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Author:

Zhang, Yiwei (Zhang, Yiwei.) | Zhang, Baohuan (Zhang, Baohuan.) | Fu, Yulan (Fu, Yulan.) | Dou, Fei (Dou, Fei.) | Guo, Jinxin (Guo, Jinxin.) | Zhang, Xinping (Zhang, Xinping.) (Scholars:张新平)

Indexed by:

EI Scopus SCIE

Abstract:

The application of halide perovskite materials as lasing devices has recently attracted great attention. However, the instability of such materials against moisture significantly restrict the application in many occasions. In order to protect the unstable perovskite materials against oxygen and moisture, various encapsulation strategies have been proposed. Regrettably, few of them are designed for aqueous envi-ronments. Herein, we demonstrate a photo-polymerized acrylic acid (ADCP) acting as substrate and encapsulation layer to fabricate (CH3NH3)PbBr3 (MAPbBr(3)) films and realize amplified spontaneous emission (ASE) with low threshold in water. Lasing threshold from MAPbBr(3) films sandwiched by ADCP decreases slightly from 12 mJ/cm(2) in air to ~9 mJ/cm(2) in water. The specific morphology, superb wettability and high-water stability are expected to contribute to the low ASE threshold. The aqueous environment with higher refractive index is speculated to be one of the origins of the slightly lower ASE threshold. Our results demonstrate a strong potential for applications of perovskite materials in lasing devices in aqueous environment and a new path to realize low threshold lasing. (C)& nbsp;2022 Elsevier Ltd. All rights reserved.

Keyword:

Nano crystals Low threshold Photopolymer MAPbBr(3) Encapsulation

Author Community:

  • [ 1 ] [Zhang, Yiwei]Beijing Univ Technol, Inst Informat Photon Technol, Fac Sci, Beijing 100124, Peoples R China
  • [ 2 ] [Zhang, Baohuan]Beijing Univ Technol, Inst Informat Photon Technol, Fac Sci, Beijing 100124, Peoples R China
  • [ 3 ] [Fu, Yulan]Beijing Univ Technol, Inst Informat Photon Technol, Fac Sci, Beijing 100124, Peoples R China
  • [ 4 ] [Dou, Fei]Beijing Univ Technol, Inst Informat Photon Technol, Fac Sci, Beijing 100124, Peoples R China
  • [ 5 ] [Guo, Jinxin]Beijing Univ Technol, Inst Informat Photon Technol, Fac Sci, Beijing 100124, Peoples R China
  • [ 6 ] [Zhang, Xinping]Beijing Univ Technol, Inst Informat Photon Technol, Fac Sci, Beijing 100124, Peoples R China

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Source :

MATERIALS TODAY PHYSICS

ISSN: 2542-5293

Year: 2022

Volume: 24

1 1 . 5

JCR@2022

1 1 . 5 0 0

JCR@2022

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 1

SCOPUS Cited Count: 1

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 8

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