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Author:

Yang, Lixue (Yang, Lixue.) | Li, Lin (Li, Lin.) | Wang, Qiang (Wang, Qiang.) | Xing, Cheng (Xing, Cheng.) | Ma, Lin (Ma, Lin.) | Zeng, Yong (Zeng, Yong.) | Zhao, Yan (Zhao, Yan.) (Scholars:赵艳) | Yan, Yinzhou (Yan, Yinzhou.) (Scholars:闫胤洲)

Indexed by:

EI Scopus SCIE

Abstract:

The development of quantum dot (QD) composite films for lighting and displays is of great importance because of their exceptional mechanical flexibility, chemical stability, and optical tunability. Generally, QDs are attached to plasmonic nanostructures to enhance their photoluminescence (PL) emission. However, plasmonic QD composite films suffer from deteriorated inherent quantum yields and lower enhancement ratios due to variations in the refractive index and dielectricity in the composites. Herein, the use of a dielectric microsphere cavity is reported to realize over 1000-fold enhancement of the PL in CdSe/ZnS QD/polydimethylsiloxane films with a highly unidirectional emission angle of approximate to 9 degrees. The field regulation by the optical whispering-gallery resonance and directional antenna effect at the microscale is revealed to interpret the PL enhancement mechanism. Additionally, the microsphere cavity allows for the enhancement of white-light emission in the RGB-QD hybrid composite film. The present work inspires a straightforward strategy for boosting the light efficiency in QD composite films, with promising applications in flexible lighting/display devices.

Keyword:

whispering-gallery mode microsphere cavity unidirectional emission photoluminescence enhancement quantum dots

Author Community:

  • [ 1 ] [Yang, Lixue]Beijing Univ Technol, Inst Laser Engn, Beijing 100124, Peoples R China
  • [ 2 ] [Wang, Qiang]Beijing Univ Technol, Inst Laser Engn, Beijing 100124, Peoples R China
  • [ 3 ] [Xing, Cheng]Beijing Univ Technol, Inst Laser Engn, Beijing 100124, Peoples R China
  • [ 4 ] [Zhao, Yan]Beijing Univ Technol, Inst Laser Engn, Beijing 100124, Peoples R China
  • [ 5 ] [Yan, Yinzhou]Beijing Univ Technol, Inst Laser Engn, Beijing 100124, Peoples R China
  • [ 6 ] [Li, Lin]Univ Manchester, Sch Mech Aerosp & Civil Engn, Laser Proc Res Ctr, Manchester M13 9PL, Lancs, England
  • [ 7 ] [Ma, Lin]Beijing Univ Technol, Inst Microstruct & Property Adv Mat, Beijing 100124, Peoples R China
  • [ 8 ] [Zeng, Yong]Beijing Univ Technol, Beijing Engn Res Ctr Printing Digital Med Hlth 3D, Beijing 100124, Peoples R China
  • [ 9 ] [Zhao, Yan]Beijing Univ Technol, Beijing Engn Res Ctr Laser Technol, Beijing 100124, Peoples R China
  • [ 10 ] [Yan, Yinzhou]Beijing Univ Technol, Beijing Engn Res Ctr Laser Technol, Beijing 100124, Peoples R China
  • [ 11 ] [Zhao, Yan]Beijing Univ Technol, Key Lab Trans Scale Laser Mfg, Minist Educ, Beijing 100124, Peoples R China
  • [ 12 ] [Yan, Yinzhou]Beijing Univ Technol, Key Lab Trans Scale Laser Mfg, Minist Educ, Beijing 100124, Peoples R China

Reprint Author's Address:

  • 闫胤洲

    [Yan, Yinzhou]Beijing Univ Technol, Inst Laser Engn, Beijing 100124, Peoples R China;;[Yan, Yinzhou]Beijing Univ Technol, Beijing Engn Res Ctr Laser Technol, Beijing 100124, Peoples R China;;[Yan, Yinzhou]Beijing Univ Technol, Key Lab Trans Scale Laser Mfg, Minist Educ, Beijing 100124, Peoples R China

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Source :

ADVANCED OPTICAL MATERIALS

ISSN: 2195-1071

Year: 2019

Issue: 24

Volume: 7

9 . 0 0 0

JCR@2022

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:211

JCR Journal Grade:1

Cited Count:

WoS CC Cited Count: 19

SCOPUS Cited Count: 23

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 7

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