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Abstract:
A catalytic reverse flow reactor was employed for the combustion of lean carbon monoxide in air mixture. The catalytic combustion of CO over a Pd mixed oxide supported on cordierite coated with Ce/La was investigated. The catalysts were prepared using a sol-gel method and characterized using BET and SEM. The effects of Pd content, preheated temperature, calcination temperature and calcination time on catalyst performance were studied. Furthermore, the performances of the reactor such as pressure drop and bed temperature distribution were investigated. The catalysts calcined at 550 degrees C for 3 h with Pd content being 2.5 wt% exhibited the highest catalytic activity. The conversion attained 90% when the switch time was 8 min, the GHSV was 8000h(-1), and the initial concentration was 100ppm. The pressure drop of the system was small when the GHSV was lower than 10000h(-1). The initial preheating temperature of the catalyst had a greater influence on the temperature distribution in the reactor.
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FRESENIUS ENVIRONMENTAL BULLETIN
ISSN: 1018-4619
Year: 2018
Issue: 12
Volume: 27
Page: 8297-8307
ESI Discipline: ENVIRONMENT/ECOLOGY;
ESI HC Threshold:203
JCR Journal Grade:4
Cited Count:
WoS CC Cited Count: 0
SCOPUS Cited Count:
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 12
Affiliated Colleges: