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Author:

Zheng Yongzhi (Zheng Yongzhi.) | Gong Xinyu (Gong Xinyu.) | Zhou Wenyuan (Zhou Wenyuan.) | Hu Peng (Hu Peng.) | Wang Jinshu (Wang Jinshu.)

Indexed by:

EI Scopus

Abstract:

Electrochemical water splitting by electrocatalyst is one of the most promising ways for generating and utilizing hydrogen energy, and it is critical to effectively mitigate the serious energy crisis and environmental pollution. However,the widely application of electrocatalysis technology is still limited by its low conversion efficiency and high cost. For this purpose,developing electrocatalyst materials with high activity,low cost and well stability are critical to solve the above limitions. As an inexpensive and readily available two-dimensional material,molybdenum disulfide is considered as a promising candidate to replace noble metal catalysts due to its good catalytic activity for electrocatalytic hydrogen evolution,which realize the industrial application. However,the inert basal plane and low electrical conductivity of pristine MoS2 limit the further improvement of its electrocatalytic performance. In this review, starting from the mechanism of water electrolysis and the inherent feature of molybdenum disulfide electrocatalysts,the latest research progress of various modification strategies to improve the catalytic performance of MoS2 was summarized. Moreover,the intrinsic mechanism of different modification strategies in the catalytic reaction process was highlighted and their respective drawbacks were indicated. Finally,it was pointed out that the current molybdenum disulfide catalyst should be further developed towards a combination of multiple modification measures,theoretical guidance for experiments,and rapid and effective synthesis.

Keyword:

modification strategy electrocatalytic hydrogen evolution electronic structure electrocatalyst molybdenum disulfide

Author Community:

  • [ 1 ] [Zheng Yongzhi]Beijing Univ Technol, Fac Mat & Manufacture, Beijing 100124, Peoples R China
  • [ 2 ] [Gong Xinyu]Beijing Univ Technol, Fac Mat & Manufacture, Beijing 100124, Peoples R China
  • [ 3 ] [Zhou Wenyuan]Beijing Univ Technol, Fac Mat & Manufacture, Beijing 100124, Peoples R China
  • [ 4 ] [Hu Peng]Beijing Univ Technol, Fac Mat & Manufacture, Beijing 100124, Peoples R China
  • [ 5 ] [Wang Jinshu]Beijing Univ Technol, Fac Mat & Manufacture, Beijing 100124, Peoples R China

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Source :

CAILIAO GONGCHENG-JOURNAL OF MATERIALS ENGINEERING

ISSN: 1001-4381

Year: 2023

Issue: 12

Volume: 51

Page: 35-46

Cited Count:

WoS CC Cited Count: 0

SCOPUS Cited Count: 1

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 5

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