The　coassembly　of　primary　particles　into　heterostructures　represents　a　significant　strategy　for　advanced　fabrication　of　multi-functional　materials　or　devices,　and　templated　assembly　has　shown　remarkable　advantage　for　deterministic　placement　of　particles　and　the　efficient　integration　with　substrates.　However,　template　induced　particles　coassembly,　which　is　significant　for　integrating　multicomponents　at　desired　positions,　is　still　challenging.　Herein,　a　facile　strategy　of　embossed　templateinduced　particles　coassembly　for　diverse　superstructures　and　precise　patterns　is　reported.　Tunable　region　selective　assembly　of　particles　is　demonstrated　by　controlling　the　resistance　force　via　designing　the　embossed　edge　and　surface　roughness　of　the　template.　Through　regulating　the　template　morphologies　and　particles　composition,　well-controlled　coassembly　of　＂flower＂　shaped　heterostructure　and　chiral　superstructure　arrays　are　realized.　Furthermore,　the　printable　nanomaterials　self-assembly　template　is　employed　to　achieve　totally　bottom-up　fabrication　of　excitation　responsive　heterostructure　arrays,　in　which　the　multi-photons　process　based　energy　transfer　is　studied　to　show　the　application　in　high-secure　encryption.　With　the　advantage　of　accurate　position　and　compatible　to　different　materials,　this　strategy　is　expected　to　provide　a　promising　platform　for　fabricating　micro/nanoscale　advanced　devices.