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Author:

Tan, Huan (Tan, Huan.) | Zhang, Bin (Zhang, Bin.) | Wang, Guoyu (Wang, Guoyu.) | Chen, Yongjin (Chen, Yongjin.) | Shen, Xingchen (Shen, Xingchen.) | Guo, Lijie (Guo, Lijie.) | Han, Xiaodong (Han, Xiaodong.) (Scholars:韩晓东) | Lu, Xu (Lu, Xu.) | Zhou, Xiaoyuan (Zhou, Xiaoyuan.)

Indexed by:

EI Scopus SCIE

Abstract:

Thermoelectric semiconductors based on GeTe has been proved to be an important materials for converting waste heat into electricity. In this study, we demonstrate an enhancement of thermoelectric performance for p-type Ge0.9Sb0.1Te1+x by a unique melt spinning method combined with hot pressing (MS-HP), through which increased Seebeck coefficients and reduced thermal conductivities are achieved simultaneously. Moreover, the MS technique greatly gives rise to a variety of microstructures, such as the fine Ge precipitates, twins and nano-domains, all of which contribute to the significantly reduced thermal conductivities. Finally, the Ge0.9Sb0.1Te1.03 reaches a maximum zT value of similar to 1.9 at 760 K and a giant average zT of similar to 1.2 between 300 K and 820 K, which is comparable to the reported results for GeTe based materials. Combined with the rapid fabrication, Ge-0.9Sb0.1Te1+x prepared by melt spinning process is an attractive p-type material for thermoelectric power generation application. (C) 2018 Published by Elsevier B.V.

Keyword:

Thermoelectric properties Thermal conductivity GeTe Rapid fabrication Hierarchical microstructure

Author Community:

  • [ 1 ] [Tan, Huan]Chongqing Univ, Coll Phys, Chongqing Key Lab Soft Condensed Matter Phys & Sm, Chongqing 400044, Peoples R China
  • [ 2 ] [Shen, Xingchen]Chongqing Univ, Coll Phys, Chongqing Key Lab Soft Condensed Matter Phys & Sm, Chongqing 400044, Peoples R China
  • [ 3 ] [Guo, Lijie]Chongqing Univ, Coll Phys, Chongqing Key Lab Soft Condensed Matter Phys & Sm, Chongqing 400044, Peoples R China
  • [ 4 ] [Lu, Xu]Chongqing Univ, Coll Phys, Chongqing Key Lab Soft Condensed Matter Phys & Sm, Chongqing 400044, Peoples R China
  • [ 5 ] [Zhou, Xiaoyuan]Chongqing Univ, Coll Phys, Chongqing Key Lab Soft Condensed Matter Phys & Sm, Chongqing 400044, Peoples R China
  • [ 6 ] [Zhang, Bin]Chongqing Univ, Analyt & Testing Ctr, Chongqing 401331, Peoples R China
  • [ 7 ] [Zhou, Xiaoyuan]Chongqing Univ, Analyt & Testing Ctr, Chongqing 401331, Peoples R China
  • [ 8 ] [Wang, Guoyu]Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China
  • [ 9 ] [Shen, Xingchen]Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China
  • [ 10 ] [Wang, Guoyu]China & Univ Chinese Acad Sci, Beijing 100044, Peoples R China
  • [ 11 ] [Shen, Xingchen]China & Univ Chinese Acad Sci, Beijing 100044, Peoples R China
  • [ 12 ] [Chen, Yongjin]Beijing Univ Technol, Beijing Key Lab, Beijing 100124, Peoples R China
  • [ 13 ] [Han, Xiaodong]Beijing Univ Technol, Beijing Key Lab, Beijing 100124, Peoples R China
  • [ 14 ] [Chen, Yongjin]Beijing Univ Technol, Inst Microstruct & Property Adv Mat, Beijing 100124, Peoples R China
  • [ 15 ] [Han, Xiaodong]Beijing Univ Technol, Inst Microstruct & Property Adv Mat, Beijing 100124, Peoples R China

Reprint Author's Address:

  • [Lu, Xu]Chongqing Univ, Coll Phys, Chongqing Key Lab Soft Condensed Matter Phys & Sm, Chongqing 400044, Peoples R China;;[Zhou, Xiaoyuan]Chongqing Univ, Coll Phys, Chongqing Key Lab Soft Condensed Matter Phys & Sm, Chongqing 400044, Peoples R China

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Source :

JOURNAL OF ALLOYS AND COMPOUNDS

ISSN: 0925-8388

Year: 2019

Volume: 774

Page: 129-136

6 . 2 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:211

JCR Journal Grade:2

Cited Count:

WoS CC Cited Count: 18

SCOPUS Cited Count: 18

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 5

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