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Two-dimensional (2D) ferroelectric field-effect transistors (Fe-FETs) based on p-n junctions are the basic units of future neuromorphic hardware. The In2Se3 semiconductor with ferroelectric, photoelectric, and phase transition properties possesses great application potential for in-sensor computing, but its ferroelectric p-n junction (FePNJ) is not well investigated. Here, we present an optoelectronic synapse made of uniformly full-coverage alpha-In2Se3/WSe2 FePNJ, achieving ultralow-power classification recognition and multiscale signal processing. Using chemical vapor deposition (CVD), we can obtain beta '-In2Se3/WSe2 subferroelectric p-n junctions by direct growth on SiO2/Si substrate and alpha-In2Se3/WSe2 FePNJ by phase transition. Modulated by the synergistic effect of the polarization electric field and the built-in electric field, the FePNJ exhibits significantly enhanced and highly tunable synaptic effects (memory retention >2500 s and >8 multilevel current states under single optical/electrical pulses), along with power consumption down to atto-joule levels. Utilizing these photoelectric properties, we constructed an all-ferroelectric in-sensor reservoir computing system, comprising both reservoir and readout networks, achieving ultralow-power handwritten digit recognition. We also created a multiscale reservoir computing system through the gate-voltage-modulated relaxation time scale of the FePNJ, which can efficiently detect motions in the 1 to 100 km h(-1) speed range.
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ACS NANO
ISSN: 1936-0851
Year: 2025
Issue: 13
Volume: 19
Page: 13220-13229
1 7 . 1 0 0
JCR@2022
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ESI Highly Cited Papers on the List: 0 Unfold All
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Chinese Cited Count:
30 Days PV: 2
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