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Author:

Li, Jing (Li, Jing.) | Wang, Xiaoting (Wang, Xiaoting.) | Ma, Yang (Ma, Yang.) | Han, Wei (Han, Wei.) | Li, Kexin (Li, Kexin.) | Li, Jingtao (Li, Jingtao.) | Wu, Yi (Wu, Yi.) | Zhao, Yuehui (Zhao, Yuehui.) | Yan, Tao (Yan, Tao.) | Liu, Xiu (Liu, Xiu.) | Shi, Haolin (Shi, Haolin.) | Chen, Xiaoqing (Chen, Xiaoqing.) | Zhang, Yongzhe (Zhang, Yongzhe.) (Scholars:张永哲)

Indexed by:

Scopus SCIE

Abstract:

Two-dimensional (2D) ferroelectric field-effect transistors (Fe-FETs) based on p-n junctions are the basic units of future neuromorphic hardware. The In2Se3 semiconductor with ferroelectric, photoelectric, and phase transition properties possesses great application potential for in-sensor computing, but its ferroelectric p-n junction (FePNJ) is not well investigated. Here, we present an optoelectronic synapse made of uniformly full-coverage alpha-In2Se3/WSe2 FePNJ, achieving ultralow-power classification recognition and multiscale signal processing. Using chemical vapor deposition (CVD), we can obtain beta '-In2Se3/WSe2 subferroelectric p-n junctions by direct growth on SiO2/Si substrate and alpha-In2Se3/WSe2 FePNJ by phase transition. Modulated by the synergistic effect of the polarization electric field and the built-in electric field, the FePNJ exhibits significantly enhanced and highly tunable synaptic effects (memory retention >2500 s and >8 multilevel current states under single optical/electrical pulses), along with power consumption down to atto-joule levels. Utilizing these photoelectric properties, we constructed an all-ferroelectric in-sensor reservoir computing system, comprising both reservoir and readout networks, achieving ultralow-power handwritten digit recognition. We also created a multiscale reservoir computing system through the gate-voltage-modulated relaxation time scale of the FePNJ, which can efficiently detect motions in the 1 to 100 km h(-1) speed range.

Keyword:

ferroelectric p-njunction multiscale signal processing optoelectronic synapse ultralow power chemical vapor deposition

Author Community:

  • [ 1 ] [Li, Jing]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 2 ] [Wang, Xiaoting]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 3 ] [Ma, Yang]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 4 ] [Li, Kexin]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 5 ] [Li, Jingtao]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 6 ] [Wu, Yi]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 7 ] [Zhao, Yuehui]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 8 ] [Yan, Tao]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 9 ] [Liu, Xiu]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 10 ] [Shi, Haolin]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 11 ] [Chen, Xiaoqing]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 12 ] [Zhang, Yongzhe]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China
  • [ 13 ] [Han, Wei]Hubei Univ, Sch Microelect, Hubei Key Lab Micronanoelect Mat & Devices, Minist Educ,Key Lab Intelligent Sensing Syst & Sec, Wuhan 430062, Peoples R China

Reprint Author's Address:

  • 张永哲

    [Wang, Xiaoting]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China;;[Zhang, Yongzhe]Beijing Univ Technol, Sch Informat Sci & Technol, Key Lab Optoelect Technol Educ, Beijing 100124, Peoples R China

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Source :

ACS NANO

ISSN: 1936-0851

Year: 2025

Issue: 13

Volume: 19

Page: 13220-13229

1 7 . 1 0 0

JCR@2022

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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