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Author:

Song, Yuwei (Song, Yuwei.) | Nie, Songlin (Nie, Songlin.) (Scholars:聂松林) | Ji, Hui (Ji, Hui.) | Qin, Tingting (Qin, Tingting.) | Ma, Zhonghai (Ma, Zhonghai.)

Indexed by:

EI Scopus SCIE

Abstract:

Combining multiple advanced oxidation processes (AOPs) is essential for the efficient treatment of dye wastewater. In this study, the degradation efficiencies of various oxidation methods, including hydrodynamic cavitation (HC), dielectric barrier discharge (DBD) plasma oxidation, ultraviolet C (UVC), and their combination HC + DBD + UVC, were investigated for Methyl Orange (MO). The photolysis of ozone (O-3) and the degradation mechanism associated with HC + DBD + UVC were analyzed to elucidate the pathway of MO degradation. The results demonstrated that the combination of HC + DBD + UVC exhibited a significantly enhanced degradation efficiency compared to other process combinations, achieving a removal efficiency exceeding 91% within a 5-min timeframe. Optimal parameters for achieving a 99.5% degradation rate of 10 mg/L MO were determined as follows: pH 4, inlet pressure of 1.5 MPa, utilization of eight UV lamps with a power input of 46.11 W. During the degradation process, hydroxyl radicals (OH) and ozone (O-3) played crucial roles, while the incorporation of UV lamps effectively mitigated ozone (O-3) emissions and enhanced the oxidation of ozone (O-3). In conjunction with the analysis of degradation products using liquid chromatography-mass spectrometry, it is highly probable that the MO degradation pathway involves reductive cleavage of the azo bond through OH attack. Compared to other experimental methods in literature, HC + DBD + UVC exhibits significant advantages such as enhanced efficiency and absence of additives. This innovative approach offers a rapid and practical on-site solution for efficient MO dye wastewater treatment.

Keyword:

Ultraviolet C DBD plasma Methyl orange Degradation Hydrodynamic cavitation

Author Community:

  • [ 1 ] [Song, Yuwei]Beijing Univ Technol, Beijing Key Lab Adv Mfg Technol, Beijing 100124, Peoples R China
  • [ 2 ] [Nie, Songlin]Beijing Univ Technol, Beijing Key Lab Adv Mfg Technol, Beijing 100124, Peoples R China
  • [ 3 ] [Ji, Hui]Beijing Univ Technol, Beijing Key Lab Adv Mfg Technol, Beijing 100124, Peoples R China
  • [ 4 ] [Qin, Tingting]Beijing Univ Technol, Beijing Key Lab Adv Mfg Technol, Beijing 100124, Peoples R China
  • [ 5 ] [Ma, Zhonghai]Beijing Univ Technol, Beijing Key Lab Adv Mfg Technol, Beijing 100124, Peoples R China

Reprint Author's Address:

  • [Ji, Hui]Beijing Univ Technol, Beijing Key Lab Adv Mfg Technol, Beijing 100124, Peoples R China;;

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Source :

JOURNAL OF CLEANER PRODUCTION

ISSN: 0959-6526

Year: 2024

Volume: 467

1 1 . 1 0 0

JCR@2022

Cited Count:

WoS CC Cited Count: 2

SCOPUS Cited Count: 4

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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