method based on metal-organic frameworks (MOFs) and leaf biomass as precursors. The obtained Co@N-BC possessed more functional group, large specific surface area and less cobalt ion leaching, which were used for efficient persulfate (PS) activation for approximately 92.72% DOX (50 mg/L) removal in 30 min. The quenching test, electron paramagnetic resonance (EPR), and electrochemical characterization of the Co@N-BC/ PS system revealed that electron transfer was the primary pathway for DOX elimination. Moreover, the Co@N- BC/PS system had satisfactory stability in a wide pH range (2-10) and was not adversely affected by the various anions or water matrix. This research will shed new light on the design and development of MOF derivatives, as well as provide technical support for the eradication of antibiotics.
Keyword ：
Electron transfer Electron transfer Biochar Biochar Persulfate Persulfate Co nanoparticles Co nanoparticles MOFs derivatives MOFs derivatives Doxycycline Doxycycline
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| GB/T 7714 | Jiang, Zijian , Wei, Jia , Zhang, Yifei et al. Electron transfer mechanism mediated nitrogen-enriched biochar encapsulated cobalt nanoparticles catalyst as an effective persulfate activator for doxycycline removal [J]. | JOURNAL OF CLEANER PRODUCTION , 2022 , 384 . |
| MLA | Jiang, Zijian et al. "Electron transfer mechanism mediated nitrogen-enriched biochar encapsulated cobalt nanoparticles catalyst as an effective persulfate activator for doxycycline removal" . | JOURNAL OF CLEANER PRODUCTION 384 (2022) . |
| APA | Jiang, Zijian , Wei, Jia , Zhang, Yifei , Niu, Xiruo , Li, Jiamei , Li, Yanan et al. Electron transfer mechanism mediated nitrogen-enriched biochar encapsulated cobalt nanoparticles catalyst as an effective persulfate activator for doxycycline removal . | JOURNAL OF CLEANER PRODUCTION , 2022 , 384 . |
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Abstract ：
There has been extensive research on biochar materials in the field of adsorption, catalysis, etc. Hereon, we reported a gentle synthesis of electrode by abundant biomass of municipal sludge and cheap precursor of boric acid as carbon source and boron source. Experimental results demonstrated that a small amount of boron doping had a profound impact on the elemental composition and active sites of sludge-based biochar significantly, resulting the improvement of EF activity for sulfamerazine (SMR) removal. Under the optimal reaction conditions, including initial pH, added divalent iron, applied current and air flow, 95.12% of SMR could be removed in 180 min in EF system. It was confirmed that hydroxyl radical (center dot OH) and superoxide radical (center dot O-2(-)) were the primary active substances for SMR degradation. The effect experiments of various ions, types of wastewater and pollutants were carried out and the stability experiments were conducted for eight cycles without significant efficiency loss, which proved the exceptional applicability and reusability of the gained boron doped sludge-based biochar electrode BSBC-E. These functions of boron-doped sludge-based biochar cathode could be a promising material for emerging organic contaminants remediation.
Keyword ：
Boron-doped Boron-doped Electro-Fenton Electro-Fenton Emerging organic contaminants Emerging organic contaminants Biochar Biochar Sludge Sludge
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| GB/T 7714 | Xing, Luyi , Wei, Jia , Zhang, Yifei et al. Boosting active sites of protogenetic sludge-based biochar by boron doping for electro-Fenton degradation towards emerging organic contaminants [J]. | SEPARATION AND PURIFICATION TECHNOLOGY , 2022 , 294 . |
| MLA | Xing, Luyi et al. "Boosting active sites of protogenetic sludge-based biochar by boron doping for electro-Fenton degradation towards emerging organic contaminants" . | SEPARATION AND PURIFICATION TECHNOLOGY 294 (2022) . |
| APA | Xing, Luyi , Wei, Jia , Zhang, Yifei , Xu, Mengdie , Pan, Guoping , Li, Jiamei et al. Boosting active sites of protogenetic sludge-based biochar by boron doping for electro-Fenton degradation towards emerging organic contaminants . | SEPARATION AND PURIFICATION TECHNOLOGY , 2022 , 294 . |
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Abstract ：
An innovative nitrogen-doped sludge-derived biochar (NSBC) electro-Fenton cathode was fabricated by a hydrothermal and pyrolysis combination method, which was applied to the degradation of sulfamethoxazole (SMX). The superficial characteristics of the optimal cathode (NSBC*@Ni-F) showed a large number of oxygen reduction reaction (ORR) electrocatalytic active sites under acidic conditions with high electrons transfer efficiency. The two nitrogen species (pyridinic-N and graphite-N) dominated the ORR electrocatalytic active sites. The H2O2 yield (195.99 mg L-1) and corresponding current efficiency (73.69 +/- 1.2%) using NSBC*@Ni-F cathode were 7 times higher than that of bare sludge biochar as cathode in EF system. An excellent SMX removal efficiency (95.72%) was achieved as well. The TOC removal achieved 85.11% and corresponding energy consumption reached as low as 12.03 kW h kg(-1). Rational reaction intermediates were put forward during EF procedure to predict and explore the SMX degradation pathway for water remediation. This study is hopeful to hew out a new road to develop eco-friendliness and cost-effective cathode material in EF system with adequate activity and reuse stabilization.
Keyword ：
Sewage sludge Sewage sludge Sulfonamide antibiotics Sulfonamide antibiotics Nitrogen-doped Nitrogen-doped Electro-Fenton Electro-Fenton Biochar Biochar
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| GB/T 7714 | Xing, Luyi , Wei, Jia , Liu, Xiaohui et al. Application of energy sustainable utilization strategy for highly efficient electro-Fenton treatment of antibiotics [J]. | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING , 2021 , 10 (1) . |
| MLA | Xing, Luyi et al. "Application of energy sustainable utilization strategy for highly efficient electro-Fenton treatment of antibiotics" . | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING 10 . 1 (2021) . |
| APA | Xing, Luyi , Wei, Jia , Liu, Xiaohui , Zhang, Yifei , Xu, Mengdie , Li, Jiamei et al. Application of energy sustainable utilization strategy for highly efficient electro-Fenton treatment of antibiotics . | JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING , 2021 , 10 (1) . |
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