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Author:

Yang, Zhibo (Yang, Zhibo.) | Lin, Bingquan (Lin, Bingquan.) | Wang, Liyan (Wang, Liyan.) | Du, Jianyu (Du, Jianyu.) | Sun, Shishuai (Sun, Shishuai.)

Indexed by:

EI Scopus SCIE

Abstract:

Fabricating self-driven UV detection photodetectors based on PbI2 materials remains a challenging issue due to chemical disorder and Fermi-level pinning. Here, we propose a self-driven PbI2-based ultraviolet photodetector, in which metal electrodes and graphene are prefabricated and physically laminated onto PbI2. The self-driven photodetector demonstrates an ultrafast response time (rise: 3.76, fall: 3.81 mu s). Furthermore, the photodetector exhibits high responsivity (18.7 A/W), detectivity (1.56 x 10(11) Jones), and external quantum efficiency (6206%). The excellent performance is attributed to the clean metal-semiconductor interface and the asymmetric heterojunction, which lead to a more efficient and faster collection of photogenerated carriers. These results highlight the potential of PbI2 for high-speed UV detection and propose an effective approach for improving 2D material-based photodetectors.

Keyword:

PbI2 asymmetricheterojunction self-driven UV detector ultrafast response

Author Community:

  • [ 1 ] [Yang, Zhibo]Tianjin Univ Technol, Sch Sci, Tianjin Key Lab Quantum Opt & Intelligent Photon, Tianjin 300384, Peoples R China
  • [ 2 ] [Wang, Liyan]Tianjin Univ Technol, Sch Sci, Tianjin Key Lab Quantum Opt & Intelligent Photon, Tianjin 300384, Peoples R China
  • [ 3 ] [Du, Jianyu]Tianjin Univ Technol, Sch Sci, Tianjin Key Lab Quantum Opt & Intelligent Photon, Tianjin 300384, Peoples R China
  • [ 4 ] [Sun, Shishuai]Tianjin Univ Technol, Sch Sci, Tianjin Key Lab Quantum Opt & Intelligent Photon, Tianjin 300384, Peoples R China
  • [ 5 ] [Lin, Bingquan]Beijing Univ Technol, Beijing Key Lab Microstruct & Properties Solids, Beijing 100124, Peoples R China

Reprint Author's Address:

  • [Du, Jianyu]Tianjin Univ Technol, Sch Sci, Tianjin Key Lab Quantum Opt & Intelligent Photon, Tianjin 300384, Peoples R China;;[Sun, Shishuai]Tianjin Univ Technol, Sch Sci, Tianjin Key Lab Quantum Opt & Intelligent Photon, Tianjin 300384, Peoples R China

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Source :

ACS APPLIED ELECTRONIC MATERIALS

Year: 2025

Issue: 9

Volume: 7

Page: 4125-4132

4 . 7 0 0

JCR@2022

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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