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Author:

Yang, Z. (Yang, Z..) | Lin, B. (Lin, B..) | Wang, L. (Wang, L..) | Du, J. (Du, J..) | Sun, S. (Sun, S..)

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Scopus

Abstract:

Fabricating self-driven UV detection photodetectors based on PbI2 materials remains a challenging issue due to chemical disorder and Fermi-level pinning. Here, we propose a self-driven PbI2-based ultraviolet photodetector, in which metal electrodes and graphene are prefabricated and physically laminated onto PbI2. The self-driven photodetector demonstrates an ultrafast response time (rise: 3.76, fall: 3.81 μs). Furthermore, the photodetector exhibits high responsivity (18.7 A/W), detectivity (1.56 × 1011 Jones), and external quantum efficiency (6206%). The excellent performance is attributed to the clean metal-semiconductor interface and the asymmetric heterojunction, which lead to a more efficient and faster collection of photogenerated carriers. These results highlight the potential of PbI2 for high-speed UV detection and propose an effective approach for improving 2D material-based photodetectors. © 2025 American Chemical Society.

Keyword:

asymmetric heterojunction PbI2 self-driven ultrafast response UV detector

Author Community:

  • [ 1 ] [Yang Z.]Tianjin Key Laboratory of Quantum Optics and Intelligent Photonics, School of Science, Tianjin University of Technology, Tianjin, 300384, China
  • [ 2 ] [Lin B.]Beijing Key Laboratory of Microstructure and Properties of Solids, Beijing University of Technology, Beijing, 100124, China
  • [ 3 ] [Wang L.]Tianjin Key Laboratory of Quantum Optics and Intelligent Photonics, School of Science, Tianjin University of Technology, Tianjin, 300384, China
  • [ 4 ] [Du J.]Tianjin Key Laboratory of Quantum Optics and Intelligent Photonics, School of Science, Tianjin University of Technology, Tianjin, 300384, China
  • [ 5 ] [Sun S.]Tianjin Key Laboratory of Quantum Optics and Intelligent Photonics, School of Science, Tianjin University of Technology, Tianjin, 300384, China

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Source :

ACS Applied Electronic Materials

ISSN: 2637-6113

Year: 2025

Issue: 9

Volume: 7

Page: 4125-4132

4 . 7 0 0

JCR@2022

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 3

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