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Author:

Yu, Lichao (Yu, Lichao.) | Lu, Qingmei (Lu, Qingmei.) | Cong, Liying (Cong, Liying.) | Yang, Xinyuan (Yang, Xinyuan.) | Liu, Weiqiang (Liu, Weiqiang.) | Dong, Gaihua (Dong, Gaihua.) | Huang, Shulin (Huang, Shulin.) | Deng, Yuan (Deng, Yuan.) | Meng, Lijuan (Meng, Lijuan.) | Liu, Youhao (Liu, Youhao.) | Yi, Xiaofei (Yi, Xiaofei.) | Wu, Yufeng (Wu, Yufeng.) | Yue, Ming (Yue, Ming.)

Indexed by:

EI Scopus SCIE

Abstract:

In this work, single-phase spherical Nd-Fe-B regenerated single crystals powder (SRP) was recycled via calcium reduction method from sintered Nd-Fe-B (S-NdFeB) sludge, followed by blending with high remanence alloy (HRA) and Pr-rich alloy at varying weight ratios from 45 % to 85 % for fabricating regenerated magnets (RM). We conducted a series of analyses of phases, microstructures, magnetic performance, and magnetization reversal behaviors on the RM samples, expounding the SRP proportion impacts and the magnetic recovery mechanism. With the increasing SRP proportion, the comprehensive magnetic performance exhibits a trend of initially raising and then decreasing, reaching a summit for magnet RM-65 %. Br, (BH)max and the squareness (Hk/Hcj) are well recovered to 103.8 %, 104.5 %, and 102.2 % of the original magnet, respectively due to the high orientation induced by SRP, the high Br from HRA alloy, and uniform grain size. Hcj is recovered to 73.1 % with a satisfying value exceeding 15 kOe. The introduction of Pr-rich alloy facilitates the formation of thin, continuous grain boundaries, enhancing the magnetic isolation effect between the main phase grains; on the other hand, the Pr-rich-shell structure with high anisotropic field, and the chemical heterogeneity of the multiple main phase grains, improve the nucleation field of the reversed domain, contributing to the high Hcj together. © 2024

Keyword:

Praseodymium alloys Remanence Neodymium alloys Magnetization reversal Sintering Crystal orientation Grain boundaries Iron alloys

Author Community:

  • [ 1 ] [Yu, Lichao]College of Materials and Engineering, Key Laboratory of Advanced Functional Materials, Ministry of Education of China, Beijing University of Technology, Beijing; 100124, China
  • [ 2 ] [Lu, Qingmei]College of Materials and Engineering, Key Laboratory of Advanced Functional Materials, Ministry of Education of China, Beijing University of Technology, Beijing; 100124, China
  • [ 3 ] [Lu, Qingmei]State Key Laboratory of Rare Earth Permanent Magnetic Materials, China
  • [ 4 ] [Cong, Liying]College of Materials and Engineering, Key Laboratory of Advanced Functional Materials, Ministry of Education of China, Beijing University of Technology, Beijing; 100124, China
  • [ 5 ] [Yang, Xinyuan]College of Materials and Engineering, Key Laboratory of Advanced Functional Materials, Ministry of Education of China, Beijing University of Technology, Beijing; 100124, China
  • [ 6 ] [Liu, Weiqiang]College of Materials and Engineering, Key Laboratory of Advanced Functional Materials, Ministry of Education of China, Beijing University of Technology, Beijing; 100124, China
  • [ 7 ] [Liu, Weiqiang]State Key Laboratory of Rare Earth Permanent Magnetic Materials, China
  • [ 8 ] [Dong, Gaihua]Baotou Inst Magnetic New Material Co., Ltd., Inner Mongolia, Baotou; 014030, China
  • [ 9 ] [Huang, Shulin]Baotou Inst Magnetic New Material Co., Ltd., Inner Mongolia, Baotou; 014030, China
  • [ 10 ] [Deng, Yuan]Inner Mongolia Rare Earth Functional Materials Innovation Center Co., Ltd., Inner Mongolia, Baotou; 014030, China
  • [ 11 ] [Meng, Lijuan]Inner Mongolia Rare Earth Functional Materials Innovation Center Co., Ltd., Inner Mongolia, Baotou; 014030, China
  • [ 12 ] [Liu, Youhao]Earth-Panda Advanced Magnetic Materials Co., Ltd., Lujiang County, Anhui, Hefei; 231500, China
  • [ 13 ] [Liu, Youhao]State Key Laboratory of Rare Earth Permanent Magnetic Materials, China
  • [ 14 ] [Yi, Xiaofei]Earth-Panda Advanced Magnetic Materials Co., Ltd., Lujiang County, Anhui, Hefei; 231500, China
  • [ 15 ] [Yi, Xiaofei]State Key Laboratory of Rare Earth Permanent Magnetic Materials, China
  • [ 16 ] [Wu, Yufeng]College of Materials and Engineering, Key Laboratory of Advanced Functional Materials, Ministry of Education of China, Beijing University of Technology, Beijing; 100124, China
  • [ 17 ] [Yue, Ming]College of Materials and Engineering, Key Laboratory of Advanced Functional Materials, Ministry of Education of China, Beijing University of Technology, Beijing; 100124, China
  • [ 18 ] [Yue, Ming]State Key Laboratory of Rare Earth Permanent Magnetic Materials, China

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Source :

Sustainable Materials and Technologies

ISSN: 2214-9929

Year: 2025

Volume: 43

9 . 6 0 0

JCR@2022

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 11

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