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Fabricating self-driven UV detection photodetectors based on PbI2 materials remains a challenging issue due to chemical disorder and Fermi-level pinning. Here, we propose a self-driven PbI2-based ultraviolet photodetector, in which metal electrodes and graphene are prefabricated and physically laminated onto PbI2. The self-driven photodetector demonstrates an ultrafast response time (rise: 3.76, fall: 3.81 μs). Furthermore, the photodetector exhibits high responsivity (18.7 A/W), detectivity (1.56 × 1011 Jones), and external quantum efficiency (6206%). The excellent performance is attributed to the clean metal-semiconductor interface and the asymmetric heterojunction, which lead to a more efficient and faster collection of photogenerated carriers. These results highlight the potential of PbI2 for high-speed UV detection and propose an effective approach for improving 2D material-based photodetectors. © 2025 American Chemical Society.
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ACS Applied Electronic Materials
ISSN: 2637-6113
Year: 2025
Issue: 9
Volume: 7
Page: 4125-4132
4 . 7 0 0
JCR@2022
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ESI Highly Cited Papers on the List: 0 Unfold All
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30 Days PV: 3
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