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Author:

Du, Peng (Du, Peng.) | Wang, Ruyue (Wang, Ruyue.) | Deng, Bohan (Deng, Bohan.) | He, Xian (He, Xian.) | Long, Yuanzheng (Long, Yuanzheng.) | Yang, Cheng (Yang, Cheng.) | Wang, Zhiwei (Wang, Zhiwei.) | Ge, Binghui (Ge, Binghui.) | Huang, Kai (Huang, Kai.) | Zhang, Ru (Zhang, Ru.) | Lei, Ming (Lei, Ming.) | Wu, Hui (Wu, Hui.)

Indexed by:

EI Scopus SCIE

Abstract:

The running of environmental purification usually employs massive consumption of energy, and it is of signif-icant scientific importance and real impact to reduce the energy cost in environmental treatments. In particular, it is urgently required to minimalize the energy cost of the catalytic oxidation of gaseous pollutants represented by volatile organic compounds (VOCs). Herein, we develop a rapid in-situ Joule-heating configuration to drive the catalytic VOCs oxidation with ultra-low energy consumption. As a prototypical illustration, atomically dispersed Pt/CeO2 catalyst was decorated on conductive Nickle foam substrate to act as both catalytic and electric components with minimal pressure drop and high compatibility. The catalytic system exhibited 100% conversion toward toluene (1000 ppm, 33 mL min-1) with an ultralow input power of 6.5 W, which was 87% lower than that of a conventional heating furnace. Moreover, the long-term stability, high universality for various VOCs, and responsiveness for real-time changing components were also demonstrated. The outstanding electro-thermal properties of the system can be extended to more gaseous catalytic reactions with much lower energy consumption.

Keyword:

Catalytic oxidation Environmental treatment VOCs decomposition Energy-saving

Author Community:

  • [ 1 ] [Du, Peng]Beijing Univ Posts & Telecommun, Sch Sci, State Key Lab Informat Photon & Opt Commun, Beijing 100876, Peoples R China
  • [ 2 ] [Wang, Ruyue]Beijing Univ Posts & Telecommun, Sch Sci, State Key Lab Informat Photon & Opt Commun, Beijing 100876, Peoples R China
  • [ 3 ] [He, Xian]Beijing Univ Posts & Telecommun, Sch Sci, State Key Lab Informat Photon & Opt Commun, Beijing 100876, Peoples R China
  • [ 4 ] [Huang, Kai]Beijing Univ Posts & Telecommun, Sch Sci, State Key Lab Informat Photon & Opt Commun, Beijing 100876, Peoples R China
  • [ 5 ] [Zhang, Ru]Beijing Univ Posts & Telecommun, Sch Sci, State Key Lab Informat Photon & Opt Commun, Beijing 100876, Peoples R China
  • [ 6 ] [Lei, Ming]Beijing Univ Posts & Telecommun, Sch Sci, State Key Lab Informat Photon & Opt Commun, Beijing 100876, Peoples R China
  • [ 7 ] [Du, Peng]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 8 ] [Wang, Ruyue]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 9 ] [Deng, Bohan]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 10 ] [He, Xian]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 11 ] [Long, Yuanzheng]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 12 ] [Yang, Cheng]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 13 ] [Wu, Hui]Tsinghua Univ, Sch Mat Sci & Engn, State Key Lab New Ceram & Fine Proc, Beijing 100084, Peoples R China
  • [ 14 ] [Du, Peng]Beijing Univ Posts & Telecommun BUPT, Beijing Key Lab Space ground Interconnect & Conver, Xitucheng Rd 10, Beijing 100876, Peoples R China
  • [ 15 ] [Wang, Ruyue]Beijing Univ Posts & Telecommun BUPT, Beijing Key Lab Space ground Interconnect & Conver, Xitucheng Rd 10, Beijing 100876, Peoples R China
  • [ 16 ] [Wang, Zhiwei]Beijing Univ Technol, Ctr Excellence Environm Safety & Biol Effects, Key Lab Beijing Reg Air Pollut Control, Beijing Key Lab Green Catalysis & Separat, Beijing 100124, Peoples R China
  • [ 17 ] [Ge, Binghui]Anhui Univ, Inst Phys Sci & Informat Technol, Hefei 230601, Peoples R China

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Source :

NANO ENERGY

ISSN: 2211-2855

Year: 2022

Volume: 102

1 7 . 6

JCR@2022

1 7 . 6 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:66

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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